Beschreibung: Changes in the emission, transport and deposition of aeolian dust have profound effects on regional climate, so that characterizing the lifecycle of dust in observations and improving the representation of dust in global climate models is necessary. A fundamental aspect of characterizing the dust cycle is quantifying surface dust fluxes, yet no spatially explicit estimates of this flux exist for the World's major source regions. Here we present a novel technique for creating a map of the annual mean emitted dust flux for North Africa based on retrievals of dust storm frequency from the Meteosat Second Generation Spinning Enhanced Visible and InfraRed Imager (SEVIRI) and the relationship between dust storm frequency and emitted mass flux derived from the output of five models that simulate dust. Our results suggest that 64 (±16)% of all dust emitted from North Africa is from the Bodélé depression, and that 13 (±3)% of the North African dust flux is from a depression lying in the lee of the Aïr and Hoggar Mountains, making this area the second most important region of emission within North Africa.

Beschreibung: Sammlung von atmosphärischen Referenzmessungen über Ozeanen (CARO)

Beschreibung: Meso-α/β/γ scale atmospheric processes of jet dynamics responsible for generating Harmattan, Saudi Arabian, and Bodélé Depression dust storms are analyzed with observations and high-resolution modeling. The analysis of the role of jet adjustment processes in each dust storm shows similarities as follows: (1) the presence of a well-organized baroclinic synoptic scale system, (2) cross mountain flows that produced a leeside inversion layer prior to the large-scale dust storm, (3) the presence of thermal wind imbalance in the exit region of the midtropospheric jet streak in the lee of the respective mountains shortly after the time of the inversion formation, (4) dust storm formation accompanied by large magnitude ageostrophic isallobaric low-level winds as part of the meso-β scale adjustment process, (5) substantial low-level turbulence kinetic energy (TKE), and (6) emission and uplift of mineral dust in the lee of nearby mountains. The thermally forced meso-γ scale adjustment processes, which occurred in the canyons/small valleys, may have been the cause of numerous observed dust streaks leading to the entry of the dust into the atmosphere due to the presence of significant vertical motion and TKE generation. This study points to the importance of meso-β to meso-γ scale adjustment processes at low atmospheric levels due to an imbalance within the exit region of an upper level jet streak for the formation of severe dust storms. The low level TKE, which is one of the prerequisites to deflate the dust from the surface, cannot be detected with the low resolution data sets; so our results show that a high spatial resolution is required for better representing TKE as a proxy for dust emission. Key Points: - Thermal wind imbalance in the exit region of the jet streak resulted in a mesoscale jetlet in the lee of the mountains - Thermally direct transverse ageostrophic circulation in the exit region of the jetlet led to the upward motion and adiabatic expansion - Low-level pressure rise generated the ageostrophic isallobaric wind that advected cold air toward the thermally induced low pressure area

Beschreibung: We present the first forcing interpretation of the future anthropogenic aerosol scenarios of CMIP6 with the simple plumes parameterisation MACv2-SP. The nine scenarios for 2015 to 2100 are based on anthropogenic aerosol emissions for use in CMIP6 (Riahi et al., 2017; Gidden et al., 2018). We use the emissions to scale the observationally informed anthropogenic aerosol optical properties and the associated effect on the cloud albedo of present-day (Fiedler et al., 2017; Stevens et al., 2017) into the future. The resulting scenarios in MACv2-SP are then ranked according to their strength in forcing magnitude and spatial asymmetries for anthropogenic aerosol. All scenarios, except SSP3-70 and SSP4-60, show a decrease in anthropogenic aerosol by 2100 with a range from 108 % to 36 % of the anthropogenic aerosol optical depth in 2015. We estimate the radiative forcing of anthropogenic aerosol from high- and low-end scenarios in the mid-2090s by performing ensembles of simulations with the atmosphere-only configuration of MPI-ESM1.2. MACv2-SP translates the CMIP6 emission scenarios for inducing anthropogenic aerosol forcing. With the implementation in our model, we obtain forcing estimates for both the shortwave instantaneous radiative forcing (RF) and the effective radiative forcing (ERF) of anthropogenic aerosol relative to 1850. Here, ERF accounts for rapid atmospheric adjustments and natural variability internal to the model. The ERF of anthropogenic aerosol for the mid-2090s ranges from −0.15 W m−2 for SSP1-19 to −0.54 W m−2 for SSP3-70, i.e. the mid-2090s ERF is 30 %–108 % of the value in the mid-2000s due to differences in the emission pathway alone. Assuming a stronger Twomey effect changes these ERFs to −0.39 and −0.92 W m−2, respectively, which are similar to estimates obtained from models with complex aerosol parameterisations. The year-to-year standard deviations around 0.3 W m−2 associated with natural variability highlight the necessity to average over sufficiently long time periods for estimating ERF; this is in contrast to RF that is typically well constrained after simulating just 1 year. The scenario interpretation of MACv2-SP will be used within the framework of CMIP6 and other cutting-edge scientific endeavours.

Beschreibung: This study assesses the change in anthropogenic aerosol forcing from the mid-1970s to the mid-2000s. Both decades had similar global-mean anthropogenic aerosol optical depths but substantially different global distributions. For both years, we quantify (i) the forcing spread due to model-internal variability and (ii) the forcing spread among models. Our assessment is based on new ensembles of atmosphere-only simulations with five state-of-the-art Earth system models. Four of these models will be used in the sixth Coupled Model Intercomparison Project (CMIP6; Eyring et al., 2016). Here, the complexity of the anthropogenic aerosol has been reduced in the participating models. In all our simulations, we prescribe the same patterns of the anthropogenic aerosol optical properties and associated effects on the cloud droplet number concentration. We calculate the instantaneous radiative forcing (RF) and the effective radiative forcing (ERF). Their difference defines the net contribution from rapid adjustments. Our simulations show a model spread in ERF from −0.4 to −0.9 W m−2. The standard deviation in annual ERF is 0.3 W m−2, based on 180 individual estimates from each participating model. This result implies that identifying the model spread in ERF due to systematic differences requires averaging over a sufficiently large number of years. Moreover, we find almost identical ERFs for the mid-1970s and mid-2000s for individual models, although there are major model differences in natural aerosols and clouds. The model-ensemble mean ERF is −0.54 W m−2 for the pre-industrial era to the mid-1970s and −0.59 W m−2 for the pre-industrial era to the mid-2000s. Our result suggests that comparing ERF changes between two observable periods rather than absolute magnitudes relative to a poorly constrained pre-industrial state might provide a better test for a model's ability to represent transient climate changes.

Beschreibung: ICON-A is the new icosahedral nonhydrostatic (ICON) atmospheric general circulation model in a configuration using the Max Planck Institute physics package, which originates from the ECHAM6 general circulation model, and has been adapted to account for the changed dynamical core framework. The coupling scheme between dynamics and physics employs a sequential updating by dynamics and physics, and a fixed sequence of the physical processes similar to ECHAM6. To allow a meaningful initial comparison between ICON-A and the established ECHAM6-LR model, a setup with similar, low resolution in terms of number of grid points and levels is chosen. The ICON-A model is tuned on the base of the Atmospheric Model Intercomparison Project (AMIP) experiment aiming primarily at a well balanced top-of atmosphere energy budget to make the model suitable for coupled climate and Earth system modeling. The tuning addresses first the moisture and cloud distribution to achieve the top-of-atmosphere energy balance, followed by the tuning of the parameterized dynamic drag aiming at reduced wind errors in the troposphere. The resulting version of ICON-A has overall biases, which are comparable to those of ECHAM6. Problematic specific biases remain in the vertical distribution of clouds and in the stratospheric circulation, where the winter vortices are too weak. Biases in precipitable water and tropospheric temperature are, however, reduced compared to the ECHAM6. ICON-A will serve as the basis of further development and as the atmosphere component to the coupled model, ICON-Earth system model (ESM). Key Points: - Physics package for climate modeling is coupled to a nonhydrostatic dynamical core - Tuning in five steps to obtain a balanced net radiation at top of atmosphere - Overall biases of ICON-A are comparable to ECHAM6.3, but circulation biases remain due to problems with parameterized drag

Beschreibung: Dust aerosol is important in the Earth system, but the relative impact of meteorological mechanisms on North African dust emission remains unclear. This study presents the first climatology of dust emission amounts associated with Harmattan surges (HSs), characterized by postfrontal strengthening of near-surface winds. A new automated identification uses their strong isallobaric winds as an indicator for HSs in 32 years of ERA-Interim reanalysis. Their impact on dust aerosol emission is estimated by combining the identified events with derived dust emissions. The estimate highlights that about one third of the total emission mass is associated with HSs. Spring shows the largest associated emissions of 30–50% of the monthly totals consistent with the largest number and duration of HSs. Regional emission contributions of up to 80% in the north coincide with the overall largest emission maxima in spring. The importance of HSs for dust emission implies that aerosol-climate models need to accurately represent synoptic-scale storms. Key Points: - First climatology of North African dust emission mass linked with Harmattan surges (HSs) - One third of total emission linked to HSs annually and spatially averaged - Regionally up to 80% of springtime maximum in emission mass is associated with HSs

Beschreibung: We performed detailed mesoscale observational analyses and Weather Research and Forecasting (WRF) model simulations to study the terrain-induced downslope winds that generated dust-emitting winds at the beginning of three strong subtropical dust storms in three distinctly different regions of North Africa and the Arabian Peninsula. We revisit the Harmattan dust storm of 2 March 2004, the Saudi dust storm of 9 March 2009, and the Bodélé Depression dust storm of 8 December 2011 and use high-resolution WRF modeling to assess the dynamical processes during the onset of the storms in more depth. Our results highlight the generation of terrain-induced downslope winds in response to the transition of the atmospheric flow from a subcritical to supercritical state in all three cases. These events precede the unbalanced adjustment processes in the lee of the mountain ranges that produced larger-scale dust aerosol mobilization and transport. We see that only the higher-resolution data sets can resolve the mesoscale processes, which are mainly responsible for creating strong low-level terrain-induced downslope winds leading to the initial dust storms. Key Points: - Downslope winds resulted in strong low-level vertical wind shear, which interacted with the development of near-surface positively buoyant air during the morning and generated significant turbulence kinetic energy - The strong and gusty winds caused moderate meso-γ- to β-scale dust storms as an early stage of precursor to later severe dust storms that affected large areas

Beschreibung: Kretzschmar et al., in a comment in 2017, use the spread in the output of aerosol–climate models to argue that the models refute the hypothesis (presented in a paper by Stevens in 2015) that for the mid-twentieth-century warming to be consistent with observations, then the present-day aerosol forcing, must be less negative than −1 W m−2. The main point of contention is the nature of the relationship between global SO2 emissions and In contrast to the concave (log-linear) relationship used by Stevens and in earlier studies, whereby becomes progressively less sensitive to SO2 emissions, some models suggest a convex relationship, which would imply a less negative lower bound. The model that best exemplifies this difference, and that is most clearly in conflict with the hypothesis of Stevens, does so because of an implausible aerosol response to the initial rise in anthropogenic aerosol precursor emissions in East and South Asia—already in 1975 this model’s clear-sky reflectance from anthropogenic aerosol over the North Pacific exceeds present-day estimates of the clear-sky reflectance by the total aerosol. The authors perform experiments using a new (observationally constrained) climatology of anthropogenic aerosols to further show that the effects of changing patterns of aerosol and aerosol precursor emissions during the late twentieth century have, for the same global emissions, relatively little effect on These findings suggest that the behavior Kretzschmar et al. identify as being in conflict with the lower bound in Stevens arises from an implausible relationship between SO2 emissions and and thus provides little basis for revising this lower bound.

Beschreibung: In the framework of the World Meteorological Organisation's Sand and Dust Storm Warning Advisory and Assessment System, we evaluated the predictions of five state-of-the-art dust forecast models during an intense Saharan dust outbreak affecting western and northern Europe in April 2011. We assessed the capacity of the models to predict the evolution of the dust cloud with lead times of up to 72 h using observations of aerosol optical depth (AOD) from the AErosol RObotic NETwork (AERONET) and the Moderate Resolution Imaging Spectroradiometer (MODIS) and dust surface concentrations from a ground-based measurement network. In addition, the predicted vertical dust distribution was evaluated with vertical extinction profiles from the Cloud and Aerosol Lidar with Orthogonal Polarization (CALIOP). To assess the diversity in forecast capability among the models, the analysis was extended to wind field (both surface and profile), synoptic conditions, emissions and deposition fluxes. Models predict the onset and evolution of the AOD for all analysed lead times. On average, differences among the models are larger than differences among lead times for each individual model. In spite of large differences in emission and deposition, the models present comparable skill for AOD. In general, models are better in predicting AOD than near-surface dust concentration over the Iberian Peninsula. Models tend to underestimate the long-range transport towards northern Europe. Our analysis suggests that this is partly due to difficulties in simulating the vertical distribution dust and horizontal wind. Differences in the size distribution and wet scavenging efficiency may also account for model diversity in long-range transport.