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  • 1
    In: Geophysical research letters, Hoboken, NJ : Wiley, 1974, 36(2009), 1944-8007
    In: volume:36
    In: year:2009
    In: extent:5
    Description / Table of Contents: A major stratospheric sudden warming (SSW) in January 2009 was the strongest and most prolonged on record. Aura Microwave Limb Sounder (MLS) observations are used to provide an overview of dynamics and transport during the 2009 SSW, and to compare with the intense, long-lasting SSW in January 2006. The Arctic polar vortex split during the 2009 SSW, whereas the 2006 SSW was a vortex displacement event. Winds reversed to easterly more rapidly and reverted to westerly more slowly in 2009 than in 2006. More mixing of trace gases out of the vortex during the decay of the vortex fragments, and less before the fulfillment of major SSW criteria, was seen in 2009 than in 2006; persistent well-defined fragments of vortex and anticyclone air were more prevalent in 2009. The 2009 SSW had a more profound impact on the lower stratosphere than any previously observed SSW, with no significant recovery of the vortex in that region. The stratopause breakdown and subsequent reformation at very high altitude, accompanied by enhanced descent into a rapidly strengthening upper stratospheric vortex, were similar in 2009 and 2006. Many differences between 2006 and 2009 appear to be related to the different character of the SSWs in the two years.
    Type of Medium: Online Resource
    Pages: 5 , graph. Darst
    ISSN: 1944-8007
    Language: English
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  • 2
    Publication Date: 2022-09-27
    Description: The significant climate feedback of stratospheric water vapor (SWV) necessitates quantitative estimates of SWV budget changes. Model simulations driven by the newest European Centre for Medium‐Range Weather Forecast reanalysis ERA5, satellite observations from the Stratospheric Water and OzOne Satellite Homogenized data set, Microwave Limb Sounder, and in situ frost point hygrometer observations from Boulder all show substantial and persistent stratospheric moistening after a sharp drop in water vapor at the turn of the millennium. This moistening occurred mainly during 2000–2006 and SWV abundances then remained high over the last decade. We find strong positive trends in the Northern Hemisphere and weak negative trends over the South Pole, mainly during austral winter. Moistening of the tropical stratosphere after 2000 occurred during late boreal winter/spring, reached values of ∼0.2 ppm/decade, was well correlated with a warming of the cold point tropopause by ∼0.4 K/decade and can only be partially attributed to El Nino‐Southern Oscillation and volcanic eruptions.
    Description: Plain Language Summary: Water vapor is an effective greenhouse gas. Human‐induced climate change has led to warmer air in the troposphere, which consequently can hold more moisture, thus enhancing the greenhouse effect. The long‐term change in stratospheric water vapor (SWV) is less clear and currently under debate. Using satellite observations, balloon soundings and model simulations, we find an increase of SWV after 2000. This moistening occurred mainly during 2000–2006 and the stratospheric moisture content then remained high over the last decade. The increase of SWV is stronger in the Northern than in the Southern Hemisphere. Over the South Pole, a weak decrease was found. Moistening of the tropical stratosphere occurred mainly during late winter and spring, and was in line with warming of the tropical tropopause, the coldest region that separates the troposphere and stratosphere. Natural causes such as volcanic eruptions cannot completely explain this stratospheric moistening.
    Description: Key Points: Stratospheric moistening after 2000 is clearly detectable in ERA5‐driven simulations, satellite and in situ observations. Hemispheric asymmetry is found with strong positive trends in the Northern Hemisphere and weak negative trends over the South Pole. Moistening of the lower tropical stratosphere is only partially caused by El Nino‐Southern Oscillation and volcanic eruptions.
    Description: https://doi.org/10.5067/Aura/MLS/DATA2508
    Description: https://doi.org/10.5067/GLOSSAC-L3-V2.0
    Description: https://doi.org/10.5067/GLOSSAC-L3-V2.0
    Keywords: ddc:551.6
    Language: English
    Type: doc-type:article
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  • 3
    Publication Date: 2012-02-23
    Type: Conference or Workshop Item , NonPeerReviewed
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  • 4
    Publication Date: 2020-02-06
    Description: The climate research community uses atmospheric reanalysis data sets to understand a wide range of processes and variability in the atmosphere, yet different reanalyses may give very different results for the same diagnostics. The Stratosphere–troposphere Processes And their Role in Climate (SPARC) Reanalysis Intercomparison Project (S-RIP) is a coordinated activity to compare reanalysis data sets using a variety of key diagnostics. The objectives of this project are to identify differences among reanalyses and understand their underlying causes, to provide guidance on appropriate usage of various reanalysis products in scientific studies, particularly those of relevance to SPARC, and to contribute to future improvements in the reanalysis products by establishing collaborative links between reanalysis centres and data users. The project focuses predominantly on differences among reanalyses, although studies that include operational analyses and studies comparing reanalyses with observations are also included when appropriate. The emphasis is on diagnostics of the upper troposphere, stratosphere, and lower mesosphere. This paper summarizes the motivation and goals of the S-RIP activity and extensively reviews key technical aspects of the reanalysis data sets that are the focus of this activity. The special issue "The SPARC Reanalysis Intercomparison Project (S-RIP)" in this journal serves to collect research with relevance to the S-RIP in preparation for the publication of the planned two (interim and full) S-RIP reports.
    Type: Article , PeerReviewed
    Format: text
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  • 5
    Publication Date: 2020-09-21
    Description: [1] We present the first intercomparison between the two most comprehensive records of gas‐phase HNO3 profiles in the Antarctic stratosphere, covering the greater part of 1993 and 1995. We compare measurements by the Stony Brook Ground‐Based Millimeter‐wave Spectrometer (GBMS) at the South Pole with Version 5 HNO3 data from the Microwave Limb Sounder (MLS) aboard the Upper Atmospheric Research Satellite. Trajectory tracing was used to select MLS measurements in the 70°–80°S latitude band that sampled air observed by the GBMS during passage over the Pole. When temperatures were near the HNO3 condensation range, additional screening was performed to select MLS measurements that sampled air parcels within 1.5 K of the temperature they experienced over the Pole. Quantitative comparisons are given at 7 different potential temperature levels spanning the range ∼19–30 km. Agreement between the data sets is quite good between 465 and 655 K (∼20–25 km) during a large fraction of the year. Agreement is best during winter and spring, when seasonally averaged differences are generally within 1 ppbv below ∼25 km. At higher altitudes, and during summer and fall, the agreement becomes worse, and GBMS measurements can exceed MLS values by more than 3 ppbv. We provide evidence that differences occurring in the lower stratosphere during fall are due to lack of colocation between the two data sets during a period of strong poleward gradients in HNO3. Remaining discrepancies between GBMS and MLS V5 HNO3 measurements are thought to be due to instrumental or retrieval biases.
    Description: Published
    Description: id 4809
    Description: 5A. Ricerche polari e paleoclima
    Description: JCR Journal
    Keywords: MLS ; Nitric acid ; polar stratosphere ; 01.01. Atmosphere
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 6
    Publication Date: 2019-07-16
    Description: We investigate how important details of the microphysics of Polar Stratospheric Clouds (PSCs) and background aerosol particles are for the representation of polar ozone loss in chemistry transport models. For this purpose, the Lagrangian Chemistry and Transport Model ATLAS was applied to simulate the stratospheric chemistry in the Arctic winter 2009/2010. After a validation of the model results against measurements by the satelliteborne Microwave Limb Sounder (MLS), a number of sensitivity runs were performed. Thus, the efficiency of chlorine activation on different types of liquid aerosols versus activation on nitric acid trihydrate (NAT) clouds was explored. Moreover, the effects of particle composition and denitrification on ozone loss were analysed. It is shown that even large changes in the underlying assumptions regarding detailed activation surfaces have only a small impact on the modelled ozone loss. Differences in column ozone between the various sensitivity runs remain below 10% at the end of the winter. Chlorine activation on liquid aerosols alone is able to explain the observed magnitude and morphology of the mixing ratios of active chlorine, reservoir gases and ozone. This is even true for cold binary aerosols (no uptake of HNO3 from the gas-phase allowed in the model). This demonstrates that the heterogeneous chlorine activation in the polar stratosphere is dominated by the temperature dependence of the heterogeneous reaction rate constants rather than by the composition of the solid or liquid aerosol particles.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Conference , notRev
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  • 7
    Publication Date: 2019-07-16
    Description: We investigate how important details of the microphysics of Polar Stratospheric Clouds (PSCs) and background aerosol particles are for the representation of polar ozone loss in chemistry transport models. For this purpose, the Lagrangian Chemistry and Transport Model ATLAS was applied to simulate the stratospheric chemistry in the Arctic winter 2009/2010. After a validation of the model results against measurements by the satelliteborne Microwave Limb Sounder (MLS), a number of sensitivity runs were performed. Thus, the efficiency of chlorine activation on different types of liquid aerosols versus activation on nitric acid trihydrate (NAT) clouds was explored. Moreover, the effects of particle composition and denitrification on ozone loss were analysed. It is shown that even large changes in the underlying assumptions regarding detailed activation surfaces have only a small impact on the modelled ozone loss. Differences in column ozone between the various sensitivity runs remain below 10% at the end of the winter. Chlorine activation on liquid aerosols alone is able to explain the observed magnitude and morphology of the mixing ratios of active chlorine, reservoir gases and ozone. This is even true for cold binary aerosols (no uptake of HNO3 from the gas-phase allowed in the model). This demonstrates that the heterogeneous chlorine activation in the polar stratosphere is dominated by the temperature dependence of the heterogeneous reaction rate constants rather than by the composition of the solid or liquid aerosol particles.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Conference , notRev
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  • 8
    Publication Date: 2019-07-16
    Description: Chemical ozone destruction occurs over both polar regions in local winter–spring. In the Antarctic, essentially complete removal of lower-stratospheric ozone currently results in an ozone hole every year, whereas in the Arctic, ozone loss is highly variable and has until now been much more limited. Here we demonstrate that chemical ozone destruction over the Arctic in early 2011 was—for the first time in the observational record—comparable to that in the Antarctic ozone hole. Unusually long-lasting cold conditions in the Arctic lower stratosphere led to persistent enhancement in ozone-destroying forms of chlorine and to unprecedented ozone loss, which exceeded 80 per cent over 18–20 kilometres altitude. Our results show that Arctic ozone holes are possible even with temperatures much milder than those in the Antarctic. We cannot at present predict when such severe Arctic ozone depletion may be matched or exceeded.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev
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  • 9
    Publication Date: 2014-09-17
    Repository Name: EPIC Alfred Wegener Institut
    Type: Conference , notRev
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  • 10
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    American Geophysical Union (AGU)
    In:  EPIC3Geophysical Research Letters, American Geophysical Union (AGU), 51(4), ISSN: 0094-8276
    Publication Date: 2024-03-27
    Description: The eruption of the Hunga Tonga‐Hunga Ha'apai volcano on 15 January 2022 was one of the most explosive eruptions of the last decades. The amount of water vapor injected into the stratosphere was unprecedented in the observational record, increasing the stratospheric water vapor burden by about 10%. Using model runs from the ATLAS chemistry and transport model and Microwave Limb Sounder (MLS) satellite observations, we show that while 20%–40% more water vapor than usual was entrained into the Antarctic polar vortex in 2023 as it formed, the direct chemical effect of the increased water vapor on Antarctic ozone depletion in June through October was minor (less than 4 DU). This is because low temperatures in the vortex, as occur every year in the Antarctic, limit water vapor to the saturation pressure and thus reset any anomalies through the process of dehydration before they can affect ozone loss.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev
    Format: application/pdf
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