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  • 1
    In: Atmospheric chemistry and physics, Katlenburg-Lindau : EGU, 2001, 8(2008), 3, Seite 505-522, 1680-7324
    In: volume:8
    In: year:2008
    In: number:3
    In: pages:505-522
    Description / Table of Contents: The first three Arctic winters of the ACE mission represented two extremes of winter variability: Stratospheric sudden warmings (SSWs) in 2004 and 2006 were among the strongest, most prolonged on record; 2005 was a record cold winter. Canadian Arctic Atmospheric Chemistry Experiment (ACE) Validation Campaigns were conducted at Eureka (80° N, 86° W) during each of these winters. New satellite measurements from ACE-Fourier Transform Spectrometer (ACE-FTS), Sounding of the Atmosphere using Broadband Emission Radiometry (SABER), and Aura Microwave Limb Sounder (MLS), along with meteorological analyses and Eureka lidar temperatures, are used to detail the meteorology in these winters, to demonstrate its influence on transport, and to provide a context for interpretation of ACE-FTS and validation campaign observations. During the 2004 and 2006 SSWs, the vortex broke down throughout the stratosphere, reformed quickly in the upper stratosphere, and remained weak in the middle and lower stratosphere. The stratopause reformed at very high altitude, near 75 km. ACE measurements covered both vortex and extra-vortex conditions in each winter, except in late-February through mid-March 2004 and 2006, when the strong, pole-centered vortex that reformed after the SSWs resulted in ACE sampling only inside the vortex in the middle through upper stratosphere. The 2004 and 2006 Eureka campaigns were during the recovery from the SSWs, with the redeveloping vortex over Eureka. 2005 was the coldest winter on record in the lower stratosphere, but with an early final warming in mid-March. The vortex was over Eureka at the start of the 2005 campaign, but moved away as it broke up. Disparate temperature profile structure and vortex evolution resulted in much lower (higher) temperatures in the upper (lower) stratosphere in 2004 and 2006 than in 2005. Satellite temperatures agree well with lidar data up to 5060 km, and ACE-FTS, MLS and SABER show good agreement in high-latitude temperatures throughout the winters. Consistent with a strong, cold upper stratospheric vortex and enhanced radiative cooling after the SSWs, MLS and ACE-FTS trace gas measurements show strongly enhanced descent in the upper stratospheric vortex in late January through March 2006 compared to that in 2005.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
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  • 2
    ISSN: 1476-4687
    Source: Nature Archives 1869 - 2009
    Topics: Biology , Chemistry and Pharmacology , Medicine , Natural Sciences in General , Physics
    Notes: [Auszug] Satellite observations of ozone and chlorine monoxide concentrations during winter 1992–1993 show that in February 1993 chlorine in the lower stratosphere was mostly in chemically reactive forms. Decreases in stratospheric ozone concentration during February and early March 1993 are ...
    Type of Medium: Electronic Resource
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  • 3
    ISSN: 1476-4687
    Source: Nature Archives 1869 - 2009
    Topics: Biology , Chemistry and Pharmacology , Medicine , Natural Sciences in General , Physics
    Notes: [Auszug] Concentrations of atmospheric ozone and of CIO (the predominant form of reactive chlorine responsible for stratospheric ozone depletion) are reported for both the Arctic and Antarctic winters of the past 18 months. Chlorine in the lower stratosphere was almost completely converted to chemically ...
    Type of Medium: Electronic Resource
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  • 4
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    In:  [Poster] In: 21. Conference on Atmospheric and Oceanic Fluid Dynamics / 19. Conference on Middle Atmosphere, 26.-30.06.2017, Portland, OR, USA .
    Publication Date: 2018-12-10
    Type: Conference or Workshop Item , NonPeerReviewed
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  • 5
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    In:  [Talk] In: 5. International Conference on Reanalysis, 13.-17.11.2017, Rom, Italy .
    Publication Date: 2017-12-21
    Type: Conference or Workshop Item , NonPeerReviewed
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  • 6
    Publication Date: 2017-12-21
    Type: Conference or Workshop Item , NonPeerReviewed
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  • 7
    Publication Date: 2018-02-06
    Description: Global satellite observations of temperature and geopotential height (GPH) from the Microwave Limb Sounder (MLS) on the EOS Aura spacecraft are discussed. The precision, resolution, and accuracy of the data produced by the MLS version 2.2 processing algorithms are quantified, and recommendations for data screening are made. Temperature precision is 1 K or better from 316 hPa to 3.16 hPa, degrading to ∼3 K at 0.001 hPa. The vertical resolution is 3 km at 31.6 hPa, degrading to 6 km at 316 hPa and to ∼13 km at 0.001 hPa. Comparisons with analyses (Goddard Earth Observing System version 5.0.1 (GEOS-5), European Centre for Medium-range Weather Forecasts (ECMWF), Met Office (MetO)) and other observations (CHAllenging Minisatellite Payload (CHAMP), Atmospheric Infrared Sounder/Advanced Microwave Sounder Unit (AIRS/AMSU), Sounding of the Atmosphere using Broadband Radiometry (SABER), Halogen Occultation Experiment (HALOE), Atmospheric Chemistry Experiment (ACE), radiosondes) indicate that MLS temperature has persistent, pressure-dependent biases which are between −2.5 K and +1 K between 316 hPa and 10 hPa. The 100-hPa MLS v2.2 GPH surface has a bias of ∼150 m relative to the GEOS-5 values. These biases are compared to modeled systematic uncertainties. GPH biases relative to correlative measurements generally increase with height owing to an overall cold bias in MLS temperature relative to correlative temperature measurements in the upper stratosphere and mesosphere.
    Type: Article , PeerReviewed
    Format: text
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  • 8
    Publication Date: 2021-03-23
    Description: In the Antarctic ozone hole, ozone mixing ratios have been decreasing to extremely low values of 0.01–0.1 ppm in nearly all spring seasons since the late 1980s, corresponding to 95–99% local chemical loss. In contrast, Arctic ozone loss has been much more limited and mixing ratios have never before fallen below 0.5 ppm. In Arctic spring 2020, however, ozonesonde measurements in the most depleted parts of the polar vortex show a highly depleted layer, with ozone loss averaged over sondes peaking at 93% at 18 km. Typical minimum mixing ratios of 0.2 ppm were observed, with individual profiles showing values as low as 0.13 ppm (96% loss). The reason for the unprecedented chemical loss was an unusually strong, long-lasting, and cold polar vortex, showing that for individual winters the effect of the slow decline of ozone-depleting substances on ozone depletion may be counteracted by low temperatures.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev
    Format: application/pdf
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  • 9
    Publication Date: 2017-04-03
    Description: We assess the quality of the version 2.2 (v2.2) HNO3 measurements from the Microwave Limb Sounder (MLS) on the Earth Observing System Aura satellite. The MLS HNO3 product has been greatly improved over that in the previous version (v1.5), with smoother profiles, much more realistic behavior at the lowest retrieval levels, and correction of a high bias caused by an error in one of the spectroscopy files used in v1.5 processing. The v2.2 HNO3 data are scientifically useful over the range 215 to 3.2 hPa, with single-profile precision of 0.7 ppbv throughout. Vertical resolution is 3–4 km in the upper troposphere and lower stratosphere, degrading to 5 km in the middle and upper stratosphere. The impact of various sources of systematic uncertainty has been quantified through a comprehensive set of retrieval simulations. In aggregate, systematic uncertainties are estimated to induce in the v2.2 HNO3 measurements biases that vary with altitude between ±0.5 and ±2 ppbv and multiplicative errors of ±5–15% throughout the stratosphere, rising to ±30% at 215 hPa. Consistent with this uncertainty analysis, comparisons with correlative data sets show that relative to HNO3 measurements from ground-based, balloon-borne, and satellite instruments operating in both the infrared and microwave regions of the spectrum, MLS v2.2 HNO3 mixing ratios are uniformly low by 10–30% throughout most of the stratosphere. Comparisons with in situ measurements made from the DC-8 and WB-57 aircraft in the upper troposphere and lowermost stratosphere indicate that the MLS HNO3 values are low in this region as well, but are useful for scientific studies (with appropriate averaging).
    Description: Published
    Description: D24S40
    Description: 1.7. Osservazioni di alta e media atmosfera
    Description: JCR Journal
    Description: reserved
    Keywords: satellite validation ; stratospheric HNO3 ; 01. Atmosphere::01.01. Atmosphere::01.01.01. Composition and Structure
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 10
    Publication Date: 2019-07-16
    Description: A number of studies have reported empirical estimates of ozone loss in the Arctic vortex.They have used satellite and in situ measurements and have principally covered the Arcticwinters in the 1990s. While there is qualitative consistency between the patterns of ozone loss, aquantitative comparison of the published values shows apparent disagreements. In this paper weexamine these disagreements in more detail. We choose to concentrate on the five maintechniques (Match, Système d'Analyse par Observation Zénithale (SAOZ)/REPROBUS,Microwave Limb Sounder (MLS), vortex average descent, and the Halogen OccultationExperiment (HALOE) ozone tracer approach). Estimates of the ozone losses in three winters(1994/1995, 1995/1996 and 1996/1997) are recalculated so that the same time periods, altituderanges, and definitions of the Arctic vortex are used. This recalculation reveals a remarkably goodagreement between the various estimates. For example, a superficial comparison of results fromMatch and from MLS indicates a big discrepancy (2.0 ± 0.3 and 0.85 ppmv, respectively, for airending at ~460 K in March 1995). However, the more precise comparisons presented here revealgood agreement for the individual MLS periods (0.5 ± 0.1 versus 0.5 ppmv; 0.4 ± 0.2 versus0.3-0.4 ppmv; and 0.16 ± 0.09 ppmv versus no significant loss). Initial comparisons of the columnlosses derived for 1999/2000 also show good agreement with four techniques, giving 105 DU(SAOZ/REPROBUS), 80 DU (380-700 K partial column from Polar Ozone and Aerosol Monitoring(POAM)/REPROBUS), 85 ± 10 DU (HALOE ozone tracer), and 88 ± 13 (400-580 partial columnfrom Match). There are some remaining discrepancies with ozone losses calculated using HALOEozone tracer relations; it is important to ensure that the initial relation is truly representative of thevortex prior to the period of ozone loss.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev
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