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  • 1
    Electronic Resource
    Electronic Resource
    Computational study of molecular hydrogen in zeolite Na–A. II. Density of rotational states and inelastic neutron scattering spectra (2001)
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 114 (2001), S. 10137-10150 
    Details
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Part I of this series [J. Chem. Phys. 111, 7599 (1999)] describes a simulation of H2 adsorbed within zeolite Na–A in which a block Lanczos procedure is used to generate the first several (9) rotational eigenstates of H2, modeled as a rigid rotor, and equilibrated at a given temperature via Monte Carlo sampling. Here, we show that rotational states are strongly perturbed by the electrostatic fields in the solid. Wave functions and densities of rotational energy states are presented. Simulated neutron spectra are compared with inelastic neutron scattering data. Comparisons are made with IR spectra in which rotational levels may appear due to rovibrational coupling. © 2001 American Institute of Physics.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.1352733
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  • 2
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    Parametric subharmonic instability of the internal tide at 29°N (2013)
    American Meteorological Society
    Details
    Publication Date: 2022-05-25
    Description: Author Posting. © American Meteorological Society, 2013. This article is posted here by permission of American Meteorological Society for personal use, not for redistribution. The definitive version was published in Journal of Physical Oceanography 43 (2013): 17–28, doi:10.1175/JPO-D-11-0108.1.
    Description: Observational evidence is presented for transfer of energy from the internal tide to near-inertial motions near 29°N in the Pacific Ocean. The transfer is accomplished via parametric subharmonic instability (PSI), which involves interaction between a primary wave (the internal tide in this case) and two smaller-scale waves of nearly half the frequency. The internal tide at this location is a complex superposition of a low-mode waves propagating north from Hawaii and higher-mode waves generated at local seamounts, making application of PSI theory challenging. Nevertheless, a statistically significant phase locking is documented between the internal tide and upward- and downward-propagating near-inertial waves. The phase between those three waves is consistent with that expected from PSI theory. Calculated energy transfer rates from the tide to near-inertial motions are modest, consistent with local dissipation rate estimates. The conclusion is that while PSI does befall the tide near a critical latitude of 29°N, it does not do so catastrophically.
    Description: This work was sponsored by NSF OCE 04-25283.
    Description: 2013-07-01
    Keywords: Diapycnal mixing ; Internal waves ; Nonlinear dynamics
    Repository Name: Woods Hole Open Access Server
    Type: Article
    Format: application/pdf
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  • 3
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    Submesoscale processes at shallow salinity fronts in the Bay of Bengal : observations during the winter monsoon (2018)
    American Meteorological Society
    Details
    Publication Date: 2022-05-25
    Description: Author Posting. © American Meteorological Society, 2018. This article is posted here by permission of American Meteorological Society for personal use, not for redistribution. The definitive version was published in Journal of Physical Oceanography 48 (2018): 479-509, doi:10.1175/JPO-D-16-0283.1.
    Description: Lateral submesoscale processes and their influence on vertical stratification at shallow salinity fronts in the central Bay of Bengal during the winter monsoon are explored using high-resolution data from a cruise in November 2013. The observations are from a radiator survey centered at a salinity-controlled density front, embedded in a zone of moderate mesoscale strain (0.15 times the Coriolis parameter) and forced by winds with a downfront orientation. Below a thin mixed layer, often ≤10 m, the analysis shows several dynamical signatures indicative of submesoscale processes: (i) negative Ertel potential vorticity (PV); (ii) low-PV anomalies with O(1–10) km lateral extent, where the vorticity estimated on isopycnals and the isopycnal thickness are tightly coupled, varying in lockstep to yield low PV; (iii) flow conditions susceptible to forced symmetric instability (FSI) or bearing the imprint of earlier FSI events; (iv) negative lateral gradients in the absolute momentum field (inertial instability); and (v) strong contribution from differential sheared advection at O(1) km scales to the growth rate of the depth-averaged stratification. The findings here show one-dimensional vertical processes alone cannot explain the vertical stratification and its lateral variability over O(1–10) km scales at the radiator survey.
    Description: S. Ramachandran acknowledges support from the National Science Foundation through award OCE 1558849 and the U.S. Office of Naval Research, Grants N00014-13-1-0456 and N00014-17- 1-2355. A. Tandon acknowledges support from the U.S. Office of Naval Research, Grants N00014-13-1-0456 and N00014-17-1-2355. J. T. Farrar and R. A. Weller were supported by the U.S. Office of Naval Research, Grant N00014-13-1-0453, to collect the UCTD data and process theUCTD and shipboard meteorological data. J. Nash, J. Mackinnon, and A. F. Waterhouse acknowledge support from the U. S. Office of Naval Research, Grants N00014-13-1-0503 and N00014-14-1-0455. E. Shroyer acknowledges support from the U. S. Office of Naval Research, Grants N00014-14-10236 and N00014-15- 12634. A. Mahadevan acknowledges support fromthe U. S. Office of Naval Research, Grant N00014-13-10451. A. J. Lucas and R. Pinkel acknowledge support from the U. S. Office of Naval Research, Grant N00014-13-1-0489.
    Description: 2018-08-26
    Keywords: Indian Ocean ; Baroclinic flows ; Potential vorticity ; Fronts ; Monsoons ; Oceanic mixed layer
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 4
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    The formation and fate of internal waves in the South China Sea (2015)
    Details
    Publication Date: 2022-05-25
    Description: Author Posting. © The Author(s), 2015. This is the author's version of the work. It is posted here by permission of Nature Publishing Group for personal use, not for redistribution. The definitive version was published in Nature 521 (2015): 65-69, doi:10.1038/nature14399.
    Description: Internal gravity waves, the subsurface analogue of the familiar surface gravity waves that break on beaches, are ubiquitous in the ocean. Because of their strong vertical and horizontal currents, and the turbulent mixing caused by their breaking, they impact a panoply of ocean processes, such as the supply of nutrients for photosynthesis1, sediment and pollutant transport2 and acoustic transmission3; they also pose hazards for manmade structures in the ocean4. Generated primarily by the wind and the tides, internal waves can travel thousands of kilometres from their sources before breaking5, posing severe challenges for their observation and their inclusion in numerical climate models, which are sensitive to their effects6-7. Over a decade of studies8-11 have targeted the South China Sea, where the oceans’ most powerful internal waves are generated in the Luzon Strait and steepen dramatically as they propagate west. Confusion has persisted regarding their generation mechanism, variability and energy budget, however, due to the lack of in-situ data from the Luzon Strait, where extreme flow conditions make measurements challenging. Here we employ new observations and numerical models to (i) show that the waves begin as sinusoidal disturbances rather than from sharp hydraulic phenomena, (ii) reveal the existence of 〉200-m-high breaking internal waves in the generation region that give rise to turbulence levels 〉10,000 times that in the open ocean, (iii) determine that the Kuroshio western boundary current significantly refracts the internal wave field emanating from the Luzon Strait, and (iv) demonstrate a factor-of-two agreement between modelled and observed energy fluxes that enables the first observationally-supported energy budget of the region. Together, these findings give a cradle-to-grave picture of internal waves on a basin scale, which will support further improvements of their representation in numerical climate predictions.
    Description: Our work was supported by the U.S. Office of Naval Research and the Taiwan National Science Council.
    Description: 2015-10-29
    Repository Name: Woods Hole Open Access Server
    Type: Preprint
    Format: application/pdf
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  • 5
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    Global patterns of diapycnal mixing from measurements of the turbulent dissipation rate (2014)
    American Meteorological Society
    Details
    Publication Date: 2022-05-26
    Description: Author Posting. © American Meteorological Society, 2014. This article is posted here by permission of American Meteorological Society for personal use, not for redistribution. The definitive version was published in Journal of Physical Oceanography 44 (2014): 1854–1872, doi:10.1175/JPO-D-13-0104.1.
    Description: The authors present inferences of diapycnal diffusivity from a compilation of over 5200 microstructure profiles. As microstructure observations are sparse, these are supplemented with indirect measurements of mixing obtained from (i) Thorpe-scale overturns from moored profilers, a finescale parameterization applied to (ii) shipboard observations of upper-ocean shear, (iii) strain as measured by profiling floats, and (iv) shear and strain from full-depth lowered acoustic Doppler current profilers (LADCP) and CTD profiles. Vertical profiles of the turbulent dissipation rate are bottom enhanced over rough topography and abrupt, isolated ridges. The geography of depth-integrated dissipation rate shows spatial variability related to internal wave generation, suggesting one direct energy pathway to turbulence. The global-averaged diapycnal diffusivity below 1000-m depth is O(10−4) m2 s−1 and above 1000-m depth is O(10−5) m2 s−1. The compiled microstructure observations sample a wide range of internal wave power inputs and topographic roughness, providing a dataset with which to estimate a representative global-averaged dissipation rate and diffusivity. However, there is strong regional variability in the ratio between local internal wave generation and local dissipation. In some regions, the depth-integrated dissipation rate is comparable to the estimated power input into the local internal wave field. In a few cases, more internal wave power is dissipated than locally generated, suggesting remote internal wave sources. However, at most locations the total power lost through turbulent dissipation is less than the input into the local internal wave field. This suggests dissipation elsewhere, such as continental margins.
    Description: This research was funded by the Climate Process Team (CPT) on internal wave–driven mixing throughNSF GrantOCE-0968721. GSC acknowledges support from NSF Grants OCE-0825266 (EXITS), OCE-1029483 (SPAM), and OCE-1029722 (MIXET). LDT and CBW acknowledge support from NSF Grant OCE-0927650. SWand ACNG acknowledge support from NERC Grant NE/G001510/1 (SOFine).
    Description: 2015-01-01
    Keywords: Circulation/ Dynamics ; Diapycnal mixing ; Internal waves
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 6
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    A tale of two spicy seas (2016)
    The Oceanography Society
    Details
    Publication Date: 2022-05-26
    Description: Author Posting. © The Oceanography Society, 2016. This article is posted here by permission of The Oceanography Society for personal use, not for redistribution. The definitive version was published in Oceanography 29, no. 2 (2016): 50–61, doi:10.5670/oceanog.2016.38.
    Description: Upper-ocean turbulent heat fluxes in the Bay of Bengal and the Arctic Ocean drive regional monsoons and sea ice melt, respectively, important issues of societal interest. In both cases, accurate prediction of these heat transports depends on proper representation of the small-scale structure of vertical stratification, which in turn is created by a host of complex submesoscale processes. Though half a world apart and having dramatically different temperatures, there are surprising similarities between the two: both have (1) very fresh surface layers that are largely decoupled from the ocean below by a sharp halocline barrier, (2) evidence of interleaving lateral and vertical gradients that set upper-ocean stratification, and (3) vertical turbulent heat fluxes within the upper ocean that respond sensitively to these structures. However, there are clear differences in each ocean’s horizontal scales of variability, suggesting that despite similar background states, the sharpening and evolution of mesoscale gradients at convergence zones plays out quite differently. Here, we conduct a qualitative and statistical comparison of these two seas, with the goal of bringing to light fundamental underlying dynamics that will hopefully improve the accuracy of forecast models in both parts of the world.
    Description: We gratefully acknowledge support from the Office of Naval Research, the National Science Foundation, and the Ocean Mixing and Monsoon (OMM) program of the Monsoon Mission of India.
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 7
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    Estimating dissipation rates associated with double diffusion (2021)
    American Geophysical Union
    Details
    Publication Date: 2022-10-26
    Description: Author Posting. © American Geophysical Union, 2021. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Geophysical Research Letters 48(15), (2021): e2021GL092779, https://doi.org/10.1029/2021GL092779.
    Description: Double diffusion refers to a variety of turbulent processes in which potential energy is released into kinetic energy, made possible in the ocean by the difference in molecular diffusivities between salinity and temperature. Here, we present a new method for estimating the kinetic energy dissipation rates forced by double-diffusive convection using temperature and salinity data alone. The method estimates the up-gradient diapycnal buoyancy flux associated with double diffusion, which is hypothesized to balance the dissipation rate. To calculate the temperature and salinity gradients on small scales we apply a canonical scaling for compensated thermohaline variance (or ‘spice’) on sub-measurement scales with a fixed buoyancy gradient. Our predicted dissipation rates compare favorably with microstructure measurements collected in the Chukchi Sea. Fine et al. (2018), https://doi.org/10.1175/jpo-d-18-0028.1, showed that dissipation rates provide good estimates for heat fluxes in this region. Finally, we show the method maintains predictive skill when applied to a sub-sampling of the Conductivity, Temperature, Depth (CTD) data.
    Description: This work was supported by the Natural Environment Research Council (grant number NE/L002507/1).
    Keywords: Ocean mixing ; Double-diffusive convection ; Compensated thermohaline variance
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 8
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    Eddies, topography, and the abyssal flow by the Kyushu-Palau Ridge near Velasco Reef (2020)
    The Oceanography Society
    Details
    Publication Date: 2022-05-26
    Description: © The Author(s), 2019. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Andres, M., Siegelman, M., Hormann, V., Musgrave, R. C., Merrifield, S. T., Rudnick, D. L., Merrifield, M. A., Alford, M. H., Voet, G., Wijesekera, H. W., MacKinnon, J. A., Centurioni, L., Nash, J. D., & Terrill, E. J. Eddies, topography, and the abyssal flow by the Kyushu-Palau Ridge near Velasco Reef. Oceanography, 32(4), (2019): 46-55, doi: 10.5670/oceanog.2019.410.
    Description: Palau, an island group in the tropical western North Pacific at the southern end of Kyushu-Palau Ridge, sits near the boundary between the westward-​flowing North Equatorial Current (NEC) and the eastward-flowing North Equatorial Countercurrent. Combining remote-sensing observations of the sea surface with an unprecedented in situ set of subsurface measurements, we examine the flow near Palau with a particular focus on the abyssal circulation and on the deep expression of mesoscale eddies in the region. We find that the deep currents time-averaged over 10 months are generally very weak north of Palau and not aligned with the NEC in the upper ocean. This weak abyssal flow is punctuated by the passing of mesoscale eddies, evident as sea surface height anomalies, that disrupt the mean flow from the surface to the seafloor. Eddy influence is observed to depths exceeding 4,200 m. These deep-​reaching mesoscale eddies typically propagate westward past Palau, and as they do, any associated deep flows must contend with the topography of the Kyushu-Palau Ridge. This interaction leads to vertical structure far below the main thermocline. Observations examined here for one particularly strong and well-sampled eddy suggest that the flow was equivalent barotropic in the far field east and west of the ridge, with a more complicated vertical structure in the immediate vicinity of the ridge by the tip of Velasco Reef.
    Description: We gratefully acknowledge the help of Captain David Murline and the crew of R/V Roger Revelle and the shore-based assistance of Lori Colin and Pat Colin of the Coral Reef Research Foundation. We sincerely thank Terri Paluszkiewicz for her steadfast support of basic research programs, including FLEAT, during her many years of service to the community as Office of Naval Research (ONR) Physical Oceanography Program Manager. MA was supported by ONR grant N000141612668, MS and MAM by N00014-16-1-2671, MHA and JAM by N00014-15-1-2264 and N00014-16-1-3070, GV by N00014-15-1-2592, DLR by N00014- 15-1-2488, and STM and EJT by N00014-15-1-2304. VH and LC were supported by ONR grant N00014-15-1-2286 and NOAA GDP grant NA15OAR4320071. RCM was supported by the Postdoctoral Scholar Program at the Wood Hole Oceanographic Institution, with funding provided by the Weston Howland Jr. Postdoctoral Scholarship. We thank the Palau National Government for permission to carry out the research in Palau.
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 9
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    A warm jet in a cold ocean (2021)
    In:  EPIC3Nature Communications, 12(1), ISSN: 2041-1723
    Details
    Publication Date: 2022-10-10
    Description: Unprecedented quantities of heat are entering the Pacific sector of the Arctic Ocean through Bering Strait, particularly during summer months. Though some heat is lost to the atmosphere during autumn cooling, a significant fraction of the incoming warm, salty water subducts (dives beneath) below a cooler fresher layer of near-surface water, subsequently extending hundreds of kilometers into the Beaufort Gyre. Upward turbulent mixing of these sub-surface pockets of heat is likely accelerating sea ice melt in the region. This Pacific-origin water brings both heat and unique biogeochemical properties, contributing to a changing Arctic ecosystem. However, our ability to understand or forecast the role of this incoming water mass has been hampered by lack of understanding of the physical processes controlling subduction and evolution of this this warm water. Crucially, the processes seen here occur at small horizontal scales not resolved by regional forecast models or climate simulations; new parameterizations must be developed that accurately represent the physics. Here we present novel high resolution observations showing the detailed process of subduction and initial evolution of warm Pacific-origin water in the southern Beaufort Gyre.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev
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  • 10
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    Microstructure mixing observations and finescale parameterizations in the Beaufort Sea (2021)
    American Meteorological Society
    Details
    Publication Date: 2022-05-27
    Description: Author Posting. © American Meteorological Society, 2021. This article is posted here by permission of American Meteorological Society for personal use, not for redistribution. The definitive version was published in Journal of Physical Oceanography 51(1), (2021): 19-35, https://doi.org/10.1175/JPO-D-19-0233.1.
    Description: In the Beaufort Sea in September of 2015, concurrent mooring and microstructure observations were used to assess dissipation rates in the vicinity of 72°35′N, 145°1′W. Microstructure measurements from a free-falling profiler survey showed very low [O(10−10) W kg−1] turbulent kinetic energy dissipation rates ε. A finescale parameterization based on both shear and strain measurements was applied to estimate the ratio of shear to strain Rω and ε at the mooring location, and a strain-based parameterization was applied to the microstructure survey (which occurred approximately 100 km away from the mooring site) for direct comparison with microstructure results. The finescale parameterization worked well, with discrepancies ranging from a factor of 1–2.5 depending on depth. The largest discrepancies occurred at depths with high shear. Mean Rω was 17, and Rω showed high variability with values ranging from 3 to 50 over 8 days. Observed ε was slightly elevated (factor of 2–3 compared with a later survey of 11 profiles taken over 3 h) from 25 to 125 m following a wind event which occurred at the beginning of the mooring deployment, reaching a maximum of ε= 6 × 10−10 W kg−1 at 30-m depth. Velocity signals associated with near-inertial waves (NIWs) were observed at depths greater than 200 m, where the Atlantic Water mass represents a reservoir of oceanic heat. However, no evidence of elevated ε or heat fluxes was observed in association with NIWs at these depths in either the microstructure survey or the finescale parameterization estimates.
    Description: This work was supported by NSF Grants PLR 14-56705 and PLR-1303791 and by NSF Graduate Research Fellowship Grant DGE-1650112.
    Keywords: Ocean ; Arctic ; Internal waves ; Turbulence ; Diapycnal mixing
    Repository Name: Woods Hole Open Access Server
    Type: Article
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