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  • 1
    Online Resource
    Online Resource
    Global-scale quantification of mineralization pathways in marine sediments : a reaction-transport modeling approach (2009)
    Associated volumes
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    In: Geochemistry, geophysics, geosystems, Hoboken, NJ : Wiley, 2000, 10(2009), 10, 1525-2027
    In: volume:10
    In: year:2009
    In: number:10
    In: extent:24
    Type of Medium: Online Resource
    Pages: 24 , graph. Darst
    ISSN: 1525-2027
    DOI: 10.1029/2009GC002484
    Language: English
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  • 2
    Online Resource
    Online Resource
    Major bottom water ventilation events do not significantly reduce basin-wide benthic N and P release in the Eastern Gotland Basin (Baltic Sea) (2017)
    Associated volumes
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    In: Frontiers in Marine Science, Lausanne : Frontiers Media, 2014, Bd. 4 (2017), Article 18, 2296-7745
    In: volume:4
    In: year:2017
    Type of Medium: Online Resource
    Pages: Diagramme, Karten
    ISSN: 2296-7745
    URL: https://www.frontiersin.org/articles/10.3389/fmars.2017.00018/full
    DOI: 10.3389/fmars.2017.00018
    Language: English
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  • 3
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    A method for the calculation of anaerobic oxidation of methane rates across regional scales: an example from the Belt Seas and The Sound (North Sea–Baltic Sea transition) (2013)
    SPRINGER
    In:  EPIC3Geo-Marine Letters, SPRINGER, 33, pp. 299-310, ISSN: 0276-0460
    Details
    Publication Date: 2017-06-21
    Description: Estimating the amount of methane in the seafloor globally as well as the flux of methane from sediments toward the ocean–atmosphere system are important considerations in both geological and climate sciences. Nevertheless, global estimates of methane inventories and rates of methane production and consumption through anaerobic oxidation in marine sediments are very poorly constrained. Tools for regionally assessing methane formation and consumption rates would greatly increase our understanding of the spatial heterogeneity of the methane cycle as well as help constrain the global methane budget. In this article, an algorithm for calculating methane consumption rates in the inner shelf is applied to the gas-rich sediments of the Belt Seas and The Sound (North Sea–Baltic Sea transition). It is based on the depth of free gas determined by hydroacoustic techniques and the local methane solubility concentration. Due to the continuous nature of shipboard hydroacoustic measurements, this algorithm captures spatial heterogeneities in methane fluxes better than geochemical analyses of point sources such as observational/sampling stations. The sensibility of the algorithm with respect to the resolution of the free gas depth measurements (2 m vs. 50 cm) is proven of minor importance (a discrepancy of 〈10%) for a small part of the study area. The algorithm-derived anaerobic methane oxidation rates compare well with previous measured and modeling studies. Finally, regional results reveal that contemporary anaerobic methane oxidation in worldwide inner-shelf sediments may be an order of magnitude lower (ca. 0.24 Tmol year–1) than previous estimates (4.6 Tmol year–1). These algorithms ultimately help improve regional estimates of anaerobic oxidation of methane rates.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev
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  • 4
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    Towards improved monitoring of offshore carbon storage: A real-world field experiment detecting a controlled sub-seafloor CO2 release (2021)
    In:  EPIC3International Journal of Greenhouse Gas Control, 106, pp. 103237, ISSN: 17505836
    Details
    Publication Date: 2021-12-15
    Description: Carbon capture and storage (CCS) is a key technology to reduce carbon dioxide (CO2) emissions from industrial processes in a feasible, substantial, and timely manner. For geological CO2 storage to be safe, reliable, and accepted by society, robust strategies for CO2 leakage detection, quantification and management are crucial. The STEMM-CCS (Strategies for Environmental Monitoring of Marine Carbon Capture and Storage) project aimed to provide techniques and understanding to enable and inform cost-effective monitoring of CCS sites in the marine environment. A controlled CO2 release experiment was carried out in the central North Sea, designed to mimic an unintended emission of CO2 from a subsurface CO2 storage site to the seafloor. A total of 675 kg of CO2 were released into the shallow sediments (~3 m below seafloor), at flow rates between 6 and 143 kg/d. A combination of novel techniques, adapted versions of existing techniques, and well-proven standard techniques were used to detect, characterise and quantify gaseous and dissolved CO2 in the sediments and the overlying seawater. This paper provides an overview of this ambitious field experiment. We describe the preparatory work prior to the release experiment, the experimental layout and procedures, the methods tested, and summarise the main results and the lessons learnt.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev , info:eu-repo/semantics/article
    Format: application/pdf
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  • 5
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    Growth and survival of the winged oyster Pteria colymbus in suspended culture: influence of environmental factors associated to upwelling periods (2017)
    Springer
    In:  Aquaculture International, 25 (4). pp. 1653-1666.
    Details
    Publication Date: 2020-02-06
    Description: The present study examines the influence that environmental variables exerted on changes in condition index (CI), shell height (SH—dorsal-ventral axis) and soft tissue mass increments (STM) of the winged oyster Pteria colymbus in suspended culture during periods of upwelling (December to April) and non-upwelling (August to November) in the Cariaco Gulf, northeastern Venezuela. Environmental variables recorded between April 2012 and May 2013 included seston, water transparency, temperature, dissolved oxygen, chlorophyll a (Chl a) and the upwelling index (UI). Individuals were cultivated in lantern nets with an overall density of 56 individuals/0.123 m2. From three randomly chosen baskets, five individuals were sampled each month and changes in CI, STM and SH were related to the environmental variables using Spearman correlation and PCA. Results show that during upwelling, both Chl a and UI presented a positive and significant relationship with the oyster condition and growth parameters. During non-upwelling (low UI), this relationship was inverse, demonstrating the important influence of upwelling and non-upwelling periods on the ecophysiology of the species. Furthermore, it was shown that the non-upwelling, characterized by high temperatures and low food availability, is a critical period for P. colymbus, judging by a decrease in growth and survival rate. Nonetheless, this species reached 50 mm in 5 months, a size considered as commercially viable, suggesting that the study area is favourable to the cultivation of the winged oyster despite a dramatic decrease in upwelling intensity in the last decade.
    Type: Article , PeerReviewed
    Format: text
    DOI: 10.1007/s10499-017-0141-2
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    OceanRep: Article in a Scientific Journal - peer-reviewed
  • 6
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    Carbon regeneration in the Cariaco Basin, Venezuela (2017)
    Instituto Oceanográfico da Universidade de São Paulo, SciELO
    In:  Brazilian Journal of Oceanography, 65 (1). pp. 19-28.
    Details
    Publication Date: 2020-02-06
    Description: The carbon regeneration in the water column of the Cariaco Basin (Venezuela) was investigated using a regression model of total alkalinity (TA) and the concentration of total inorganic carbon (TCO2). Primary productivity (PP) was determined from the inorganic carbon fraction assimilated by phytoplankton and the variation of the 22 and 23ºC isotherm was used as an indicator of coastal upwelling. The results indicate that CO2 levels were lowest (1962 µmol/kg) at the surface and increased to 2451 µmol/kg below the oxic-anoxic redox interface. The vertical regeneration distribution of carbon was dominated (82%) by organic carbon originating from the soft tissue of photosynthetic organisms, whereas 18% originated from the dissolution of biogenic calcite. The regeneration of organic carbon was highest in the surface layer in agreement with the primary productivity values. However, at the oxic-anoxic interface a second more intense maximum was detected (70-80%), generated by chemotrophic respiration of organic material by microorganisms. The percentages in the anoxic layers were lower than in the oxic zone because aerobic decomposition occurs more rapidly than anaerobic respiration of organic material because more labile fractions of organic carbon have already been mineralized in the upper layers.
    Type: Article , PeerReviewed
    Format: text
    DOI: 10.1590/S1679-87592017121406501
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    OceanRep: Article in a Scientific Journal - peer-reviewed
  • 7
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    Sedimentary molybdenum cycling in the aftermath of seawater inflow to the intermittently euxinic Gotland Deep, Central Baltic Sea (2018)
    Elsevier
    In:  Chemical Geology, 491 . pp. 27-38.
    Details
    Publication Date: 2021-02-08
    Description: Molybdenum (Mo) concentrations and isotope compositions in sediments and shales are commonly used as proxies for anoxic and sulfidic (i.e., euxinic) conditions in the water column of paleo-marine systems. A basic assumption underlying this practice is that the proxy signal extracted from the geological record is controlled by long-term (order of decades to millennia) Mo scavenging in the euxinic water column rather than Mo deposition during brief episodes or events (order of weeks to months). To test whether this assumption is viable we studied the biogeochemical cycling of Mo and its isotopes in sediments of the intermittently euxinic Gotland Deep in the central Baltic Sea. Here, multiannual to decadal periods of euxinia are occasionally interrupted by inflow events during which well‑oxygenated water from the North Sea penetrates into the basin. During these events manganese (Mn) (oxyhydr)oxide minerals are precipitated in the water column, which are known to scavenge Mo. We present sediment and pore water Mo and Mo isotope data for sediment cores which were taken before and after a series of inflow events between 2014 and 2016. After seawater inflow, pore water Mo concentrations in anoxic surface sediments exceed the salinity-normalized concentration by more than two orders of magnitude and coincide with transient peaks of dissolved Mn. A fraction of the Mo liberated into the pore water is transported by diffusion in a downward direction and sequestered by organic matter within the sulfidic zone of the sediment. Diffusive flux calculations as well as a mass balance that is based on the sedimentary Mo isotope composition suggest that about equal proportions of the Mo accumulating in the basin are delivered by Mn (oxyhydr)oxide minerals during inflow events and Mo scavenging with hydrogen sulfide during euxinic periods. Since the anoxic surface sediment where Mo is released from Mn (oxyhydr)oxides are separated by several centimeters from the deeper sulfidic layers where Mo is removed, the solid phase record of Mo concentration and isotope composition would be misinterpreted if steady state Mo accumulation was assumed. Based on our observations in the Gotland Deep, we argue that short-term redox fluctuations need to be considered when interpreting Mo-based paleo-records.
    Type: Article , PeerReviewed
    Format: text
    Format: other
    Format: other
    Format: text
    DOI: 10.1016/j.chemgeo.2018.04.031
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    OceanRep: Article in a Scientific Journal - peer-reviewed
  • 8
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    Methane fluxes from tropical coastal lagoons surrounded by mangroves, Yucatán, Mexico (2017)
    AGU (American Geophysical Union) | Wiley
    In:  Journal of Geophysical Research: Biogeosciences, 122 (5). pp. 1156-1174.
    Details
    Publication Date: 2020-02-06
    Description: Methane concentrations in the water column and emissions to the atmosphere were determined for three tropical coastal lagoons surrounded by mangrove forests on the Yucatán Peninsula, Mexico. Surface water dissolved methane was sampled at different seasons over a period of 2 years in areas representing a wide range of salinities and anthropogenic impacts. The highest surface water methane concentrations (up to 8378 nM) were measured in a polluted canal associated with Terminos Lagoon. In Chelem Lagoon, methane concentrations were typically lower, except in the polluted harbor area (1796 nM). In the relatively pristine Celestún Lagoon, surface water methane concentrations ranged from 41 to 2551 nM. Methane concentrations were negatively correlated with salinity in Celestún, while in Chelem and Terminos high methane concentrations were associated with areas of known pollution inputs, irrespective of salinity. The diffusive methane flux from surface lagoon water to the atmosphere ranged from 0.0023 to 15 mmol CH4 m-2 d-1. Flux chamber measurements revealed that direct methane release as ebullition was up to 3 orders of magnitude greater than measured diffusive flux. Coastal mangrove lagoons may therefore be an important natural source of methane to the atmosphere despite their relatively high salinity. Pollution inputs are likely to substantially enhance this flux. Additional statistically rigorous data collected globally are needed to better consider methane fluxes from mangrove-surrounded coastal areas in response to sea level changes and anthropogenic pollution in order to refine projections of future atmospheric methane budgets.
    Type: Article , PeerReviewed
    Format: text
    DOI: 10.1002/2017JG003761
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  • 9
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    Benthic Dinitrogen Fixation Traversing the Oxygen Minimum Zone Off Mauritania (NW Africa) (2017)
    Frontiers
    In:  Frontiers in Marine Science, 4 (390).
    Details
    Publication Date: 2020-02-06
    Type: Article , PeerReviewed
    Format: text
    DOI: 10.3389/fmars.2017.00390
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  • 10
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    Intense molybdenum accumulation in sediments underneath a nitrogenous water column and implications for the reconstruction of paleo-redox conditions based on molybdenum isotopes (2017)
    Elsevier
    In:  Geochimica et Cosmochimica Acta, 213 . pp. 400-417.
    Details
    Publication Date: 2020-02-06
    Description: The concentration and isotope composition of molybdenum (Mo) in sediments and sedimentary rocks are widely used proxies for anoxic conditions in the water column of paleo-marine systems. While the mechanisms leading to Mo fixation in modern restricted basins with anoxic and sulfidic (euxinic) conditions are reasonably well constrained, few studies have focused on Mo cycling in the context of open-marine anoxia. Here we present Mo data for water column particulate matter, modern surface sediments and a paleo-record covering the last 140,000 years from the Peruvian continental margin. Mo concentrations in late Holocene and Eemian (penultimate interglacial) shelf sediments off Peru range from ∼70 to 100 µg g−1, an extent of Mo enrichment that is thought to be indicative of (and limited to) euxinic systems. To investigate if this putative anomaly could be related to the occasional occurrence of sulfidic conditions in the water column overlying the Peruvian shelf, we compared trace metal (Mo, vanadium, uranium) enrichments in particulate matter from oxic, nitrate-reducing (nitrogenous) and sulfidic water masses. Coincident enrichments of iron (Fe) (oxyhydr)oxides and Mo in the nitrogenous water column as well as co-variation of dissolved Fe and Mo in the sediment pore water suggest that Mo is delivered to the sediment surface by Fe (oxyhydr)oxides. Most of these precipitate in the anoxic-nitrogenous water column due to oxidation of sediment-derived dissolved Fe with nitrate as a terminal electron acceptor. Upon reductive dissolution in the surface sediment, a fraction of the Fe and Mo is re-precipitated through interaction with pore water sulfide. The Fe- and nitrate-dependent mechanism of Mo accumulation proposed here is supported by the sedimentary Mo isotope composition, which is consistent with Mo adsorption onto Fe (oxyhydr)oxides. Trace metal co-variation patterns as well as Mo and nitrogen isotope systematics suggest that the same mechanism of Mo delivery caused the ‘anomalously’ high interglacial Mo accumulation rates in the paleo-record. Our findings suggest that Fe- and nitrate-dependent Mo shuttling under nitrogenous conditions needs to be considered a possible reason for sedimentary Mo enrichments during past periods of widespread anoxia in the open ocean.
    Type: Article , PeerReviewed
    Format: text
    Format: other
    Format: other
    Format: other
    Format: other
    DOI: 10.1016/j.gca.2017.06.048
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