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  • Sea ice  (2)
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  • 1
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    Tropical Pacific influence on the source and transport of marine aerosols to West Antarctica (2014)
    American Meteorological Society
    Details
    Publication Date: 2022-05-26
    Description: Author Posting. © American Meteorological Society, 2014. This article is posted here by permission of American Meteorological Society for personal use, not for redistribution. The definitive version was published in Journal of Climate 27 (2014): 1343–1363, doi:10.1175/JCLI-D-13-00148.1.
    Description: The climate of West Antarctica is strongly influenced by remote forcing from the tropical Pacific. For example, recent surface warming over West Antarctica reflects atmospheric circulation changes over the Amundsen Sea, driven by an atmospheric Rossby wave response to tropical sea surface temperature (SST) anomalies. Here, it is demonstrated that tropical Pacific SST anomalies also influence the source and transport of marine-derived aerosols to the West Antarctic Ice Sheet. Using records from four firn cores collected along the Amundsen coast of West Antarctica, the relationship between sea ice–modulated chemical species and large-scale atmospheric variability in the tropical Pacific from 1979 to 2010 is investigated. Significant correlations are found between marine biogenic aerosols and sea salts, and SST and sea level pressure in the tropical Pacific. In particular, La Niña–like conditions generate an atmospheric Rossby wave response that influences atmospheric circulation over Pine Island Bay. Seasonal regression of atmospheric fields on methanesulfonic acid (MSA) reveals a reduction in onshore wind velocities in summer at Pine Island Bay, consistent with enhanced katabatic flow, polynya opening, and coastal dimethyl sulfide production. Seasonal regression of atmospheric fields on chloride (Cl−) reveals an intensification in onshore wind velocities in winter, consistent with sea salt transport from offshore source regions. Both the source and transport of marine aerosols to West Antarctica are found to be modulated by similar atmospheric dynamics in response to remote forcing. Finally, the regional ice-core array suggests that there is both a temporally and a spatially varying response to remote tropical forcing.
    Description: This research was supported by an award from the Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF) to ASC, a James E. and Barbara V. Moltz Research Fellowship to SBD, and grants from NSF-OPP (ANT- 0632031 and ANT-0631973), NSF-MRI (EAR- 1126217), and the NASA Cryosphere Program (NNX10AP09G), and a WHOI Andrew W. Mellon Foundation Award for Innovative Research.
    Description: 2014-08-01
    Keywords: Antarctica ; Sea ice ; Teleconnections ; Atmosphere-ocean interaction ; Climate records ; Interannual variability
    Repository Name: Woods Hole Open Access Server
    Type: Article
    Format: application/pdf
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  • 2
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    Seasonally resolved ice core records from West Antarctica indicate a sea ice source of sea-salt aerosol and a biomass burning source of ammonium (2014)
    John Wiley & Sons
    Details
    Publication Date: 2022-05-26
    Description: Author Posting. © American Geophysical Union, 2014. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Journal of Geophysical Research: Atmospheres 119 (2014): 9168–9182, doi:10.1002/2013JD020720.
    Description: The sources and transport pathways of aerosol species in Antarctica remain uncertain, partly due to limited seasonally resolved data from the harsh environment. Here, we examine the seasonal cycles of major ions in three high-accumulation West Antarctic ice cores for new information regarding the origin of aerosol species. A new method for continuous acidity measurement in ice cores is exploited to provide a comprehensive, charge-balance approach to assessing the major non-sea-salt (nss) species. The average nss-anion composition is 41% sulfate (SO42−), 36% nitrate (NO3−), 15% excess-chloride (ExCl−), and 8% methanesulfonic acid (MSA). Approximately 2% of the acid-anion content is neutralized by ammonium (NH4+), and the remainder is balanced by the acidity (Acy ≈ H+ − HCO3−). The annual cycle of NO3− shows a primary peak in summer and a secondary peak in late winter/spring that are consistent with previous air and snow studies in Antarctica. The origin of these peaks remains uncertain, however, and is an area of active research. A high correlation between NH4+ and black carbon (BC) suggests that a major source of NH4+ is midlatitude biomass burning rather than marine biomass decay, as previously assumed. The annual peak in excess chloride (ExCl−) coincides with the late-winter maximum in sea ice extent. Wintertime ExCl− is correlated with offshore sea ice concentrations and inversely correlated with temperature from nearby Byrd station. These observations suggest that the winter peak in ExCl− is an expression of fractionated sea-salt aerosol and that sea ice is therefore a major source of sea-salt aerosol in the region.
    Description: This work was supported by grants from the NSF Antarctic Program (0632031 and 1142166), NSF-MRI (1126217), the NASA Cryosphere Program (NNX10AP09G), and by an award from the Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF) to ASC.
    Description: 2015-01-21
    Keywords: Antarctica ; Ice cores ; Biomass burning ; Sea ice ; Nitrate ; Acidity
    Repository Name: Woods Hole Open Access Server
    Type: Article
    Format: application/pdf
    Location Call Number Limitation Availability
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    PAPER (OA)
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