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  • 2015-2019  (3)
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  • 1
    Publication Date: 2019-03-11
    Type: Report , NonPeerReviewed , info:eu-repo/semantics/book
    Format: text
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  • 2
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    Elsevier
    In:  International Journal of Greenhouse Gas Control, 38 . pp. 44-51.
    Publication Date: 2020-10-21
    Description: Highlights • The CO2 bubbles leaked from QICS exp. are detected at diameters from 3 to 12 mm. • Velocities of leaked bubbles are at 20–45 cm/s. • Breakup and coalescence of bubbles are detected by a high-speed camera. • The dynamics of leaked bubbles are analysed in terms of Eötvös and Reynolds numbers. Abstract The dynamic characteristics of CO2 bubbles in Scottish seawater are investigated through observational data obtained from the QICS project. Images of the leaked CO2 bubble plume rising in the seawater were captured. This observation made it possible to discuss the dynamics of the CO2 bubbles in plumes leaked in seawater from the sediments. Utilising ImageJ, an image processing program, the underwater recorded videos were analysed to measure the size and velocity of the CO2 bubbles individually. It was found that most of the bubbles deform to non-spherical bubbles and the measured equivalent diameters of the CO2 bubbles observed near the sea bed are to be between 2 and 12 mm. The data processed from the videos showed that the velocities of 75% of the leaked CO2 bubbles in the plume are in the interval 25–40 cm/s with Reynolds numbers (Re) 500–3500, which are relatively higher than those of an individual bubble in quiescent water. The drag coefficient Cd is compared with numerous laboratory investigations, where agreement was found between the laboratory and the QICS experimental results with variations mainly due to the plume induced vertical velocity component of the seawater current and the interactions between the CO2 bubbles (breakup and coalescence). The breakup of the CO2 bubbles has been characterised and defined by Eötvös number, Eo, and Re.
    Type: Article , PeerReviewed , info:eu-repo/semantics/article
    Format: text
    Format: other
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  • 3
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    Elsevier
    In:  International Journal of Greenhouse Gas Control, 38 . pp. 52-63.
    Publication Date: 2015-07-06
    Description: Highlights • The dynamics of leaked bubble plumes are analysed from the QICS experiment. • Bubble distribution and interaction sub-models validated against experimental data. • Interactions bring simulation results closer to that experienced in the experiment. • Improved small scale two phase model applied to simulate the full QICS experiment. • Limitations from neglecting both topography and the CO2 solution leaked from seabed. Abstract An oceanic two-phase plume model is developed to include bubble size distribution and bubble interactions, applied to the prediction of CO2 bubble plume and CO2 solution dynamics observed from the recent QICS field experiment in the Scottish sea at Ardmucknish Bay. Observations show bubbles form at between 2 and 12 mm in diameter, where the inclusion of the interactions within the simulations brings results of bubble plumes closer to that of the experiment. Under a given leakage flux, simulations show that the bubble size affects the maximum pCO2 dissolved in the water column, while the bubble interactions affect the vertical bubble distribution. The maximum modelled pCO2 increases from a background 360 μatm to 400, 427 and 443 μatm as CO2 injection rates increase from 80, 170 to 208 kg/day respectively at low tide. An increase of the leakage rate to 100% of the injection rate shows the maximum pCO2 could be 713 μatm, approaching the mean pCO2 observed of 740 μatm during the high leakage component of the experiment, suggesting that the flux may be greater than estimated due to the varied flux and activity across the pockmarks during the leakages.
    Type: Article , PeerReviewed , info:eu-repo/semantics/article
    Format: text
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