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  • 1
    Electronic Resource
    Electronic Resource
    [s.l.] : Nature Publishing Group
    Nature 372 (1994), S. 348-351 
    ISSN: 1476-4687
    Source: Nature Archives 1869 - 2009
    Topics: Biology , Chemistry and Pharmacology , Medicine , Natural Sciences in General , Physics
    Notes: [Auszug] The hydroxyl radical is primarily produced by the photodisso-ciation of ozone (O3) by radiation of wavelength near 310 nm in the presence of water vapour. O3+H2O+hv 2OH+O2 OH can then initiate the oxidation of SO2 to sulphuric acid. The production rate, R, of sulphuric acid is thought to be a ...
    Type of Medium: Electronic Resource
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  • 2
    Publication Date: 2017-10-17
    Description: Decreasing sea ice and increasing marine navigability in northern latitudes have changed Arctic ship traffic patterns in recent years and are predicted to increase annual ship traffic in the Arctic in the future. Development of effective regulations to manage environmental impacts of shipping requires an understanding of ship emissions and atmospheric processing in the Arctic environment. As part of the summer 2014 NETCARE (Network on Climate and Aerosols) campaign, the plume dispersion and gas and particle emission factors of effluents originating from the Canadian Coast Guard icebreaker Amundsen operating near Resolute Bay, NU, Canada, were investigated. The Amundsen burned distillate fuel with 1.5 wt% sulfur. Emissions were studied via plume intercepts using the Polar 6 aircraft measurements, an analytical plume dispersion model, and using the FLEXPART-WRF Lagrangian particle dispersion model. The first plume intercept by the research aircraft was carried out on 19 July 2014 during the operation of the Amundsen in the open water. The second and third plume intercepts were carried out on 20 and 21 July 2014 when the Amundsen had reached the ice edge and operated under ice-breaking conditions. Typical of Arctic marine navigation, the engine load was low compared to cruising conditions for all of the plume intercepts. The measured species included mixing ratios of CO2, NOx, CO, SO2, particle number concentration (CN), refractory black carbon (rBC), and cloud condensation nuclei (CCN). The results were compared to similar experimental studies in mid-latitudes. Plume expansion rates were calculated using the analytical model and found to be D0.75+0.81, 0.93+0.37, and 1.19+0.39 for plumes 1, 2, and 3, respectively. These rates were smaller than prior studies conducted at mid-latitudes, likely due to polar boundary layer dynamics, including reduced turbulent mixing compared to mid- latitudes. All emission factors were in agreement with prior observations at low engine loads in mid-latitudes. Ice-breaking increased the NOx emission factor from EFNOx 43.1+15.2 to 71.6+9.68 and 71.4+4.14 g kg-diesel-1 for plumes 1, 2, and 3, likely due to changes in combustion temperatures. The CO emission factor was EFCO 137+120, 12.5+3.70 and 8.13+1.34 g kg-diesel-1 for plumes 1, 2, and 3. The rBC emission factor was EFrBC D0.202+0.052 and 0.202+0.125 g kg-diesel-1 for plumes 1 and 2. The CN emission factor was reduced while ice-breaking from EFCN 2.41+0.47 to 0.45+0.082 and 0.507+0.037+1016 kg-diesel+1 for plumes 1, 2, and 3. At 0.6% supersaturation, the CCN emission factor was comparable to observations in mid-latitudes at low engine loads with EFCCN D3.03+0.933, 1.39+0.319, and 0.650+0.136+1014 kg-diesel-1 for plumes 1, 2, and 3.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , peerRev
    Format: application/pdf
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  • 3
    Publication Date: 2022-03-22
    Description: Integrative and Comprehensive Understanding on Polar Environments (iCUPE) project developed 24 novel datasets utilizing in-situ observational capacities within the Arctic or remote sensing observations from ground or from space. The datasets covered atmospheric, cryospheric, marine, and terrestrial domains. This paper connects the iCUPE datasets to United Nations’ Sustainable Development Goals and showcases the use of selected datasets as knowledge provision services for policy- and decision-making actions. Inclusion of indigenous and societal knowledge into the data processing pipelines enables a feedback mechanism that facilitates data driven public services.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev , info:eu-repo/semantics/article
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  • 4
    Publication Date: 2022-01-31
    Description: The cryosphere, which comprises a large portion of Earth’s surface, is rapidly changing as a consequence of global climate change. Ice, snow, and frozen ground in the polar and alpine regions of the planet are known to directly impact atmospheric composition, which for example is observed in the large influence of ice and snow on polar boundary layer chemistry. Atmospheric inputs to the cryosphere, including aerosols, nutrients, and contaminants, are also changing in the anthropocene thus driving cryosphere-atmosphere feedbacks whose understanding is crucial for understanding future climate. Here, we present the Cryosphere and ATmospheric Chemistry initiative (CATCH) which is focused on developing new multidisciplinary research approaches studying interactions of chemistry, biology, and physics within the coupled cryosphere – atmosphere system and their sensitivity to environmental change. We identify four key science areas: (1) micro-scale processes in snow and ice, (2) the coupled cryosphere-atmosphere system, (3) cryospheric change and feedbacks, and (4) improved decisions and stakeholder engagement. To pursue these goals CATCH will foster an international, multidisciplinary research community, shed light on new research needs, support the acquisition of new knowledge, train the next generation of leading scientists, and establish interactions between the science community and society.
    Type: Article , PeerReviewed , info:eu-repo/semantics/article
    Format: text
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