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  • 1
    Online Resource
    Online Resource
    American Geophysical Union (AGU) ; 2019
    In:  Geophysical Research Letters Vol. 46, No. 13 ( 2019-07-16), p. 7790-7799
    In: Geophysical Research Letters, American Geophysical Union (AGU), Vol. 46, No. 13 ( 2019-07-16), p. 7790-7799
    Abstract: SO 2 injections are simulated in different seasons and latitudes in a fully coupled climate model, resulting in a 5 × 4 space of outcomes Injections in different seasons lead to different patterns of aerosol optical depth due to differences in the stratospheric circulation Injecting only in one season leads to higher global aerosol optical depth than if the same mass were injected over the entire year
    Type of Medium: Online Resource
    ISSN: 0094-8276 , 1944-8007
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2019
    detail.hit.zdb_id: 2021599-X
    detail.hit.zdb_id: 7403-2
    SSG: 16,13
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  • 2
    Online Resource
    Online Resource
    American Geophysical Union (AGU) ; 2019
    In:  Geophysical Research Letters Vol. 46, No. 23 ( 2019-12-16), p. 14153-14163
    In: Geophysical Research Letters, American Geophysical Union (AGU), Vol. 46, No. 23 ( 2019-12-16), p. 14153-14163
    Abstract: We use a large ensemble of simulations to explore high‐latitude climate seasonal shifts under stratospheric aerosol geoengineering Stratospheric aerosol geoengineering would alter seasonal cycle of temperature, snow depth, and sea ice at high latitudes Stratospheric heating and seasonal sunlight variations are two likely mechanisms that cause shifts in high‐latitude seasonal cycle
    Type of Medium: Online Resource
    ISSN: 0094-8276 , 1944-8007
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2019
    detail.hit.zdb_id: 2021599-X
    detail.hit.zdb_id: 7403-2
    SSG: 16,13
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  • 3
    Online Resource
    Online Resource
    American Geophysical Union (AGU) ; 2023
    In:  Geophysical Research Letters Vol. 50, No. 14 ( 2023-07-28)
    In: Geophysical Research Letters, American Geophysical Union (AGU), Vol. 50, No. 14 ( 2023-07-28)
    Abstract: We compare two stratospheric aerosol injection strategies which inject SO 2 at different altitudes to meet the same temperature target The low altitude strategy requires two thirds more injection to provide the same amount of cooling We isolate and quantify the different factors which cause the high altitude injection strategy to cool the surface more efficiently
    Type of Medium: Online Resource
    ISSN: 0094-8276 , 1944-8007
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2023
    detail.hit.zdb_id: 2021599-X
    detail.hit.zdb_id: 7403-2
    SSG: 16,13
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  • 4
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 18, No. 10 ( 2018-05-25), p. 7217-7235
    Abstract: Abstract. Understanding and modeling the large-scale transport of trace gases and aerosols is important for interpreting past (and projecting future) changes in atmospheric composition. Here we show that there are large differences in the global-scale atmospheric transport properties among the models participating in the IGAC SPARC Chemistry–Climate Model Initiative (CCMI). Specifically, we find up to 40 % differences in the transport timescales connecting the Northern Hemisphere (NH) midlatitude surface to the Arctic and to Southern Hemisphere high latitudes, where the mean age ranges between 1.7 and 2.6 years. We show that these differences are related to large differences in vertical transport among the simulations, in particular to differences in parameterized convection over the oceans. While stronger convection over NH midlatitudes is associated with slower transport to the Arctic, stronger convection in the tropics and subtropics is associated with faster interhemispheric transport. We also show that the differences among simulations constrained with fields derived from the same reanalysis products are as large as (and in some cases larger than) the differences among free-running simulations, most likely due to larger differences in parameterized convection. Our results indicate that care must be taken when using simulations constrained with analyzed winds to interpret the influence of meteorology on tropospheric composition.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2018
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 5
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 21, No. 13 ( 2021-07-06), p. 10039-10063
    Abstract: Abstract. We present here results from the Geoengineering Model Intercomparison Project (GeoMIP) simulations for the experiments G6sulfur and G6solar for six Earth system models participating in the Climate Model Intercomparison Project (CMIP) Phase 6. The aim of the experiments is to reduce the warming that results from a high-tier emission scenario (Shared Socioeconomic Pathways SSP5-8.5) to that resulting from a medium-tier emission scenario (SSP2-4.5). These simulations aim to analyze the response of climate models to a reduction in incoming surface radiation as a means to reduce global surface temperatures, and they do so either by simulating a stratospheric sulfate aerosol layer or, in a more idealized way, through a uniform reduction in the solar constant in the model. We find that over the final two decades of this century there are considerable inter-model spreads in the needed injection amounts of sulfate (29 ± 9 Tg-SO2/yr between 2081 and 2100), in the latitudinal distribution of the aerosol cloud and in the stratospheric temperature changes resulting from the added aerosol layer. Even in the simpler G6solar experiment, there is a spread in the needed solar dimming to achieve the same global temperature target (1.91 ± 0.44 %). The analyzed models already show significant differences in the response to the increasing CO2 concentrations for global mean temperatures and global mean precipitation (2.05 K ± 0.42 K and 2.28 ± 0.80 %, respectively, for SSP5-8.5 minus SSP2-4.5 averaged over 2081–2100). With aerosol injection, the differences in how the aerosols spread further change some of the underlying uncertainties, such as the global mean precipitation response (−3.79 ± 0.76 % for G6sulfur compared to −2.07 ± 0.40 % for G6solar against SSP2-4.5 between 2081 and 2100). These differences in the behavior of the aerosols also result in a larger uncertainty in the regional surface temperature response among models in the case of the G6sulfur simulations, suggesting the need to devise various, more specific experiments to single out and resolve particular sources of uncertainty. The spread in the modeled response suggests that a degree of caution is necessary when using these results for assessing specific impacts of geoengineering in various aspects of the Earth system. However, all models agree that compared to a scenario with unmitigated warming, stratospheric aerosol geoengineering has the potential to both globally and locally reduce the increase in surface temperatures.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 6
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 21, No. 6 ( 2021-03-19), p. 4231-4247
    Abstract: Abstract. Solar geoengineering has been receiving increased attention in recent years as a potential temporary solution to offset global warming. One method of approximating global-scale solar geoengineering in climate models is via solar reduction experiments. Two generations of models in the Geoengineering Model Intercomparison Project (GeoMIP) have now simulated offsetting a quadrupling of the CO2 concentration with solar reduction. This simulation is idealized and designed to elicit large responses in the models. Here, we show that energetics, temperature, and hydrological cycle changes in this experiment are statistically indistinguishable between the two ensembles. Of the variables analyzed here, the only major differences involve highly parameterized and uncertain processes, such as cloud forcing or terrestrial net primary productivity. We conclude that despite numerous structural differences and uncertainties in models over the past two generations of models, including an increase in climate sensitivity in the latest generation of models, the models are consistent in their aggregate climate response to global solar dimming.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 7
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 22, No. 5 ( 2022-03-04), p. 2955-2973
    Abstract: Abstract. Studies of stratospheric solar geoengineering have tended to focus on modification of the sulfuric acid aerosol layer, and almost all climate model experiments that mechanistically increase the sulfuric acid aerosol burden assume injection of SO2. A key finding from these model studies is that the radiative forcing would increase sublinearly with increasing SO2 injection because most of the added sulfur increases the mass of existing particles, resulting in shorter aerosol residence times and aerosols that are above the optimal size for scattering. Injection of SO3 or H2SO4 from an aircraft in stratospheric flight is expected to produce particles predominantly in the accumulation-mode size range following microphysical processing within an expanding plume, and such injection may result in a smaller average stratospheric particle size, allowing a given injection of sulfur to produce more radiative forcing. We report the first multi-model intercomparison to evaluate this approach, which we label AM-H2SO4 injection. A coordinated multi-model experiment designed to represent this SO3- or H2SO4-driven geoengineering scenario was carried out with three interactive stratospheric aerosol microphysics models: the National Center for Atmospheric Research (NCAR) Community Earth System Model (CESM2) with the Whole Atmosphere Community Climate Model (WACCM) atmospheric configuration, the Max-Planck Institute's middle atmosphere version of ECHAM5 with the HAM microphysical module (MAECHAM5-HAM) and ETH's SOlar Climate Ozone Links with AER microphysics (SOCOL-AER) coordinated as a test-bed experiment within the Geoengineering Model Intercomparison Project (GeoMIP). The intercomparison explores how the injection of new accumulation-mode particles changes the large-scale particle size distribution and thus the overall radiative and dynamical response to stratospheric sulfur injection. Each model used the same injection scenarios testing AM-H2SO4 and SO2 injections at 5 and 25 Tg(S) yr−1 to test linearity and climate response sensitivity. All three models find that AM-H2SO4 injection increases the radiative efficacy, defined as the radiative forcing per unit of sulfur injected, relative to SO2 injection. Increased radiative efficacy means that when compared to the use of SO2 to produce the same radiative forcing, AM-H2SO4 emissions would reduce side effects of sulfuric acid aerosol geoengineering that are proportional to mass burden. The model studies were carried out with two different idealized geographical distributions of injection mass representing deployment scenarios with different objectives, one designed to force mainly the midlatitudes by injecting into two grid points at 30∘ N and 30∘ S, and the other designed to maximize aerosol residence time by injecting uniformly in the region between 30∘ S and 30∘ N. Analysis of aerosol size distributions in the perturbed stratosphere of the models shows that particle sizes evolve differently in response to concentrated versus dispersed injections depending on the form of the injected sulfur (SO2 gas or AM-H2SO4 particulate) and suggests that prior model results for concentrated injection of SO2 may be strongly dependent on model resolution. Differences among models arise from differences in aerosol formulation and differences in model dynamics, factors whose interplay cannot be easily untangled by this intercomparison.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2022
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 8
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 19, No. 15 ( 2019-08-12), p. 10087-10110
    Abstract: Abstract. We have derived values of the ultraviolet index (UVI) at solar noon using the Tropospheric Ultraviolet Model (TUV) driven by ozone, temperature and aerosol fields from climate simulations of the first phase of the Chemistry-Climate Model Initiative (CCMI-1). Since clouds remain one of the largest uncertainties in climate projections, we simulated only the clear-sky UVI. We compared the modelled UVI climatologies against present-day climatological values of UVI derived from both satellite data (the OMI-Aura OMUVBd product) and ground-based measurements (from the NDACC network). Depending on the region, relative differences between the UVI obtained from CCMI/TUV calculations and the ground-based measurements ranged between −5.9 % and 10.6 %. We then calculated the UVI evolution throughout the 21st century for the four Representative Concentration Pathways (RCPs 2.6, 4.5, 6.0 and 8.5). Compared to 1960s values, we found an average increase in the UVI in 2100 (of 2 %–4 %) in the tropical belt (30∘ N–30∘ S). For the mid-latitudes, we observed a 1.8 % to 3.4 % increase in the Southern Hemisphere for RCPs 2.6, 4.5 and 6.0 and found a 2.3 % decrease in RCP 8.5. Higher increases in UVI are projected in the Northern Hemisphere except for RCP 8.5. At high latitudes, ozone recovery is well identified and induces a complete return of mean UVI levels to 1960 values for RCP 8.5 in the Southern Hemisphere. In the Northern Hemisphere, UVI levels in 2100 are higher by 0.5 % to 5.5 % for RCPs 2.6, 4.5 and 6.0 and they are lower by 7.9 % for RCP 8.5. We analysed the impacts of greenhouse gases (GHGs) and ozone-depleting substances (ODSs) on UVI from 1960 by comparing CCMI sensitivity simulations (1960–2100) with fixed GHGs or ODSs at their respective 1960 levels. As expected with ODS fixed at their 1960 levels, there is no large decrease in ozone levels and consequently no sudden increase in UVI levels. With fixed GHG, we observed a delayed return of ozone to 1960 values, with a corresponding pattern of change observed on UVI, and looking at the UVI difference between 2090s values and 1960s values, we found an 8 % increase in the tropical belt during the summer of each hemisphere. Finally we show that, while in the Southern Hemisphere the UVI is mainly driven by total ozone column, in the Northern Hemisphere both total ozone column and aerosol optical depth drive UVI levels, with aerosol optical depth having twice as much influence on the UVI as total ozone column does.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2019
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 9
    In: Nature Communications, Springer Science and Business Media LLC, Vol. 9, No. 1 ( 2018-01-15)
    Abstract: The Montreal Protocol has succeeded in limiting major ozone-depleting substance emissions, and consequently stratospheric ozone concentrations are expected to recover this century. However, there is a large uncertainty in the rate of regional ozone recovery in the Northern Hemisphere. Here we identify a Eurasia-North America dipole mode in the total column ozone over the Northern Hemisphere, showing negative and positive total column ozone anomaly centres over Eurasia and North America, respectively. The positive trend of this mode explains an enhanced total column ozone decline over the Eurasian continent in the past three decades, which is closely related to the polar vortex shift towards Eurasia. Multiple chemistry-climate-model simulations indicate that the positive Eurasia-North America dipole trend in late winter is likely to continue in the near future. Our findings suggest that the anticipated ozone recovery in late winter will be sensitive not only to the ozone-depleting substance decline but also to the polar vortex changes, and could be substantially delayed in some regions of the Northern Hemisphere extratropics.
    Type of Medium: Online Resource
    ISSN: 2041-1723
    Language: English
    Publisher: Springer Science and Business Media LLC
    Publication Date: 2018
    detail.hit.zdb_id: 2553671-0
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  • 10
    Online Resource
    Online Resource
    Copernicus GmbH ; 2021
    In:  Atmospheric Chemistry and Physics Vol. 21, No. 11 ( 2021-06-08), p. 8615-8635
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 21, No. 11 ( 2021-06-08), p. 8615-8635
    Abstract: Abstract. A known adverse side effect of stratospheric aerosol modification (SAM) is the alteration of the quasi-biennial oscillation (QBO), which is caused by the stratospheric heating associated with an artificial aerosol layer. Multiple studies found the QBO to slow down or even completely vanish for point-like injections of SO2 at the Equator. The cause for this was found to be a modification of the thermal wind balance and a stronger tropical upwelling. For other injection strategies, different responses of the QBO have been observed. A theory which is able to explain those differences in a comprehensive manner has not yet been presented. This is further complicated by the fact that the simulated QBO response is highly sensitive to the used model even under identical boundary conditions. Therefore, within this study we investigate the response of the QBO to SAM for three different injection strategies (point-like injection at the Equator, point-like injection at 30∘ N and 30∘ S simultaneously, and areal injection into a 60∘ wide belt along the Equator). Our simulations confirm that the QBO response significantly depends on the injection location. Based on the thermal wind balance, we demonstrate that this dependency is explained by differences in the meridional structure of the aerosol-induced stratospheric warming, i.e., the location and meridional extension of the maximum warming. Additionally, we also tested two different injection species (SO2 and H2SO4). The QBO response is qualitatively similar for both investigated injection species. Comparing the results to corresponding results of a second model, we further demonstrate the generality of our theory as well as the importance of an interactive treatment of stratospheric ozone for the simulated QBO response.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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