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    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 88 (1988), S. 4788-4799 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The UV photolysis of HN3 at 193 nm was investigated in detail in the bulk phase at 300 K. NH radicals in the X, a, b, A, and c states were found to be formed with quantum yields ≤0.0019, 0.4, 0.017, 0.000 15, and 0.000 61, respectively. Relative rotational and vibrational populations were measured for all states except for NH(X). Average translational energies were estimated for NH(a,v=0 and 1) and NH(b,v=0). The 248 nm photolysis of HN3 was reinvestigated with respect to processes forming NH radicals other than NH(a). The observed energy distributions differ for both laser wavelengths and for high and low lying NH states. The distribution can be better described by a simple impulsive than by a statistical model. Some conclusions are drawn concerning the upper HN3 potential surfaces involved.
    Type of Medium: Electronic Resource
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