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    Online Resource
    Online Resource
    Royal Society of Chemistry (RSC) ; 2022
    In:  Physical Chemistry Chemical Physics Vol. 24, No. 40 ( 2022), p. 24873-24880
    In: Physical Chemistry Chemical Physics, Royal Society of Chemistry (RSC), Vol. 24, No. 40 ( 2022), p. 24873-24880
    Abstract: Two-dimensional ferromagnetic (FM) half-metals are promising candidates for advanced spintronic devices with small size and high capacity. Motivated by a recent report on controlling the synthesis of FM Cr 3 Te 4 nanosheets, herein, to explore their potential application in spintronics, we designed spintronic devices based on Cr 3 X 4 (X = Se, Te) monolayers and investigated their spin transport properties. We found that the Cr 3 Te 4 monolayer based device shows spin filtering and a dual-spin diode effect when applying a bias voltage, while the Cr 3 Se 4 monolayer is an excellent platform to realize a spin valve. These different transport properties are primarily ascribed to the semiconducting spin channel, which is close to and away from the Fermi level in Cr 3 Te 4 and Cr 3 Se 4 monolayers, respectively. Interestingly, the current in the Cr 3 Se 4 monolayer based device also displays a negative differential resistance effect (NDRE) and a high magnetoresistance ratio (up to 2 × 10 3 ). Moreover, we found a thermally induced spin filtering effect and a NDRE at the Cr 3 Se 4 junction under a temperature gradient instead of a bias voltage. These theoretical findings highlight the potential of Cr 3 X 4 (X = Se, Te) monolayers in spintronic applications and put forward realistic materials to realize nanoscale spintronic devices.
    Type of Medium: Online Resource
    ISSN: 1463-9076 , 1463-9084
    Language: English
    Publisher: Royal Society of Chemistry (RSC)
    Publication Date: 2022
    detail.hit.zdb_id: 1476283-3
    detail.hit.zdb_id: 1476244-4
    detail.hit.zdb_id: 1460656-2
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