Abstract
We investigate a Bose–Einstein condensate of F = 187Rb atoms in a 2D spin-dependent optical lattice generated by intersecting laser beams with a superposition of polarizations. For 87Rb the effective interaction of an atom with the electromagnetic field contains scalar and vector (called a fictitious magnetic field, Bfic) potentials. The Rb atoms behave as a quantum rotor (QR) with angular momentum given by the sum of the atomic rotational motion angular momentum and the hyperfine spin. The ground state of the QR is affected upon applying an external magnetic field, Bext, perpendicular to the plane of QR motion and a sudden change of its topology occurs as the ratio Bext/Bfic exceeds a critical value. It is shown that the change of topology of the QR ground state is a result of combined action of Zeeman and Einstein–de Haas effects. The first transfers atoms to the largest hyperfine component to polarize the sample along the field as the external magnetic field is increased. The second sweeps spin to rotational angular momentum, modifying the kinetic energy of the atoms.
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1. Introduction
Ever since the experimental realization of Bose–Einstein condensates (BECs), they have proven to be an ideal platform for study of various effects of quantum many-body interaction. One of the milestones in experimental studies of BEC was the application of all optical traps [1] which liberated atom spin degrees of freedom from the trapping mechanism and allowed for much richer internal structures and dynamics of the BEC. The study of spinor BECs involves the interplay of spin–spin interactions, magnetization, topology, symmetry, homotopy, spin-gauge coupling, and magnetic solitons, etc, making it an incredibly fertile and promising research area [2–11]. For these studies important characteristics are spin textures and vortex spin textures in spinor BECs [12], which are related to superfluidity (see reference [13] for references) and topological states in condensed matter physics [14]. In our study we investigate bosonic cold atoms subject to a 2D spin-dependent optical lattice potential (SDOLP) in the context of spin textures and transition of the ground state topology (i.e., a change of symmetry of the many-body state upon varying an external parameter). First we focus on the limit of singly occupied lattice sites and then on the limit of many atoms per lattice site, but the atoms are condensed such that the tunneling rate out of the sites is negligible (the so-called insulating regime). The superfluid phase, when tunneling between lattices sites are involved is also very exciting and will be the subject of future work. Our work is closely related to the Einstein–de Haas (EdH) effect in BECs [15–18], where transfer of atoms to other Zeeman states can be observed due to dipolar interactions, which couple the spin and the orbital degrees of freedom.
The concept of a 'ficticious magnetic field' for describing the vector component of the tensor polarizibility was first introduced by Cohen–Tannoudji in reference [19]. It was later applied for quantum state control in optical lattices by Deutsch and Jessen [20, 21] and for dispersive quantum measurement of multilevel atoms [22]. It also led to engineering novel optical lattices [23]. For studies of alkali atoms in spin-dependent optical lattices created by elliptically polarized light beams see reference [24]. Recently a study of fermionic atoms in a 2D SDOLP in the limit of singly occupied sites was carried out in reference [25]. In addition to determining the wave functions and energy levels of the atoms in the SDOLP, it was shown that such systems could be used as high precision rotation sensors, accelerometers, and magnetometers. Here we consider bosonic atoms and focus on the case of a BEC in the insulating regime. Explicitly, we consider a BEC consisting of 87Rb atoms in a spin-dependent optical lattice potential SDOLP. We show that by applying an external magnetic field, the properties of the system are significantly enriched and a radical change of the topological properties of the ground state can be observed as the strength of the external field is varied.
2. Model
We consider 87Rb atoms in a 2D SDOLP created by six laser beams, which are tightly focused in the z direction, as proposed in reference [25]. The slowly varying electric field envelope is given by , where is the unit polarization vector along the z-axis and the wave vectors are where λl is the laser wavelength. For 87Rb, where the total electronic angular momentum is J = 1/2, the effective interaction of an atom with the electromagnetic field can be described using a scalar potential V and fictitious magnetic field [25] (i.e., a vector potential), since the tensor terms vanish [see supplemental material (SM) (https://stacks.iop.org/NJP/24/033041/mmedia) [26]],
where is the atomic hyperfine angular momentum, μB is the Bohr magneton, g = 1/2, and
Here α0 and α1 are scalar and vector polarizabilities. Figure 1 shows full hexagonal potentials which are isotropic close to the site center. In the current study we focus on single site effects and assume that atomic wave function is well localized to only the center of the site, hence even though the lattice has hexagonal symmetry, potentials can be treated as isotropic (see reference [25] and the SM). Note that the divergence of the fictitious magnetic field does not vanish and corresponds to radially distributed magnetic monopole density.
First, we solve the Schrödinger equation for a single atom in a lattice cell in the presence of an additional uniform magnetic field Bext and find the energy eigenvalues and eigenfunctions. The projections of F, the orbital angular momentum of the atom about the SDOLP minimum ℓ , and the total angular momentum of the QR (where ), on the z-axis are mF, mℓ and ζ = mF + mℓ respectively. Close to the potential minimum at in a strong enough laser field the SDOLP is radially symmetric, which allows to classify energy eigenstates using principal quantum number n (n = 0, 1, 2, ...) and projection of the total angular momentum on the z axis ζ = 0, ±1, ±2, .... For details of the single-atom system see supplemental material.
Next we model a BEC of 87Rb atoms in the F = 1 state in the electromagnetic field generated by the lasers that form the SDOLP in the x–y plane (the width of the SDOLP in the z-direction is the smallest length scale, which is of order of laser wavelength λl, our unit of length) in the presence of an external magnetic field transverse to the SDOLP. The BEC ground state wave function is also an eigenstate of with eigenvalue ζ. Both spin and orbital angular momentum contribute to ζ, therefore it describes the topology of the BEC spinor components, i.e., their vortex structure. We show that an external magnetic field applied along the symmetry axis leads to a transition in which the ground state switches from ζ = 0 to ζ = 1 state as the external magnetic field varies. As both states are protected by the symmetry, this transition must be triggered by fluctuations that break the axial symmetry.
Atoms in the BEC interact by contact forces with both spin-dependent and spin-independent contributions, which are expressed by the coefficients c0 and c2 respectively, related to the scattering lengths a0 and a2, as follows: c0 = 4πℏ2(a0 + 2a2)/3m and c2 = 4πℏ2(a2 − a0)/3m. For 87Rb, a0 = 5.387 nm and a2 = 5.313 nm. The scattering length a0 parameterizes the interactions where two colliding atoms have a total spin atomic angular momentum Ftot = 0, while a2 corresponds to Ftot = 2 [3, 27]. Since our calculations are 2D, we renormalize c0 and c2 by dividing them by the vertical extend of the BEC: c0, c2 → c0/λl, c2/λl. The Hamiltonian density for an F = 1 spinor with linear Zeeman splitting induced by an external magnetic field is [4–6]
Here, is a vector composed of the field annihilation operators for an atom at point , in the hyperfine state components mF = 1, 0, and −1 respectively, m is the mass of the particles, F is the total spin atomic angular momentum vector and each component is a 3 × 3 spin-1 matrix (with Fz being a diagonal tensor), Bext is the magnitude of the (uniform) external magnetic field in the z-direction, and the last term is the linear Zeeman Hamiltonian [4].
2.1. BEC in a lattice site
The 87Rb BEC in the hyperfine F = 1 state is trapped in the SDOLP with tight confinement in the z direction. The strength of the SDOLP is determined by the intensity of laser beams, which we take to be 70 W cm−2, and the wavelength of the laser beams is taken as λl = 795 nm. We assume that there is an additional transverse external magnetic field Bext in the z direction whose strength can be tuned. Then, assuming the mean-field approximation applies, we use the imaginary-time technique [28] to find the ground state wave functions (order parameters) of a QR BEC. The wave functions form a three component spinor .
We set the total number of atoms to N = 100, and vary the external magnetic field strength in the range from 0 mG to 100 mG. In figure 2 we follow the ground state of the QR as the external magnetic field is increased, and plot the number of atoms in each spinor component as a function of external magnetic field. With Bext = 0, the mF = 0 component is the most populated, while equal number of atoms occupy the mF = ±1. This distribution is selected to minimize interaction with fictitious magnetic field. As the external magnetic field increases, atoms move from the mF = −1 and mF = 0 components to the mF = +1. This happens since the energy of a magnetic dipole gets lower when a dipole moment is oriented in the same direction as an external magnetic field. In our case Bext is oriented in the direction, which favors the mF = +1 component. As we can see from figure 2, for a certain value of Bext the number of atoms and atomic angular momentum as a function of Bext is not continuous, which is an indication of an abrupt transition. After this transition the occupation of the mF = +1 component is the largest, and there are very few atoms left in the mF = −1. In the lower panel of figure 2 we present z component of the total angular momentum, atomic hyperfine spin ⟨Fz ⟩, and the modulus of the atomic orbital angular momentum, ⟨|ℓz |⟩, calculated for the full three-component spinor as a function of external magnetic field. Orbital angular momentum per atom in mF = +1, 0, −1 spinor components before the transition is equal to mℓ = −1, 0, 1 and after the transition it changes to mℓ = 0, 1, 2, respectively.
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Standard image High-resolution imageIn the following we focus on differences in the characteristics of atom distributions (figure 3) and spin distributions (figure 4) before and after transition. Ground state density and the phase for all three spinor components are shown in figure 3, where the left column corresponds to the value of external magnetic field equal to Bext = 40 mG. We see that the density of the mF = +1 component at the position for this value of the magnetic field is equal to zero. The same is true for mF = −1, but not in mF = 0, where only a shallow minimum at is present. All density and phase profiles are in compliance with the expectation values of the orbital angular momentum per atom about the minimum of the SDOLP , which is equal to −ℏ, 0, +ℏ, for the mF = +1, 0, −1 spinor components of the ground state wave function at this value of Bext.
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Standard image High-resolution imageIn the right column of figure 3 we present analogous results for the value of external magnetic field Bext = 100 mG, above the transformation. The difference is evident since now the mF = +1 state has a Gaussian-like shape, which together with the phase structure indicates no vortex in this component. We calculated the expectation value of the atomic orbital angular momentum for each component and this time obtained values 0, ℏ, 2ℏ for the mF = +1, 0, −1 respectively. Comparing states (densities and phases) before and after the transition we see increase of angular momentum per atom by ℏ in each component. It is only possible if the components in left column belong to the ζ = 0 and in the right column to ζ = 1 states. Regardless of the distribution of atoms among the three spinor components, the expectation value of ζ = mF + mℓ per atom is equal to zero in the left column and one in the right column of figure 3. So at each particular value of Bext it is the same in each mF component, because of symmetry. This is in fact the analogue of the celebrated EdH effect [29], a manifestation of the fact that spin contributes to the total angular momentum on the equal footing with the rotational angular momentum. This explains why the radical change of the ground state topology occurs (see the discussion below).
In figure 4 we portray the spin textures by constructing vectors of expectation values ⟨Fx ⟩, ⟨Fy ⟩, and ⟨Fz ⟩ in a ground state spinor wave function. The results are shown as a 3D vector plot . Before the transition, the spin vector mainly lies in the x–y plane. After the transition the spin texture changes. In figure 4(b), the spin vector in the vicinity of , where the atoms are mostly located, is turned towards the z direction, trying to along with the external magnetic field. This happens because in this region the external magnetic field is stronger than the vector optical potential. After the transition, and further from the center, the spin vector is still aligned with the vector part of the optical potential. Reorientation of is a clear signature of the change of the ground state of the QR BEC.
3. Origin of the ground state topological transition
To understand the origin of the transition we take a closer look at the behavior of energy contributions for two lowest QR states. In figure 5 we plot the total (solid lines) and kinetic (dashed lines) energies as a function of an external magnetic field for states with indices ζ = 0 (blue) and ζ = 1 (red). The crossing of two solid lines (total energy curves) occurs approximately at Bext = 70 mG at the intensity of I = 70 W cm−2. For a hexagonal lattice geometry with a large number of atoms (N = 100) per lattice site we checked that the transformation occurs at the critical value of Bext/Bfic = 0.7, where Bfic is the magnitude of the fictitious magnetic field, equation (3), by varying the strength of the SDOLP potential (and therefore the strength of the fictitious magnetic field) over a wide range. We know from figure 3 that the topology of the ground state is changed after the crossing point, and the winding number of each spinor component is increased by one.
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Standard image High-resolution imageWhen the ratio of Bext/Bfic field is low atomic spin are mostly in x–y plain and predominantly occupy mF = 0 component, minimizing both kinetic and magnetic energies. Above the critical ratio, atoms in the ground state are moved to the mF = +1 component to minimize magnetic energy. However, the topology of the mF = +1 component is different for ζ = 0 and ζ = 1 states; the former carries 'charge' −1 vortex, while the latter has no vortex at all. There is an extra rotational kinetic energy in a vortex state, hence transferring atoms to the mF = +1 component results in the increase of the kinetic energy in ζ = 0 state and decrease in the ζ = 1 state. These two kinetic energies cross in figure 5 and the crossing point is located in the close vicinity to the crossing of total energies. Since all the other energy components (Zeeman and SDOLP field) of two lowest QR states change with external magnetic field in a similar way for both ζ = 0 and ζ = 1 states, it is exactly kinetic energy that is responsible for the transition. For this transition to occur a symmetry breaking perturbation is required.
4. Conclusions
We proposed a realization of a quantum rotor system, based on a BEC of 87Rb atoms in a 2D spin-dependent optical lattice potential. When enriched by adding a transverse external magnetic field, the system exhibits a topological transition of the ground state as a function of the strength of the external magnetic field. One observes the change of the topology of the quantum rotor BEC ground state; it switches from the one at low magnetic fields corresponding to the rotor angular momentum ζ = 0, to ζ = 1 at higher field strengths. The reason for this change is related to the transfer of atoms triggered by the external magnetic field, which combined with the EdH effect, leads to the subtle interplay between various energy components in the two lowest quantum rotor states. These two distinct ground states can be observed in experiment by measuring the density profiles of different components following Stern–Gerlach separation. Extensions of this work to consider both sides of the superconductor-insulating transition regimes and other spin-dependent optical lattice potential geometries are in progress. Although in this study we do not consider dynamics, but rather the states of the system at specific magnetic field strengths, it may be useful to study dynamics as the magnetic field strength varies in time.
Acknowledgments
MT was supported by the Polish National Science Center (NCN) Grant 2016/22/M/ST2/00261. MB and MG were supported by the NCN Grant No. 2019/32/Z/ST2/00016 through the project MAQS under QuantERA, which has received funding from the European Union's Horizon 2020 research and innovation program under Grant Agreement No. 731473. PS was supported in part by the National Science Centre (NCN), Grant No. 2017/25/B/ST2/01943.
Data availability statement
The data that support the findings of this study are available upon reasonable request from the authors.