Abstract
Purpose
The results of sediment source tracing in large river catchments depend on defined sources being adequately represented by the sampling and in subsequent numerical analysis. We hypothesise that surface soil concentrations of fallout radionuclides caesium-137 (137Cs) and lead-210 excess (210Pbex) are smaller at locations with higher soil erosion rate and that if this is not accounted for, then spatially random sampling gives a biased representation of surface soil delivered to rivers and biased source contribution estimates.
Materials and methods
Surface soil was sampled across the Burdekin River basin in northeast Australia at 90 locations stratified by three classes of modelled soil erosion rate and analysed by gamma spectroscopy. Separate probability distributions (density functions) were fitted to the 137Cs concentrations of samples of each erosion class, of subsurface soil and of river sediment. Surface soil distributions were aggregated by weighting in proportion to the upstream area and mean erosion rate of each erosion class, so that the high erosion class contributed disproportionately to the tracer properties of the surface soil source. Source contributions were estimated using a Monte Carlo mixing model.
Results and discussion
The mean surface soil concentrations of 137Cs and 210Pbex were significantly different between soil erosion classes as hypothesised. Weighting surface soil from the high erosion class more heavily increased the estimated proportion of river sediment contributed from surface soil, by 35 % larger than if surface soil sampling was confined to low erosion areas. Stratified sampling and weighting by erosion rate is of greater importance in river basins with large gradients in soil erosion and where surface soil contributes substantially to river sediment. Surface soil contributed 6 % to fine sediment at the basin outlet and 0–14 % in major tributaries, which was somewhat lower than in a prior study probably due to recent above-average rainfall increasing vegetation ground cover.
Conclusions
Surface soil sampling for source tracing using fallout radionuclides should be stratified by erosion rate. The tracer properties of high erosion areas should be weighted more heavily than low erosion areas in source mixing models. If comprehensive sampling cannot be afforded, then sampling should be biased towards more highly eroding areas. The approach should be considered for other source tracers whose properties may co-vary with soil erosion rate. Fine sediment delivered from the Burdekin River basin to the Great Barrier Reef lagoon in recent decades was predominantly derived from gully erosion, streambank erosion and rilled and scalded areas on hillslopes.
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References
Bainbridge ZT, Wolanski E, Ãlvarez-Romero JG, Lewis SE, Brodie JE (2012) Fine sediment and nutrient dynamics related to particle size and floc formation in a Burdekin River flood plume, Australia. Mar Pollut Bull 65:236–248
Bainbridge ZT, Lewis SE, Smithers SG, Kuhnert PM, Henderson BL, Brodie JE (2014) Fine suspended sediment and water budget for a large, seasonally-dry tropical catchment: Burdekin River catchment, Queensland, Australia. Water Resour Res 50:9067–9087
Bartley R, Hawdon A, Post DA, Roth CH (2007) A sediment budget for a grazed semi-arid catchment in the Burdekin Basin, Australia. Geomorphology 87:302–321
Bartley R, Bainbridge ZT, Lewis SE, Kroon FJ, Wilkinson SN, Brodie JE, Silburn DM (2014a) Relating sediment impacts on coral reefs to watershed sources, processes and management: a review. Sci Total Environ 15:468–469
Bartley R, Corfield JP, Hawdon AA, Kinsey-Henderson AE, Abbott BN, Wilkinson SN, Keen RJ (2014b) Can improved pasture management reduce runoff and sediment loss to the Great Barrier Reef? The results of a 10 year study in the Burdekin catchment, Australia. Rangel J 36:67–84
Basher LR, Matthews KM (1993) Relationship between Cs-137 in some undisturbed New-Zealand soils and rainfall. Aust J Soil Res 31:655–663
Blake WH, Wallbrink PJ, Wilkinson SN, Humphreys GS, Doerr SH, Shakesby RA, Tomkins KM (2009) Deriving hillslope sediment budgets in wildfire-affected forests using fallout radionuclide tracers. Geomorphology 104:105–116
Boomer KB, Weller DE, Jordan TE (2008) Empirical models based on the universal soil loss equation fail to predict sediment discharges from Chesapeake bay catchments. J Environ Qual 37:79–89
Caitcheon G, Olley JM, Pantus F, Hancock GJ, Leslie C (2012) The dominant erosion processes supplying fine sediment to three major rivers in tropical Australia, the Daly (NT), Mitchell (Qld) and Flinders (Qld) Rivers. Geomorphology 151–152:188–195
Carroll C, Waters D, Vardy S, Silburn DM, Attard S, Thorburn PJ, Davis AM, Halpin N, Schmidt M, Wilson B, Clark A (2012) A paddock to reef monitoring and modelling framework for the Great Barrier Reef: paddock and catchment component. Mar Pollut Bull 65:136–149
Collins AL, Walling DE, Leeks GJL (1997) Source type ascription for fluvial suspended sediment based on a quantitative composite fingerprinting technique. Catena 29:1–29
Collins AL, Anthony SG, Hawley J, Turner T (2009) The potential impact of projected change in farming by 2015 on the importance of the agricultural sector as a sediment source in England and Wales. Catena 79:243–250
De'ath G, Fabricius K (2010) Water quality as a regional driver of coral biodiversity and macroalgae on the Great Barrier Reef. Ecol Appl 20:840–850
Doering C, Akber R, Heijnis H (2006) Vertical distributions of 210Pb excess, 7Be and 137Cs in selected grass covered soils in Southeast Queensland, Australia. J Environ Radioact 87:135–147
Fabricius KE (2005) Effects of terrestrial runoff on the ecology of corals and coral reefs: review and synthesis. Mar Pollut Bull 50:125–146
Franks SW, Rowan JS (2000) Multi-parameter fingerprinting of sediment sources: uncertainty estimation and tracer selection. In: Bentley LR, Brebbia CA, Gray WG, Pinder GF, Sykes JF (eds) Computational methods in water resources. Balkema, Rotterdam, pp 1067–1074
Fry B (2013) Alternative approaches for solving underdetermined isotope mixing problems. Mar Ecol Prog Ser 472:1–13
Gibbs MM (2008) Identifying source soils in contemporary estuarine sediments: a new compound-specific isotope method. Estuar Coasts 31:344–359
Gilad U, Denham R, Tindall D (2012) Gullies, Google Earth and the Great Barrier Reef: a remote sensing methodology for mapping gullies over extensive areas, XXII ISPRS Congress. International Archives of the Photogrammetry, Remote Sensing and Spatial Information Sciences, Volume XXXIX-B8, Melbourne, Australia
Goovaerts P (1997) Geostatistics for natural resources evaluation. Oxford University Press, Oxford, UK
Hamza MA, Anderson WK (2005) Soil compaction in cropping systems—a review of the nature, causes and possible solutions. Soil Tillage Res 82:121–145
Hancock GJ, Wilkinson SN, Hawdon AA, Keen RJ (2014) The use of fallout tracers Be-7, Pb-210 and Cs-137 to distinguish the form of sub-surface soil erosion delivering sediment to rivers in large catchments. Hydrol Process 28:3855–3874
He Q, Walling DE (1997) The distribution of fallout Cs-137 and Pb-210 in undisturbed and cultivated soils. Appl Radiat Isot 48:677–690
Hughes AO, Olley JM, Croke JC, McKergow LA (2009) Sediment source changes over the last 250 years in a dry-tropical catchment, central Queensland, Australia. Geomorphology 104:262–275
Karfs RA, Abbott BN, Scarth PF, Wallace JF (2009) Land condition monitoring information for reef catchments: a new era. Rangel J 31:69–86
Kinsey-Henderson A, Sherman B, Bartley R (2007) Improved SedNet modelling of grazing lands in the Burdekin catchment. Science Report 63/07, CSIRO Land and Water, Canberra, Australia
Kroon FJ, Kuhnert PM, Henderson BL, Wilkinson SN, Kinsey-Henderson A, Abbott B, Brodie JE, Turner DR (2012) River loads of suspended solids, nitrogen, phosphorus and herbicides to the Great Barrier Reef lagoon. Mar Pollut Bull 65:167–181
Kroon F, Turner R, Smith R, Warne M, Hunter H, Bartley R, Wilkinson S, Lewis S, Waters D, Carroll C (2013) Sources of sediment, nutrients, pesticides and other pollutants in the Great Barrier Reef catchment, Chapter 4. In: Brodie J et al (eds) Land use impacts on Great Barrier Reef water quality and ecosystem condition: 2013 Scientific Consensus Statement. The State of Queensland, Brisbane, p 35
Krouse AK, Franks SW, Kalma JD, Loughan RJ, Rowan JS (2003) Multi-parameter fingerprinting of sediment deposition in a small gullied catchment in SE Australia. Catena 53:327–348
Leslie C (2009) Analysing environmental radioactivity in soils and sediments using high-purity germanium gamma detectors at CSIRO Land and Water: procedures and Protocols. CSIRO Land and Water, Canberra
Lewis SE, Bainbridge ZT, Sherman BS, Kuhnert P, Henderson B, Cooper M, Brodie JE (2013) Calculating sediment trapping efficiencies for reservoirs in tropical settings: a case study from the Burdekin Falls Dam, NE Australia. Water Resour Res 49:1017–1029
Lu H, Prosser IP, Moran CJ, Gallant J, Priestley G, Stevenson J (2003) Predicting sheetwash and rill erosion over the Australian continent. Aust J Soil Res 41:1037–1062
Lu H, Moran CJ, Prosser IP, DeRose R (2004) Investment prioritization based on broadscale spatial budgeting to meet downstream targets for suspended sediment loads. Water Resour Res 40:W09501
Mabit L, Bernard C, Laverdière MR (2007) Assessment of erosion in the Boyer River watershed (Canada) using a GIS oriented sampling strategy and 137Cs measurements. Catena 71:242–249
Mabit L, Meusburger K, Fulajtar E, Alewell C (2013) The usefulness of 137Cs as a tracer for soil erosion assessment: a critical reply to Parsons and Foster (2011). Earth Sci Rev 127:300–307
Minasny B, McBratney AB (2006) A conditioned Latin hypercube method for sampling in the presence of ancillary information. Comput Geosci 32:1378–1388
Olley J, Caitcheon G (2000) Major element chemistry of sediments from the Darling-Barwon River and its tributaries: implications for sediment and phosphorus sources. Hydrol Process 14:1159–1175
Olley JM, Murray AS, McKenzie DM, Edwards K (1993) Identification of sediment sources in a gullied catchment using natural and artificial radioactivity. Water Resour Res 29:1037–1043
Olley J, Brooks A, Spencer J, Pietsch T, Borombovits D (2013a) Subsoil erosion dominates the supply of fine sediment to rivers draining into Princess Charlotte Bay, Australia. J Environ Radioact 124:121–129
Olley J, Burton J, Smolders K, Pantus F, Pietsch T (2013b) The application of fallout radionuclides to determine the dominant erosion process in water supply catchments of subtropical South-East Queensland, Australia. Hydrol Process 27:885–895
Owens PN, Walling DE, Leeks GJL (1999) Use of floodplain sediment cores to investigate recent historical changes in overbank sedimentation rates and sediment sources in the catchment of the River Ouse, Yorkshire, UK. Catena 36:21–47
Peart MR, Walling DE (1986) Fingerprinting sediment source: the example of a drainage basin in Devon, U.K. In: Hadley RF (ed) Drainage Basin Sediment Delivery, IAHS Publ. 159. Proceedings of a conference held at Albuquerque, August 1986. IAHS Press, Wallingford, pp 41–55
Phillips JM, Russell MA, Walling DE (2000) Time-integrated sampling of fluvial suspended sediment: a simple methodology for small catchments. Hydrol Process 14:2589–2602
Porto P, Walling DE (2012) Validating the use of Cs-137 and Pb-210(ex) measurements to estimate rates of soil loss from cultivated land in southern Italy. J Environ Radioact 106:47–57
Renard KG, Foster GA, Weesies DK, McCool DK, Yoder DC (1997) Predicting soil erosion by water: a guide to conservation planning with the Revised Universal Soil Loss Equation. Agriculture Handbook 703. United States Department of Agriculture, Washington, DC
Rustomji P, Caitcheon G, Hairsine P (2008) Combining a spatial model with geochemical tracers and river station data to construct a catchment sediment budget. Water Resour Res 44:W01422
Silburn DM, Carroll C, Ciesiolka CAA, deVoil RC, Burger P (2011) Hillslope runoff and erosion on duplex soils in grazing lands in semi-arid central Queensland. I. Influences of cover, slope, and soil. Soil Res 49:105–117
Small IF, Rowan JS, Franks SW (2002) Quantitative sediment fingerprinting using a Bayesian uncertainty estimation framework. In: Dyer FJ, Thoms MC, Olley JM (eds) Structure, function and management implications of fluvial sedimentary systems. IAHS Publ, vol 276. IAHS Press, Wallingford, pp 443–450
Smith HG, Blake WH (2014) Sediment fingerprinting in agricultural catchments: a critical re-examination of source discrimination and data corrections. Geomorphology 204:177–191
Smith HG, Blake WH, Taylor A (2014) Modelling particle residence times in agricultural river basins using a sediment budget model and fallout radionuclide tracers. Earth Surf Process Landf 39:1944–1959
State of Queensland (Department of Science ITaI) (2014) Land use mapping - Queensland current dataset. http://www.qld.gov.au/environment/land/vegetation/mapping/qlump/. Accessed July 2014
Thorburn PJ, Wilkinson SN, Silburn DM (2013) Water quality in agricultural lands draining to the Great Barrier Reef: causes, management and priorities. Agric Ecosyst Environ 180:4–20
Trimble SW, Mendel AC (1995) The cow as a geomorphic agent—a critical review. Geomorphology 13:233–253
Wallbrink PJ (2004) Quantifying the erosion processes and land-uses which dominate fine sediment supply to Moreton Bay, Southeast Queensland, Australia. J Environ Radioact 76:67–80
Wallbrink PJ, Murray AS (1993) Use of fallout radionuclides as indicators of erosion processes. Hydrol Process 7:297–304
Wallbrink PJ, Murray AS, Olley JM, Olive LJ (1998) Determining the sources and transit times of suspended sediment in the Murrumbidgee River, New South Wales, Australia, using fallout 137Cs and 210Pb. Water Resour Res 34:879–887
Wallbrink PJ, Murray AS, Olley JM (1999) Relating suspended sediment to its original soil depth using fallout radionuclides. Soil Sci Soc Am J 63:369–378
Wallbrink P, Olley J, Hancock G (2002) Estimating residence times of fine sediment in river channels using fallout 210Pb. In: Dyer FJ, Thoms MC, Olley JM (eds) Structure, Function and Management Implications of Fluvial Sedimentary Systems. IAHS Publ 276, IAHS Press, Wallingford, pp 425–432
Walling DE (2005) Tracing suspended sediment sources in catchments and river systems. Sci Total Environ 344:159–184
Walling DE, Woodward JC (1992) Use of radiometric fingerprints to derive information on suspended sediment sources. In: Bogen J, Walling DE, Day TJ (eds) Erosion and sediment transport monitoring programmes in river basins, IAHS Publ 210. IAHS Press, Wallingford, UK, pp 153–164
Wasson RJ, Caitcheon G, Murray AS, McCulloch M, Quade J (2002) Sourcing sediment using multiple tracers in the catchment of Lake Argyle, Northwestern Australia. Environ Manag 29:634–646
Wasson RJ, Furlonger L, Parry D, Pietsch T, Valentine E, Williams D (2010) Sediment sources and channel dynamics, Daly River, Northern Australia. Geomorphology 114:161–174
Wilkinson SN, Wallbrink PJ, Hancock GJ, Blake WH, Shakesby RA, Doerr SH (2009) Fallout radionuclide tracers identify a switch in sediment sources and transport-limited sediment yield following wildfire in a eucalypt forest. Geomorphology 110:140–151
Wilkinson SN, Hancock GJ, Bartley B, Hawdon AA, Keen RJ (2013) Using sediment tracing to assess processes and spatial patterns of erosion in grazed rangelands, Burdekin River basin, Australia. Agric Ecosyst Environ 180:90–102
Wilkinson SN, Dougall C, Kinsey-Henderson AE, Searle R, Ellis R, Bartley B (2014) Development of a time-stepping sediment budget model for assessing land use impacts in large river basins. Sci Total Environ 468–469:1210–1224
Zaimes GN, Schultz RC, Isenhart TM (2008) Streambank soil and phosphorus losses under different riparian land-uses in Iowa. J Am Water Resour Assoc 44:935–947
Acknowledgments
This research was funded by the Queensland Government, the Commonwealth Scientific and Industrial Research Organisation (CSIRO) and the Australian Rivers Institute at Griffith University (ARI). We acknowledge Dr. Jacky Croke (ARI) and Rebecca Bartley (CSIRO) for helpful discussions during project design; Lauren O’Brien, Fred Oudyn and Ashneel Sharma (Queensland Government), Arman Haddadchi and Tanya Ellison (ARI) for assistance with field sampling; Allan Jeffery, Kate Dolan, Ashneel Sharma and Karen Carlile (Queensland Government) for sample preparation; and Rob De Hayr (Queensland Government) for guidance and assistance with laboratory analyses.
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Wilkinson, S.N., Olley, J.M., Furuichi, T. et al. Sediment source tracing with stratified sampling and weightings based on spatial gradients in soil erosion. J Soils Sediments 15, 2038–2051 (2015). https://doi.org/10.1007/s11368-015-1134-2
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DOI: https://doi.org/10.1007/s11368-015-1134-2