Issue 4, 2005

Stratospheric temperature monitoring using a vibrational Raman lidar

Part 1: aerosols and ozone interferences

Abstract

Lidar measurements of temperature for the upper troposphere and lower stratosphere are commonly derived by the Raman technique. Lidar signals derived from vibrational Raman processes have been subjected to numerous simulation tests to examine their sensitivity to the presence of aerosols and ozone in the atmosphere. The influence of aerosols characteristics (wavelength dependence of aerosol extinction and particle phase function) and of ozone concentration on Raman temperature profiles is estimated. Simulations indicate large temperature deviations for post-volcanic conditions. For a Raman backscatter at 607 nm, bias is below 1 K for a total optical depth less than 9 × 10−3 in the case of a stratospheric contamination and less than 6 × 10−3 for a tropospheric contamination. The effect of aerosols depends on phase function and a few parameters such as altitude, optical depth and the shape of the high-altitude cloud. The wavelength dependence of aerosol extinction has some influence only for severe post-volcanic conditions (Scattering Ratio, SR >2). For a Raman backscatter at 387 nm, bias is larger and can be significant even in background aerosol conditions. Changes in the ozone density profile lead to significant Raman temperature deviations only for some specific conditions. Results suggest that both aerosol and ozone corrections are necessary to obtain an accuracy better than the 1 K requested for most atmospheric applications.

Graphical abstract: Stratospheric temperature monitoring using a vibrational Raman lidar Part 1: aerosols and ozone interferences

Article information

Article type
Paper
Submitted
01 Oct 2004
Accepted
04 Feb 2005
First published
23 Feb 2005

J. Environ. Monit., 2005,7, 357-364

Stratospheric temperature monitoring using a vibrational Raman lidar

D. Faduilhe, P. Keckhut, H. Bencherif, L. Robert and S. Baldy, J. Environ. Monit., 2005, 7, 357 DOI: 10.1039/B415299A

To request permission to reproduce material from this article, please go to the Copyright Clearance Center request page.

If you are an author contributing to an RSC publication, you do not need to request permission provided correct acknowledgement is given.

If you are the author of this article, you do not need to request permission to reproduce figures and diagrams provided correct acknowledgement is given. If you want to reproduce the whole article in a third-party publication (excluding your thesis/dissertation for which permission is not required) please go to the Copyright Clearance Center request page.

Read more about how to correctly acknowledge RSC content.

Spotlight

Advertisements