Beschreibung: An advanced multiwavelength polarization Raman lidar was operated aboard the icebreaker Polarstern during the MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition to continuously monitor aerosol and cloud layers in the central Arctic up to 30 km height. The expedition lasted from September 2019 to October 2020 and measurements were mostly taken between 85 and 88.5∘ N. The lidar was integrated into a complex remote-sensing infrastructure aboard the Polarstern. In this article, novel lidar techniques, innovative concepts to study aerosol–cloud interaction in the Arctic, and unique MOSAiC findings will be presented. The highlight of the lidar measurements was the detection of a 10 km deep wildfire smoke layer over the North Pole region between 7–8 km and 17–18 km height with an aerosol optical thickness (AOT) at 532 nm of around 0.1 (in October–November 2019) and 0.05 from December to March. The dual-wavelength Raman lidar technique allowed us to unambiguously identify smoke as the dominating aerosol type in the aerosol layer in the upper troposphere and lower stratosphere (UTLS). An additional contribution to the 532 nm AOT by volcanic sulfate aerosol (Raikoke eruption) was estimated to always be lower than 15 %. The optical and microphysical properties of the UTLS smoke layer are presented in an accompanying paper (Ohneiser et al., 2021). This smoke event offered the unique opportunity to study the influence of organic aerosol particles (serving as ice-nucleating particles, INPs) on cirrus formation in the upper troposphere. An example of a closure study is presented to explain our concept of investigating aerosol–cloud interaction in this field. The smoke particles were obviously able to control the evolution of the cirrus system and caused low ice crystal number concentration. After the discussion of two typical Arctic haze events, we present a case study of the evolution of a long-lasting mixed-phase cloud layer embedded in Arctic haze in the free troposphere. The recently introduced dual-field-of-view polarization lidar technique was applied, for the first time, to mixed-phase cloud observations in order to determine the microphysical properties of the water droplets. The mixed-phase cloud closure experiment (based on combined lidar and radar observations) indicated that the observed aerosol levels controlled the number concentrations of nucleated droplets and ice crystals.

Beschreibung: During the 1-year MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition, the German icebreaker Polarstern drifted through Arctic Ocean ice from October 2019 to May 2020, mainly at latitudes between 85 and 88.5∘ N. A multiwavelength polarization Raman lidar was operated on board the research vessel and continuously monitored aerosol and cloud layers up to a height of 30 km. During our mission, we expected to observe a thin residual volcanic aerosol layer in the stratosphere, originating from the Raikoke volcanic eruption in June 2019, with an aerosol optical thickness (AOT) of 0.005–0.01 at 500 nm over the North Pole area during the winter season. However, the highlight of our measurements was the detection of a persistent, 10 km deep aerosol layer in the upper troposphere and lower stratosphere (UTLS), from about 7–8 to 17–18 km height, with clear and unambiguous wildfire smoke signatures up to 12 km and an order of magnitude higher AOT of around 0.1 in the autumn of 2019. Case studies are presented to explain the specific optical fingerprints of aged wildfire smoke in detail. The pronounced aerosol layer was present throughout the winter half-year until the strong polar vortex began to collapse in late April 2020. We hypothesize that the detected smoke originated from extraordinarily intense and long-lasting wildfires in central and eastern Siberia in July and August 2019 and may have reached the tropopause layer by the self-lifting process. In this article, we summarize the main findings of our 7-month smoke observations and characterize the aerosol in terms of geometrical, optical, and microphysical properties. The UTLS AOT at 532 nm ranged from 0.05–0.12 in October–November 2019 and 0.03–0.06 during the main winter season. The Raikoke aerosol fraction was estimated to always be lower than 15 %. We assume that the volcanic aerosol was above the smoke layer (above 13 km height). As an unambiguous sign of the dominance of smoke in the main aerosol layer from 7–13 km height, the particle extinction-to-backscatter ratio (lidar ratio) at 355 nm was found to be much lower than at 532 nm, with mean values of 55 and 85 sr, respectively. The 355–532 nm Ångström exponent of around 0.65 also clearly indicated the presence of smoke aerosol. For the first time, we show a distinct view of the aerosol layering features in the High Arctic from the surface up to 30 km height during the winter half-year. Finally, we provide a vertically resolved view on the late winter and early spring conditions regarding ozone depletion, smoke occurrence, and polar stratospheric cloud formation. The latter will largely stimulate research on a potential impact of the unexpected stratospheric aerosol perturbation on the record-breaking ozone depletion in the Arctic in spring 2020.