Electronic Resource
College Park, Md.
:
American Institute of Physics (AIP)
The Journal of Chemical Physics
112 (2000), S. 6733-6738
ISSN:
1089-7690
Source:
AIP Digital Archive
Topics:
Physics
,
Chemistry and Pharmacology
Notes:
We present an integral-equation solution of the structure of systems built through the sequential quenching of particles. The theory is based on the Replica Ornstein–Zernike equations that describe the structure of equilibrium fluids within random porous matrices. The quenched particles are treated as a polydisperse system, each of them labeled by the total density at the time of its arrival. The diagrammatic expansions of the correlation functions lead to the development of the liquid-theory closures appropriate for the present case. Numerical solutions for the deposition of hard disks show excellent agreement with simulation. We also discuss a binary-mixture treatment, which is shown to provide a very good approximation to the polydisperse approach. © 2000 American Institute of Physics.
Type of Medium:
Electronic Resource
URL:
http://dx.doi.org/10.1063/1.481240
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