Description: Feedbacks play a fundamental role in determining the magnitude of the response of the climate system to external forcing, such as from anthropogenic emissions. The latest generation of Earth system models includes aerosol and chemistry components that interact with each other and with the biosphere. These interactions introduce a complex web of feedbacks that is important to understand and quantify. This paper addresses multiple pathways for aerosol and chemical feedbacks in Earth system models. These focus on changes in natural emissions (dust, sea salt, dimethyl sulfide, biogenic volatile organic compounds (BVOCs) and lightning) and changes in reaction rates for methane and ozone chemistry. The feedback terms are then given by the sensitivity of a pathway to climate change multiplied by the radiative effect of the change. We find that the overall climate feedback through chemistry and aerosols is negative in the sixth Coupled Model Intercomparison Project (CMIP6) Earth system models due to increased negative forcing from aerosols in a climate with warmer surface temperatures following a quadrupling of CO2 concentrations. This is principally due to increased emissions of sea salt and BVOCs which are sensitive to climate change and cause strong negative radiative forcings. Increased chemical loss of ozone and methane also contributes to a negative feedback. However, overall methane lifetime is expected to increase in a warmer climate due to increased BVOCs. Increased emissions of methane from wetlands would also offset some of the negative feedbacks. The CMIP6 experimental design did not allow the methane lifetime or methane emission changes to affect climate, so we found a robust negative contribution from interactive aerosols and chemistry to climate sensitivity in CMIP6 Earth system models.

Description: Many nations responded to the corona virus disease-2019 (COVID-19) pandemic by restricting travel and other activities during 2020, resulting in temporarily reduced emissions of CO2, other greenhouse gases and ozone and aerosol precursors. We present the initial results from a coordinated Intercomparison, CovidMIP, of Earth system model simulations which assess the impact on climate of these emissions reductions. 12 models performed multiple initial-condition ensembles to produce over 300 simulations spanning both initial condition and model structural uncertainty. We find model consensus on reduced aerosol amounts (particularly over southern and eastern Asia) and associated increases in surface shortwave radiation levels. However, any impact on near-surface temperature or rainfall during 2020–2024 is extremely small and is not detectable in this initial analysis. Regional analyses on a finer scale, and closer attention to extremes (especially linked to changes in atmospheric composition and air quality) are required to test the impact of COVID-19-related emission reductions on near-term climate. Key Points: - Lockdown restrictions during COVID-19 have reduced emissions of aerosols and greenhouse gases - 12 CMIP6 Earth system models have performed coordinated experiments to assess the impact of this on climate - Aerosol amounts are reduced over southern and eastern Asia but there is no detectable change in annually averaged temperature or precipitation

Description: Lockdowns to avoid the spread of COVID-19 have created an unprecedented reduction in human emissions. While the country-level scale of emissions changes can be estimated in near real time, the more detailed, gridded emissions estimates that are required to run general circulation models (GCMs) of the climate will take longer to collect. In this paper we use recorded and projected country-and-sector activity levels to modify gridded predictions from the MESSAGE-GLOBIOM SSP2-4.5 scenario. We provide updated projections for concentrations of greenhouse gases, emissions fields for aerosols, and precursors and the ozone and optical properties that result from this. The code base to perform similar modifications to other scenarios is also provided. We outline the means by which these results may be used in a model intercomparison project (CovidMIP) to investigate the impact of national lockdown measures on climate, including regional temperature, precipitation, and circulation changes. This includes three strands: an assessment of short-term effects (5-year period) and of longer-term effects (30 years) and an investigation into the separate effects of changes in emissions of greenhouse gases and aerosols. This last strand supports the possible attribution of observed changes in the climate system; hence these simulations will also form part of the Detection and Attribution Model Intercomparison Project (DAMIP).

Description: A key driving factor behind rapid Arctic climate change is black carbon, the atmospheric aerosol that most efficiently absorbs sunlight. Our knowledge about black carbon in the Arctic is scarce, mainly limited to long-term measurements of a few ground stations and snap-shots by aircraft observations. Here, we combine observations from aircraft campaigns performed over nine years, and present vertically resolved average black carbon properties. A factor of four higher black carbon mass concentration (21.6 ng m−3 average, 14.3 ng m−3 median) was found in spring, compared to summer (4.7 ng m−3 average, 3.9 ng m−3 median). In spring, much higher inter-annual and geographic variability prevailed compared to the stable situation in summer. The shape of the black carbon size distributions remained constant between seasons with an average mass mean diameter of 202 nm in spring and 210 nm in summer. Comparison between observations and concentrations simulated by a global model shows notable discrepancies, highlighting the need for further model developments and intensified measurements.