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  • 1
    Online Resource
    Online Resource
    Copernicus GmbH ; 2022
    In:  The Cryosphere Vol. 16, No. 6 ( 2022-06-07), p. 2127-2145
    In: The Cryosphere, Copernicus GmbH, Vol. 16, No. 6 ( 2022-06-07), p. 2127-2145
    Abstract: Abstract. In recent years, airborne microplastics have been identified in a range of remote environments. However, data throughout the Southern Hemisphere, in particular Antarctica, are largely absent to date. We collected snow samples from 19 sites across the Ross Island region of Antarctica. Suspected microplastic particles were isolated and their composition confirmed using micro-Fourier transform infrared spectroscopy (µFTIR). We identified microplastics in all Antarctic snow samples at an average concentration of 29 particles L−1, with fibres the most common morphotype and polyethylene terephthalate (PET) the most common polymer. To investigate sources, backward air mass trajectories were run from the time of sampling. These indicate potential long-range transportation of up to 6000 km, assuming a residence time of 6.5 d. Local sources were also identified as potential inputs into the environment as the polymers identified were consistent with those used in clothing and equipment from nearby research stations. This study adds to the growing body of literature regarding microplastics as a ubiquitous airborne pollutant and establishes their presence in Antarctica.
    Type of Medium: Online Resource
    ISSN: 1994-0424
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2022
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  • 2
    In: Earth System Science Data, Copernicus GmbH, Vol. 13, No. 7 ( 2021-07-02), p. 3115-3153
    Abstract: Abstract. Due to its remote location and extreme weather conditions, atmospheric in situ measurements are rare in the Southern Ocean. As a result, aerosol–cloud interactions in this region are poorly understood and remain a major source of uncertainty in climate models. This, in turn, contributes substantially to persistent biases in climate model simulations such as the well-known positive shortwave radiation bias at the surface, as well as biases in numerical weather prediction models and reanalyses. It has been shown in previous studies that in situ and ground-based remote sensing measurements across the Southern Ocean are critical for complementing satellite data sets due to the importance of boundary layer and low-level cloud processes. These processes are poorly sampled by satellite-based measurements and are often obscured by multiple overlying cloud layers. Satellite measurements also do not constrain the aerosol–cloud processes very well with imprecise estimation of cloud condensation nuclei. In this work, we present a comprehensive set of ship-based aerosol and meteorological observations collected on the 6-week Southern Ocean Ross Sea Marine Ecosystem and Environment voyage (TAN1802) voyage of RV Tangaroa across the Southern Ocean, from Wellington, New Zealand, to the Ross Sea, Antarctica. The voyage was carried out from 8 February to 21 March 2018. Many distinct, but contemporaneous, data sets were collected throughout the voyage. The compiled data sets include measurements from a range of instruments, such as (i) meteorological conditions at the sea surface and profile measurements; (ii) the size and concentration of particles; (iii) trace gases dissolved in the ocean surface such as dimethyl sulfide and carbonyl sulfide; (iv) and remotely sensed observations of low clouds. Here, we describe the voyage, the instruments, and data processing, and provide a brief overview of some of the data products available. We encourage the scientific community to use these measurements for further analysis and model evaluation studies, in particular, for studies of Southern Ocean clouds, aerosol, and their interaction. The data sets presented in this study are publicly available at https://doi.org/10.5281/zenodo.4060237 (Kremser et al., 2020).
    Type of Medium: Online Resource
    ISSN: 1866-3516
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2475469-9
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  • 3
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 23, No. 24 ( 2023-12-14), p. 15181-15196
    Abstract: Abstract. The biogeochemical formation of dimethyl sulfide (DMS) from the Southern Ocean is complex, dynamic, and driven by physical, chemical, and biological processes. Such processes, produced by marine biogenic activity, are the dominant source of sulfate aerosol over the Southern Ocean. Using an atmosphere-only configuration of the United Kingdom Earth System Model (UKESM1-AMIP), we performed eight 10-year simulations for the recent past (2009–2018) during austral summer. We tested the sensitivity of atmospheric DMS to four oceanic DMS datasets and three DMS transfer velocity parameterizations. One oceanic DMS dataset was developed here from satellite chlorophyll a. We find that the choice of oceanic DMS dataset has a larger influence on atmospheric DMS than the choice of DMS transfer velocity. Simulations with linear transfer velocity parameterizations show a more accurate representation of atmospheric DMS concentration than those using quadratic relationships. This work highlights that the oceanic DMS and DMS transfer velocity parameterizations currently used in climate models are poorly constrained for the Southern Ocean region. Simulations using oceanic DMS derived from satellite chlorophyll a data, and when combined with a recently developed linear transfer velocity parameterization for DMS, show better spatial variability than the UKESM1 configuration. We also demonstrate that capturing large-scale spatial variability can be more important than large-scale interannual variability. We recommend that models use a DMS transfer velocity parameterization that was developed specifically for DMS and improvements to oceanic DMS spatial variability. Such improvements may provide a more accurate process-based representation of oceanic and atmospheric DMS, and therefore sulfate aerosol, in the Southern Ocean region.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2023
    detail.hit.zdb_id: 2069847-1
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  • 4
    Online Resource
    Online Resource
    American Geophysical Union (AGU) ; 2019
    In:  Geophysical Research Letters Vol. 46, No. 6 ( 2019-03-28), p. 3446-3453
    In: Geophysical Research Letters, American Geophysical Union (AGU), Vol. 46, No. 6 ( 2019-03-28), p. 3446-3453
    Abstract: A novel method for climate model evaluation is used to identify both mean errors and potential compensating errors As an example, we apply this methodology to investigate the quality of different cloud parameterizations over the Southern Ocean Changes to the cloud phase parameterizations can reduce shortwave radiative bias regionally, but large compensating errors remain
    Type of Medium: Online Resource
    ISSN: 0094-8276 , 1944-8007
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2019
    detail.hit.zdb_id: 2021599-X
    detail.hit.zdb_id: 7403-2
    SSG: 16,13
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  • 5
    Online Resource
    Online Resource
    Springer Science and Business Media LLC ; 2023
    In:  Nature Geoscience Vol. 16, No. 5 ( 2023-05), p. 410-415
    In: Nature Geoscience, Springer Science and Business Media LLC, Vol. 16, No. 5 ( 2023-05), p. 410-415
    Abstract: Understanding precipitation is essential for quantifying weather and climate-related risks. Changes in precipitation climatology are typically based on independent analysis of precipitation frequency and intensity. Here we show that where it rains more often, it also rains harder. When grouping global precipitation reanalysis data and observations from the past 40 years into regions of similar wet-day frequency, regardless of geographical separation, there is a strong correlation with wet-day intensity distributions. These wet-day-frequency regions are also more physically coherent than regions based on geographical location. We find the coherent relationship between wet-day frequency and intensity distributions is partially explained by wet-day-frequency regions having similar vertical velocity and convective available potential energy distributions, once polar regions are excluded. These represent dynamic and thermodynamic processes that indicate how conducive wet-day-frequency regions are to large-scale and convective precipitation. This suggests that the main drivers of precipitation are universal. We also show that extreme-precipitation metrics are dependent on wet-day frequency within our framework. Our results imply that wet-day frequency could be used to derive estimates of extreme-precipitation climate indices and corresponding uncertainties, these uncertainties being related to local processes.
    Type of Medium: Online Resource
    ISSN: 1752-0894 , 1752-0908
    Language: English
    Publisher: Springer Science and Business Media LLC
    Publication Date: 2023
    detail.hit.zdb_id: 2396648-8
    detail.hit.zdb_id: 2405323-5
    SSG: 16,13
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  • 6
    Online Resource
    Online Resource
    American Geophysical Union (AGU) ; 2016
    In:  Journal of Geophysical Research: Atmospheres Vol. 121, No. 21 ( 2016-11-16)
    In: Journal of Geophysical Research: Atmospheres, American Geophysical Union (AGU), Vol. 121, No. 21 ( 2016-11-16)
    Abstract: SOM analysis of ISCCP data produces a subset of the regimes derived in previous studies using k ‐means clustering with finer detail in areas ISCCP flux data and ERA‐Interim vertical velocity and lower tropospheric stability demonstrate that the clusters are physically meaningful The objective organization of the SOM allows a quantitative analysis of cloud regimes daily transition frequency and persistence
    Type of Medium: Online Resource
    ISSN: 2169-897X , 2169-8996
    URL: Issue
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2016
    detail.hit.zdb_id: 710256-2
    detail.hit.zdb_id: 2016800-7
    detail.hit.zdb_id: 2969341-X
    SSG: 16,13
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  • 7
    Online Resource
    Online Resource
    American Geophysical Union (AGU) ; 2018
    In:  Journal of Geophysical Research: Atmospheres Vol. 123, No. 8 ( 2018-04-27), p. 4259-4272
    In: Journal of Geophysical Research: Atmospheres, American Geophysical Union (AGU), Vol. 123, No. 8 ( 2018-04-27), p. 4259-4272
    Abstract: Clusters are generated by applying a self‐organizing map to MODIS joint histograms of cloud Radiative differences between the model and observations are attributed to specific clusters Regional cloud radiative effect errors are obscured by compensating errors between clusters
    Type of Medium: Online Resource
    ISSN: 2169-897X , 2169-8996
    URL: Issue
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2018
    detail.hit.zdb_id: 710256-2
    detail.hit.zdb_id: 2016800-7
    detail.hit.zdb_id: 2969341-X
    SSG: 16,13
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  • 8
    Online Resource
    Online Resource
    American Geophysical Union (AGU) ; 2021
    In:  Journal of Geophysical Research: Atmospheres Vol. 126, No. 6 ( 2021-03-27)
    In: Journal of Geophysical Research: Atmospheres, American Geophysical Union (AGU), Vol. 126, No. 6 ( 2021-03-27)
    Abstract: 2BCL5 and DARDAR cloud occurrences show large differences at low‐levels globally, with the largest disparities at high southern latitudes Comparison with Antarctic ground observations tentatively suggests that this difference is likely due to false detections in DARDAR Some 2BCL5 and DARDAR cloud phase estimates do not adhere to physical constraints set by temperature from ECMWF‐AUX or local radiosondes
    Type of Medium: Online Resource
    ISSN: 2169-897X , 2169-8996
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2021
    detail.hit.zdb_id: 710256-2
    detail.hit.zdb_id: 2016800-7
    detail.hit.zdb_id: 2969341-X
    SSG: 16,13
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  • 9
    Online Resource
    Online Resource
    American Geophysical Union (AGU) ; 2023
    In:  Geophysical Research Letters Vol. 50, No. 17 ( 2023-09-16)
    In: Geophysical Research Letters, American Geophysical Union (AGU), Vol. 50, No. 17 ( 2023-09-16)
    Abstract: We detail a new methodology to assess precipitation extremes within cyclone composites using a spatially dependent precipitation threshold Extreme precipitation occurs preferentially and makes up a larger fraction of total accumulation before cyclones reach peak intensity Extreme precipitation is more constrained around the cyclone center and weakens more rapidly over time compared to moderate precipitation
    Type of Medium: Online Resource
    ISSN: 0094-8276 , 1944-8007
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2023
    detail.hit.zdb_id: 2021599-X
    detail.hit.zdb_id: 7403-2
    SSG: 16,13
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  • 10
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 19, No. 24 ( 2019-12-17), p. 15447-15466
    Abstract: Abstract. With low concentrations of tropospheric aerosol, the Southern Ocean offers a “natural laboratory” for studies of aerosol–cloud interactions. Aerosols over the Southern Ocean are produced from biogenic activity in the ocean, which generates sulfate aerosol via dimethylsulfide (DMS) oxidation, and from strong winds and waves that lead to bubble bursting and sea spray emission. Here, we evaluate the representation of Southern Ocean aerosols in the Hadley Centre Global Environmental Model version 3, Global Atmosphere 7.1 (HadGEM3-GA7.1) chemistry–climate model. Compared with aerosol optical depth (AOD) observations from two satellite instruments (the Moderate Resolution Imaging Spectroradiometer, MODIS-Aqua c6.1, and the Multi-angle Imaging Spectroradiometer, MISR), the model simulates too-high AOD during winter and too-low AOD during summer. By switching off DMS emission in the model, we show that sea spray aerosol is the dominant contributor to AOD during winter. In turn, the simulated sea spray aerosol flux depends on near-surface wind speed. By examining MODIS AOD as a function of wind speed from the ERA-Interim reanalysis and comparing it with the model, we show that the sea spray aerosol source function in HadGEM3-GA7.1 overestimates the wind speed dependency. We test a recently developed sea spray aerosol source function derived from measurements made on a Southern Ocean research voyage in 2018. In this source function, the wind speed dependency of the sea spray aerosol flux is less than in the formulation currently implemented in HadGEM3-GA7.1. The new source function leads to good agreement between simulated and observed wintertime AODs over the Southern Ocean; however, it reveals partially compensating errors in DMS-derived AOD. While previous work has tested assumptions regarding the seawater climatology or sea–air flux of DMS, we test the sensitivity of simulated AOD, cloud condensation nuclei and cloud droplet number concentration to three atmospheric sulfate chemistry schemes. The first scheme adds DMS oxidation by halogens and the other two test a recently developed sulfate chemistry scheme for the marine troposphere; one tests gas-phase chemistry only, while the second adds extra aqueous-phase sulfate reactions. We show how simulated sulfur dioxide and sulfuric acid profiles over the Southern Ocean change as a result and how the number concentration and particle size of the soluble Aitken, accumulation and coarse aerosol modes are affected. The new DMS chemistry scheme leads to a 20 % increase in the number concentration of cloud condensation nuclei and cloud droplets, which improves agreement with observations. Our results highlight the importance of atmospheric chemistry for simulating aerosols and clouds accurately over the Southern Ocean.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2019
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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