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  • 1
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 22, No. 15 ( 2022-08-10), p. 10221-10245
    Abstract: Abstract. Aerosol-aware microphysics parameterisation schemes are increasingly being introduced into numerical weather prediction models, allowing for regional and case-specific parameterisation of cloud condensation nuclei (CCN) and cloud droplet interactions. In this paper, the Thompson aerosol-aware microphysics scheme, within the Weather Research and Forecasting (WRF) model, is used for two fog cases during September 2017 over Namibia. Measurements of CCN and fog microphysics were undertaken during the AErosols, RadiatiOn and CLOuds in southern Africa (AEROCLO-sA) field campaign at Henties Bay on the coast of Namibia during September 2017. A key concept of the microphysics scheme is the conversion of water-friendly aerosols to cloud droplets (hereafter referred to as CCN activation), which could be estimated from the observations. A fog monitor 100 (FM-100) provided cloud droplet size distribution, number concentration (Nt), liquid water content (LWC), and mean volumetric diameter (MVD). These measurements are used to evaluate and parameterise WRF model simulations of Nt, LWC, and MVD. A sensitivity analysis was conducted through variations to the initial CCN concentration, CCN radius, and the minimum updraft speed, which are important factors that influence droplet activation in the microphysics scheme of the model. The first model scenario made use of the default settings with a constant initial CCN number concentration of 300 cm−3 and underestimated the cloud droplet number concentration, while the LWC was in good agreement with the observations. This resulted in droplet size being larger than the observations. Another scenario used modelled data as CCN initial conditions, which were an order of magnitude higher than other scenarios. However, these provided the most realistic values of Nt, LWC, MVD, and droplet size distribution. From this, it was concluded that CCN activation of around 10 % in the simulations is too low, while the observed appears to be higher reaching between 20 % and 80 %, with a mean (median) of 0.55 (0.56) during fog events. To achieve this level of activation in the model, the minimum updraft speed for CCN activation was increased from 0.01 to 0.1 m s−1. This scenario provided Nt, LWC, MVD, and droplet size distribution in the range of the observations, with the added benefit of a realistic initial CCN concentration. These results demonstrate the benefits of a dynamic aerosol-aware scheme when parameterised with observations.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2022
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 2
    Online Resource
    Online Resource
    Springer Science and Business Media LLC ; 2022
    In:  Air Quality, Atmosphere & Health Vol. 15, No. 12 ( 2022-12), p. 2157-2169
    In: Air Quality, Atmosphere & Health, Springer Science and Business Media LLC, Vol. 15, No. 12 ( 2022-12), p. 2157-2169
    Type of Medium: Online Resource
    ISSN: 1873-9318 , 1873-9326
    Language: English
    Publisher: Springer Science and Business Media LLC
    Publication Date: 2022
    detail.hit.zdb_id: 2424084-9
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  • 3
    In: Bulletin of the American Meteorological Society, American Meteorological Society, Vol. 100, No. 7 ( 2019-07), p. 1277-1298
    Abstract: The Aerosol, Radiation and Clouds in southern Africa (AEROCLO-sA) project investigates the role of aerosols on the regional climate of southern Africa. This is a unique environment where natural and anthropogenic aerosols and a semipermanent and widespread stratocumulus (Sc) cloud deck are found. The project aims to understand the dynamical, chemical, and radiative processes involved in aerosol–cloud–radiation interactions over land and ocean and under various meteorological conditions. The AEROCLO-sA field campaign was conducted in August and September of 2017 over Namibia. An aircraft equipped with active and passive remote sensors and aerosol in situ probes performed a total of 30 research flight hours. In parallel, a ground-based mobile station with state-of-the-art in situ aerosol probes and remote sensing instrumentation was implemented over coastal Namibia, and complemented by ground-based and balloonborne observations of the dynamical, thermodynamical, and physical properties of the lower troposphere. The focus laid on mineral dust emitted from salty pans and ephemeral riverbeds in northern Namibia, the advection of biomass-burning aerosol plumes from Angola subsequently transported over the Atlantic Ocean, and aerosols in the marine boundary layer at the ocean–atmosphere interface. This article presents an overview of the AEROCLO-sA field campaign with results from the airborne and surface measurements. These observations provide new knowledge of the interactions of aerosols and radiation in cloudy and clear skies in connection with the atmospheric dynamics over southern Africa. They will foster new advanced climate simulations and enhance the capability of spaceborne sensors, ultimately allowing a better prediction of future climate and weather in southern Africa.
    Type of Medium: Online Resource
    ISSN: 0003-0007 , 1520-0477
    Language: Unknown
    Publisher: American Meteorological Society
    Publication Date: 2019
    detail.hit.zdb_id: 2029396-3
    detail.hit.zdb_id: 419957-1
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  • 4
    Online Resource
    Online Resource
    Copernicus GmbH ; 2022
    In:  Atmospheric Chemistry and Physics Vol. 22, No. 8 ( 2022-05-02), p. 5701-5724
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 22, No. 8 ( 2022-05-02), p. 5701-5724
    Abstract: Abstract. The formation of a river of smoke crossing southern Africa was investigated during the Aerosols, Radiation and Clouds in southern Africa (AEROCLO-sA) campaign in September 2017. A complementary set of global and mesoscale numerical simulations as well as ground-based, airborne and space-borne observations of the dynamics, thermodynamics and composition of the atmosphere are used to characterize the river of smoke in terms of timing and vertical extent of the biomass burning aerosol (BBA) layer. The study area was under the synoptic influence of a coastal low rooted in a tropical easterly wave and a high-pressure system over the continent and westerly waves at mid latitudes, one of which had an embedded cut-off low (CoL). The coastal low interacted with the second of two approaching westerly waves and ultimately formed a mid-level tropical temperate trough (TTT). The TTT created the fast-moving air mass transported to the southwestern Indian Ocean as a river of smoke. The CoL, which developed and intensified in the upper levels associated with the first (easternmost) westerly wave, remained stationary above northern Namibia prior to the formation of the TTT and was responsible for the thickening of the BBA layer. This shows that the evolution of the river of smoke is very much tied to the evolution of the TTT, while its vertical extent is related to the presence of the CoL. The mechanisms by which the CoL, observed over Namibia in the entrance region of the river of smoke, influences the vertical structure of the BBA layer is mainly associated with the ascending motion above the BBA layer. In the presence of the CoL, the top of the BBA layer over northern Namibia reaches altitudes above 8 km. This is much higher than the average height of the top of the BBA layer over the regions where the smoke comes from (Angola, Zambia, Zimbabwe, Mozambique), which is 5 to 6 km. The results suggest that the interaction between the TTTs and the CoLs which form during the winter may have a role in promoting the transport of BBA from fire-prone regions in the tropical band to the temperate mid latitudes and the southwestern Indian Ocean.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2022
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 5
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 18, No. 23 ( 2018-11-30), p. 17003-17016
    Abstract: Abstract. Continuous measurements between July 2012 and December 2015 at the Henties Bay Aerosol Observatory (HBAO; 22∘ S, 14∘05′ E), Namibia, show that, during the austral wintertime, transport of light-absorbing black carbon aerosols occurs at low level into the marine boundary layer. The average of daily concentrations of equivalent black carbon (eBC) over the whole sampling period is 53 (±55) ng m−3. Peak values above 200 ng m−3 and up to 800 ng m−3 occur seasonally from May to August, ahead of the dry season peak of biomass burning in southern Africa (August to October). Analysis of 3-day air mass back-trajectories show that air masses from the South Atlantic Ocean south of Henties Bay are generally cleaner than air having originated over the ocean north of Henties Bay, influenced by the outflow of the major biomass burning plume, and from the continent, where wildfires occur. Additional episodic peak concentrations, even for oceanic transport, indicate that pollution from distant sources in South Africa and maritime traffic along the Atlantic ship tracks could be important. While we expect the direct radiative effect to be negligible, the indirect effect on the microphysical properties of the stratocumulus clouds and the deposition to the ocean could be significant and deserve further investigation, specifically ahead of the dry season.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2018
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 6
    Online Resource
    Online Resource
    MDPI AG ; 2021
    In:  Atmosphere Vol. 12, No. 11 ( 2021-10-26), p. 1405-
    In: Atmosphere, MDPI AG, Vol. 12, No. 11 ( 2021-10-26), p. 1405-
    Abstract: Emissions from residential solid fuel burning in densely populated low-income settlements is a significant source of air pollution over the South African Highveld. The area is densely populated and highly industrialized, resulting in high concentrations of pollutants over the area. Although emissions from industrial sources are much larger, exposure to household emissions poses the most significant risk to human health. Interventions aimed at reducing solid fuel burning in low-income settlements on the Highveld have the potential to reduce exposure, but quantifying their true impact remains a challenge. We aimed to estimate the health and associated economic benefits of the regional implementation of thermal insulation as intervention measure in low-income settlements to predict the potential impact on the regional scale. We used a land use type regression model to estimate pre-intervention PM2.5 concentrations over the Highveld and then used sampled post-intervention air quality data from a pilot offset programme to relate changes in air quality to changes in avoided premature mortalities. We estimate that the large-scale implementation of this intervention could result in 143 avoided premature mortalities with an estimated economic benefit of just under ZAR (2011) 341.6 million, equivalent to USD (2011) 49.4 million.
    Type of Medium: Online Resource
    ISSN: 2073-4433
    Language: English
    Publisher: MDPI AG
    Publication Date: 2021
    detail.hit.zdb_id: 2605928-9
    SSG: 23
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  • 7
    In: Toxics, MDPI AG, Vol. 10, No. 2 ( 2022-02-04), p. 67-
    Abstract: Emissions from residential solid fuels reduce ambient air quality and cause indoor air pollution resulting in adverse human health. The traditional solid fuels used for cooking include coal, straws, dung, and wood, with the latter identified as the prevalent energy source in developing countries. Emissions from such fuel sources appear to be significant hazards and risk factors for asthma and other respiratory diseases. This study aimed at reporting factors influencing the choice of dominant solid fuel for cooking and determine the emission risk from such solid fuel in three villages of Phalaborwa, Limpopo province, South Africa. The study used descriptive analysis to show the relationship between the socio-economic variables and the choice of cooking fuel at the household level. Multiple correspondence analysis (MCA) was used further to detect and represent underlying structures in the choice of dominant fuels. MCA shows the diversity and existing relationship of how variables are related analytically and graphically. Generalised linear logistic weight estimation procedure (WLS) was also used to investigate the factors influencing choice of fuel used and the inherent emission risks. In the three villages, wood was the prevalent cooking fuel with 76.8% of participant households using it during the summer and winter seasons. Variables such as low monthly income, level of education, and system of burning are revealed as strong predictors of wood fuel usage. Moreover, income, water heating energy, types of wood, and number of cooking hours are significant (p ≤ 0.05) in influencing emission from wood fuel in the community. A notable conclusion is that variables such as income, education status and system of burning are determinants of wood fuel usage in the three villages, while income, water heating energy, types of wood and number of hours influence vulnerability to household emission and possible health risks in the use of solid energy sources.
    Type of Medium: Online Resource
    ISSN: 2305-6304
    Language: English
    Publisher: MDPI AG
    Publication Date: 2022
    detail.hit.zdb_id: 2733883-6
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  • 8
    Online Resource
    Online Resource
    Elsevier BV ; 2017
    In:  Journal of Analytical and Applied Pyrolysis Vol. 126 ( 2017-07), p. 158-168
    In: Journal of Analytical and Applied Pyrolysis, Elsevier BV, Vol. 126 ( 2017-07), p. 158-168
    Type of Medium: Online Resource
    ISSN: 0165-2370
    Language: English
    Publisher: Elsevier BV
    Publication Date: 2017
    detail.hit.zdb_id: 1484647-0
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  • 9
    Online Resource
    Online Resource
    Academy of Science of South Africa ; 2020
    In:  South African Journal of Science Vol. 116, No. 3/4 ( 2020-03-26)
    In: South African Journal of Science, Academy of Science of South Africa, Vol. 116, No. 3/4 ( 2020-03-26)
    Abstract: Biomass burning in Africa provides a prolific source of aerosols that are transported from the source region to distant areas, as far away as South America and Australia. Models have long predicted the primary outflow and transport routes. Over time, field studies have validated the basic production and dynamics that underlie these transport patterns. In more recent years, the advancement of spaceborne active remote-sensing techniques has allowed for more detailed verification of the models and, importantly, verification of the vertical distribution of the aerosols in the transport regions, particularly with respect to westerly transport over the Atlantic Ocean. The Cloud-Aerosol Transport System (CATS) lidar on the International Space Station has detection sensitivity that provides observations that support long-held theories of aerosol transport from the African subcontinent over the remote Indian Ocean and as far downstream as Australia. Significance: Biomass burning in Africa can have impacts as far away as Australia. Flow of aerosols from Africa towards Australia has long been postulated by transport models, but has been poorly characterised due to a lack of measurements. The CATS instrument on the International Space Station has detection sensitivity that captures aerosol transport from Africa over the Indian Ocean to Australia. Open data set:  https://cats.gsfc.nasa.gov/
    Type of Medium: Online Resource
    ISSN: 1996-7489
    Language: Unknown
    Publisher: Academy of Science of South Africa
    Publication Date: 2020
    detail.hit.zdb_id: 2067033-3
    detail.hit.zdb_id: 2482725-3
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  • 10
    In: Sustainability, MDPI AG, Vol. 13, No. 19 ( 2021-09-25), p. 10659-
    Abstract: The brick making industry, despite its contribution to environmental pollution, plays a major role in the economic growth of South Africa, with the traditional technology accounting for a significant proportion of the total clay brick production. The aim of this study is to undertake a comprehensive description of the production phases of the traditional brick making sector in Vhembe district and how this contributes to air pollution. The study comprised a series of interviews and questionnaires of key role players from two small villages, Manini and Tshilungoma in the Vhembe district. In-situ observations of the production methods and phases were also undertaken between June and December 2019. The brick making production phases used in Vhembe district are excavation, preparation, moulding, drying and firing. An average estimate of 34,683 bricks is fired monthly per brick kiln in Vhembe district. Emissions from brick making organisations had resulted into several public health and environmental risks. To reduce environmental degradation, the incorporation of industrial and environmental wastes into brick making and the gradual transition to environmentally friendly technology such as Vertical Shaft brick kiln (VSBK) should be embraced. Thus, traditional brick making implemented with appropriate sustainable environmental technology has the potential to improve the socio-economic status of the brick makers.
    Type of Medium: Online Resource
    ISSN: 2071-1050
    Language: English
    Publisher: MDPI AG
    Publication Date: 2021
    detail.hit.zdb_id: 2518383-7
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