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  • 1
    In: Nature, Springer Science and Business Media LLC, Vol. 586, No. 7828 ( 2020-10-08), p. 248-256
    Type of Medium: Online Resource
    ISSN: 0028-0836 , 1476-4687
    RVK:
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    Language: English
    Publisher: Springer Science and Business Media LLC
    Publication Date: 2020
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    detail.hit.zdb_id: 1413423-8
    SSG: 11
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  • 2
    In: Nature Climate Change, Springer Science and Business Media LLC, Vol. 13, No. 6 ( 2023-06), p. 579-587
    Type of Medium: Online Resource
    ISSN: 1758-678X , 1758-6798
    Language: English
    Publisher: Springer Science and Business Media LLC
    Publication Date: 2023
    detail.hit.zdb_id: 2603450-5
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  • 3
    In: Earth System Science Data, Copernicus GmbH, Vol. 12, No. 3 ( 2020-07-15), p. 1561-1623
    Abstract: Abstract. Understanding and quantifying the global methane (CH4) budget is important for assessing realistic pathways to mitigate climate change. Atmospheric emissions and concentrations of CH4 continue to increase, making CH4 the second most important human-influenced greenhouse gas in terms of climate forcing, after carbon dioxide (CO2). The relative importance of CH4 compared to CO2 depends on its shorter atmospheric lifetime, stronger warming potential, and variations in atmospheric growth rate over the past decade, the causes of which are still debated. Two major challenges in reducing uncertainties in the atmospheric growth rate arise from the variety of geographically overlapping CH4 sources and from the destruction of CH4 by short-lived hydroxyl radicals (OH). To address these challenges, we have established a consortium of multidisciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate new research aimed at improving and regularly updating the global methane budget. Following Saunois et al. (2016), we present here the second version of the living review paper dedicated to the decadal methane budget, integrating results of top-down studies (atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up estimates (including process-based models for estimating land surface emissions and atmospheric chemistry, inventories of anthropogenic emissions, and data-driven extrapolations). For the 2008–2017 decade, global methane emissions are estimated by atmospheric inversions (a top-down approach) to be 576 Tg CH4 yr−1 (range 550–594, corresponding to the minimum and maximum estimates of the model ensemble). Of this total, 359 Tg CH4 yr−1 or ∼ 60 % is attributed to anthropogenic sources, that is emissions caused by direct human activity (i.e. anthropogenic emissions; range 336–376 Tg CH4 yr−1 or 50 %–65 %). The mean annual total emission for the new decade (2008–2017) is 29 Tg CH4 yr−1 larger than our estimate for the previous decade (2000–2009), and 24 Tg CH4 yr−1 larger than the one reported in the previous budget for 2003–2012 (Saunois et al., 2016). Since 2012, global CH4 emissions have been tracking the warmest scenarios assessed by the Intergovernmental Panel on Climate Change. Bottom-up methods suggest almost 30 % larger global emissions (737 Tg CH4 yr−1, range 594–881) than top-down inversion methods. Indeed, bottom-up estimates for natural sources such as natural wetlands, other inland water systems, and geological sources are higher than top-down estimates. The atmospheric constraints on the top-down budget suggest that at least some of these bottom-up emissions are overestimated. The latitudinal distribution of atmospheric observation-based emissions indicates a predominance of tropical emissions (∼ 65 % of the global budget, 〈 30∘ N) compared to mid-latitudes (∼ 30 %, 30–60∘ N) and high northern latitudes (∼ 4 %, 60–90∘ N). The most important source of uncertainty in the methane budget is attributable to natural emissions, especially those from wetlands and other inland waters. Some of our global source estimates are smaller than those in previously published budgets (Saunois et al., 2016; Kirschke et al., 2013). In particular wetland emissions are about 35 Tg CH4 yr−1 lower due to improved partition wetlands and other inland waters. Emissions from geological sources and wild animals are also found to be smaller by 7 Tg CH4 yr−1 by 8 Tg CH4 yr−1, respectively. However, the overall discrepancy between bottom-up and top-down estimates has been reduced by only 5 % compared to Saunois et al. (2016), due to a higher estimate of emissions from inland waters, highlighting the need for more detailed research on emissions factors. Priorities for improving the methane budget include (i) a global, high-resolution map of water-saturated soils and inundated areas emitting methane based on a robust classification of different types of emitting habitats; (ii) further development of process-based models for inland-water emissions; (iii) intensification of methane observations at local scales (e.g., FLUXNET-CH4 measurements) and urban-scale monitoring to constrain bottom-up land surface models, and at regional scales (surface networks and satellites) to constrain atmospheric inversions; (iv) improvements of transport models and the representation of photochemical sinks in top-down inversions; and (v) development of a 3D variational inversion system using isotopic and/or co-emitted species such as ethane to improve source partitioning. The data presented here can be downloaded from https://doi.org/10.18160/GCP-CH4-2019 (Saunois et al., 2020) and from the Global Carbon Project.
    Type of Medium: Online Resource
    ISSN: 1866-3516
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2020
    detail.hit.zdb_id: 2475469-9
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  • 4
    In: Frontiers in Marine Science, Frontiers Media SA, Vol. 6 ( 2019-4-26)
    Type of Medium: Online Resource
    ISSN: 2296-7745
    Language: Unknown
    Publisher: Frontiers Media SA
    Publication Date: 2019
    detail.hit.zdb_id: 2757748-X
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  • 5
    In: Global Biogeochemical Cycles, American Geophysical Union (AGU), Vol. 35, No. 2 ( 2021-02)
    Abstract: In a Global Ocean Biogeochemical Model, we simulate short continental shelf water residence times driven by dominant open ocean inflows These hydrodynamical features lead to net autotrophy and a slight sink of atmospheric CO 2 over the preindustrial global shelf The results also suggest that the global continental shelf is a less efficient sink of anthropogenic CO 2 than the open ocean
    Type of Medium: Online Resource
    ISSN: 0886-6236 , 1944-9224
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2021
    detail.hit.zdb_id: 2021601-4
    SSG: 12
    SSG: 13
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  • 6
    Online Resource
    Online Resource
    American Geophysical Union (AGU) ; 2015
    In:  Global Biogeochemical Cycles Vol. 29, No. 5 ( 2015-05), p. 534-554
    In: Global Biogeochemical Cycles, American Geophysical Union (AGU), Vol. 29, No. 5 ( 2015-05), p. 534-554
    Abstract: First global maps of river CO 2 partial pressures and evasion at 0.5° resolution Global river CO 2 evasion estimated at 650 (483–846) Tg C yr −1 Latitudes between 10°N and 10°S contribute half of the global CO 2 evasion
    Type of Medium: Online Resource
    ISSN: 0886-6236 , 1944-9224
    URL: Issue
    Language: English
    Publisher: American Geophysical Union (AGU)
    Publication Date: 2015
    detail.hit.zdb_id: 2021601-4
    SSG: 12
    SSG: 13
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  • 7
    In: Biogeosciences, Copernicus GmbH, Vol. 15, No. 6 ( 2018-03-22), p. 1701-1720
    Abstract: Abstract. The calculation of the air–water CO2 exchange (FCO2) in the ocean not only depends on the gradient in CO2 partial pressure at the air–water interface but also on the parameterization of the gas exchange transfer velocity (k) and the choice of wind product. Here, we present regional and global-scale quantifications of the uncertainty in FCO2 induced by several widely used k formulations and four wind speed data products (CCMP, ERA, NCEP1 and NCEP2). The analysis is performed at a 1°  ×  1° resolution using the sea surface pCO2 climatology generated by Landschützer et al. (2015a) for the 1991–2011 period, while the regional assessment relies on the segmentation proposed by the Regional Carbon Cycle Assessment and Processes (RECCAP) project. First, we use k formulations derived from the global 14C inventory relying on a quadratic relationship between k and wind speed (k = c ⋅ U102; Sweeney et al., 2007; Takahashi et al., 2009; Wanninkhof, 2014), where c is a calibration coefficient and U10 is the wind speed measured 10 m above the surface. Our results show that the range of global FCO2, calculated with these k relationships, diverge by 12 % when using CCMP, ERA or NCEP1. Due to differences in the regional wind patterns, regional discrepancies in FCO2 are more pronounced than global. These global and regional differences significantly increase when using NCEP2 or other k formulations which include earlier relationships (i.e., Wanninkhof, 1992; Wanninkhof et al., 2009) as well as numerous local and regional parameterizations derived experimentally. To minimize uncertainties associated with the choice of wind product, it is possible to recalculate the coefficient c globally (hereafter called c∗) for a given wind product and its spatio-temporal resolution, in order to match the last evaluation of the global k value. We thus performed these recalculations for each wind product at the resolution and time period of our study but the resulting global FCO2 estimates still diverge by 10 %. These results also reveal that the Equatorial Pacific, the North Atlantic and the Southern Ocean are the regions in which the choice of wind product will most strongly affect the estimation of the FCO2, even when using c∗.
    Type of Medium: Online Resource
    ISSN: 1726-4189
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2018
    detail.hit.zdb_id: 2158181-2
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  • 8
    In: Biogeosciences, Copernicus GmbH, Vol. 14, No. 19 ( 2017-10-13), p. 4545-4561
    Abstract: Abstract. In spite of the recent strong increase in the number of measurements of the partial pressure of CO2 in the surface ocean (pCO2), the air–sea CO2 balance of the continental shelf seas remains poorly quantified. This is a consequence of these regions remaining strongly under-sampled in both time and space and of surface pCO2 exhibiting much higher temporal and spatial variability in these regions compared to the open ocean. Here, we use a modified version of a two-step artificial neural network method (SOM-FFN; Landschützer et al., 2013) to interpolate the pCO2 data along the continental margins with a spatial resolution of 0.25° and with monthly resolution from 1998 to 2015. The most important modifications compared to the original SOM-FFN method are (i) the much higher spatial resolution and (ii) the inclusion of sea ice and wind speed as predictors of pCO2. The SOM-FFN is first trained with pCO2 measurements extracted from the SOCATv4 database. Then, the validity of our interpolation, in both space and time, is assessed by comparing the generated pCO2 field with independent data extracted from the LDVEO2015 database. The new coastal pCO2 product confirms a previously suggested general meridional trend of the annual mean pCO2 in all the continental shelves with high values in the tropics and dropping to values beneath those of the atmosphere at higher latitudes. The monthly resolution of our data product permits us to reveal significant differences in the seasonality of pCO2 across the ocean basins. The shelves of the western and northern Pacific, as well as the shelves in the temperate northern Atlantic, display particularly pronounced seasonal variations in pCO2,  while the shelves in the southeastern Atlantic and in the southern Pacific reveal a much smaller seasonality. The calculation of temperature normalized pCO2 for several latitudes in different oceanic basins confirms that the seasonality in shelf pCO2 cannot solely be explained by temperature-induced changes in solubility but are also the result of seasonal changes in circulation, mixing and biological productivity. Our results also reveal that the amplitudes of both thermal and nonthermal seasonal variations in pCO2 are significantly larger at high latitudes. Finally, because this product's spatial extent includes parts of the open ocean as well, it can be readily merged with existing global open-ocean products to produce a true global perspective of the spatial and temporal variability of surface ocean pCO2.
    Type of Medium: Online Resource
    ISSN: 1726-4189
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2017
    detail.hit.zdb_id: 2158181-2
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  • 9
    In: Annual Review of Earth and Planetary Sciences, Annual Reviews, Vol. 50, No. 1 ( 2022-05-31), p. 593-626
    Abstract: This review examines the current understanding of the global coastal ocean carbon cycle and provides a new quantitative synthesis of air-sea CO 2 exchange. This reanalysis yields an estimate for the globally integrated coastal ocean CO 2 flux of −0.25 ± 0.05 Pg C year −1 , with polar and subpolar regions accounting for most of the CO 2 removal ( 〉 90%). A framework that classifies river-dominated ocean margin (RiOMar) and ocean-dominated margin (OceMar) systems is used to conceptualizecoastal carbon cycle processes. The carbon dynamics in three contrasting case study regions, the Baltic Sea, the Mid-Atlantic Bight, and the South China Sea, are compared in terms of the spatio-temporal variability of surface pCO 2 . Ocean carbon models that range from box models to three-dimensional coupled circulation-biogeochemical models are reviewed in terms of the ability to simulate key processes and project future changes in different continental shelf regions. Common unresolved challenges remain for implementation of these models across RiOMar and OceMar systems. The long-term trends in coastal ocean carbon fluxes for different coastal systems under anthropogenic stress that are emerging in observations and numerical simulations are highlighted. Knowledge gaps in projecting future perturbations associated with before and after net-zero CO 2 emissions in the context of concurrent changes in the land-ocean-atmosphere coupled system pose a key challenge. ▪ A new synthesis yields an estimate for a globally integrated coastal ocean carbon sink of −0.25 Pg C year −1 , with greater than 90% of atmospheric CO 2 removal occurring in polar and subpolar regions. ▪ The sustained coastal and open ocean carbon sink is vital in mitigating climate change and meeting the target set by the Paris Agreement. ▪ Uncertainties in the future coastal ocean carbon cycle are associated with concurrent trends and changes in the land-ocean-atmosphere coupled system. ▪ The major gaps and challenges identified for current coastal ocean carbon research have important implications for climate and sustainability policies.
    Type of Medium: Online Resource
    ISSN: 0084-6597 , 1545-4495
    URL: Issue
    Language: English
    Publisher: Annual Reviews
    Publication Date: 2022
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    detail.hit.zdb_id: 2010309-8
    SSG: 16,13
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  • 10
    In: Science of The Total Environment, Elsevier BV, Vol. 881 ( 2023-07), p. 163450-
    Type of Medium: Online Resource
    ISSN: 0048-9697
    RVK:
    Language: English
    Publisher: Elsevier BV
    Publication Date: 2023
    detail.hit.zdb_id: 1498726-0
    detail.hit.zdb_id: 121506-1
    SSG: 12
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