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  • Physics  (3)
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  • Physics  (3)
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  • 1
    In: Advanced Materials, Wiley, Vol. 34, No. 31 ( 2022-08)
    Abstract: Organic solar cells (OSCs) are promising candidates for next‐generation photovoltaic technologies, with their power conversion efficiencies (PCEs) reaching 19%. However, the typically used spin‐coating method, toxic halogenated processing solvents, and the conventional bulk‐heterojunction (BHJ), which causes excessive charge recombination, hamper the commercialization and further efficiency promotion of OSCs. Here, a simple but effective dual‐slot‐die sequential processing (DSDS) strategy is proposed to address the above issues by achieving a continuous solution supply, avoiding the solubility limit of the nonhalogen solvents, and creating a graded‐BHJ morphology. As a result, an excellent PCE of 17.07% is obtained with the device processed with o ‐xylene in an open‐air environment with no post‐treatment required, while a PCE of over 14% is preserved in a wide range of active‐layer thickness. The unique film‐formation mechanism is further identified during the DSDS processing, which suggests the formation of the graded‐BHJ morphology by the mutual diffusion between the donor and acceptor and the subsequent progressive aggregation. The graded‐BHJ structure leads to improved charge transport, inhibited charge recombination, and thus an excellent PCE. Therefore, the newly developed DSDS approach can effectively contribute to the realm of high‐efficiency and eco‐friendly OSCs, which can also possibly be generalized to other organic photoelectric devices.
    Type of Medium: Online Resource
    ISSN: 0935-9648 , 1521-4095
    URL: Issue
    RVK:
    Language: English
    Publisher: Wiley
    Publication Date: 2022
    detail.hit.zdb_id: 1474949-X
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  • 2
    Online Resource
    Online Resource
    AIP Publishing ; 2014
    In:  Applied Physics Letters Vol. 105, No. 13 ( 2014-09-29)
    In: Applied Physics Letters, AIP Publishing, Vol. 105, No. 13 ( 2014-09-29)
    Abstract: Particle image velocimetry was applied in the study focusing on the structure and velocity of water jets injected into a Ma = 2.1 crossflow. The instantaneous structures of the jet, including surface waves in the near-injector region and vortices in the far-field, were visualized clearly. Spray velocity increases rapidly to 66% of the mainstream velocity in the region of x/d  & lt; 15, owing to the strong gas-liquid interaction near the orifice. By contrast, the velocity grows slowly in the far-field region, where the liquid inside the spray is accelerated mainly by the continuous driven force provided by the mainstream with the gas-liquid shear. The injection and atomization of liquid jet in a supersonic crossflow serves as a foundation of scramjet combustion process, by affecting the combustion efficiency and some other performances. With various forces acting on the liquid jet (Mashayek et al. [AIAA J. 46, 2674–2686 (2008)] and Wang et al. [AIAA J. 50, 1360–1366 (2012)] ), the atomization process involves very complex flow physics. These physical processes include strong vortical structures, small-scale wave formation, stripping of small droplets from the jet surface, formations of ligaments, and droplets with a wide range of sizes.
    Type of Medium: Online Resource
    ISSN: 0003-6951 , 1077-3118
    RVK:
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2014
    detail.hit.zdb_id: 211245-0
    detail.hit.zdb_id: 1469436-0
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  • 3
    Online Resource
    Online Resource
    AIP Publishing ; 2015
    In:  Applied Physics Letters Vol. 107, No. 10 ( 2015-09-07)
    In: Applied Physics Letters, AIP Publishing, Vol. 107, No. 10 ( 2015-09-07)
    Abstract: Phase Doppler anemometry was applied to investigate the atomization processes of a kerosene jet injected into Ma = 1.86 crossflow. Physical behaviors, such as breakup and coalescence, are reproduced through the analysis of the spatial distribution of kerosene droplets' size. It is concluded that Sauter mean diameter distribution shape transforms into “I” type from “C” type as the atomization development. Simultaneously, the breakup of large droplets and the coalescence of small droplets can be observed throughout the whole atomization process.
    Type of Medium: Online Resource
    ISSN: 0003-6951 , 1077-3118
    RVK:
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2015
    detail.hit.zdb_id: 211245-0
    detail.hit.zdb_id: 1469436-0
    Location Call Number Limitation Availability
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