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  • 1
    Online Resource
    Online Resource
    Enzyme‐Mediated Tumor Starvation and Phototherapy Enhance Mild‐Temperature Photothermal Therapy
    Wiley ; 2020
    In:  Advanced Functional Materials Vol. 30, No. 16 ( 2020-04)
    Details
    In: Advanced Functional Materials, Wiley, Vol. 30, No. 16 ( 2020-04)
    Abstract: Compared with conventional tumor photothermal therapy (PTT), mild‐temperature PTT brings less damage to normal tissues, but also tumor thermoresistance, introduced by the overexpressed heat shock protein (HSP). A high dose of HSP inhibitor during mild‐temperature PTT might lead to toxic side effects. Glucose oxidase (GOx) consumes glucose, leading to adenosine triphosphate supply restriction and consequent HSP inhibition. Therefore, a combinational use of an HSP inhibitor and GOx not only enhances mild‐temperature PTT but also minimizes the toxicity of the inhibitor. However, a GOx and HSP inhibitor‐encapsulating nanostructure, designed for enhancing its mild‐temperature tumor PTT efficiency, has not been reported. Thermosensitive GOx/indocyanine green/gambogic acid (GA) liposomes (GOIGLs) are reported to enhance the efficiency of mild‐temperature PTT of tumors via synergistic inhibition of tumor HSP by the released GA and GOx, together with another enzyme‐enhanced phototherapy effect. In vitro and in vivo results indicate that this strategy of tumor starvation and phototherapy significantly enhances mild‐temperature tumor PTT efficiency. This strategy could inspire people to design more delicate platforms combining mild‐temperature PTT with other therapeutic methods for more efficient cancer treatment.
    Type of Medium: Online Resource
    ISSN: 1616-301X , 1616-3028
    URL: Issue
    URL: Article
    DOI: 10.1002/adfm.v30.16
    DOI: 10.1002/adfm.201909391
    Language: English
    Publisher: Wiley
    Publication Date: 2020
    detail.hit.zdb_id: 2029061-5
    detail.hit.zdb_id: 2039420-2
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  • 2
    Online Resource
    Online Resource
    Influence of Temperature and Current Stressing on Cu‐Sn Intermetallic Compound Growth Characteristics of Lead‐Free Microbump
    Wiley ; 2023
    In:  Advanced Theory and Simulations Vol. 6, No. 4 ( 2023-04)
    Details
    In: Advanced Theory and Simulations, Wiley, Vol. 6, No. 4 ( 2023-04)
    Abstract: A numerical analysis of the Cu flux on Cu/Sn/Cu is successfully used to establish kinetic models that are verified with reported data. Kinetic models are adopted to discuss the polarity effect of intermetallic compounds (IMCs) growth at different alloying stages. The models reveal that, before Sn solder is depleted during thermal aging, the net thermodiffusion Cu flux in Cu 6 Sn 5 is over three times larger than that in Cu 3 Sn. While coupling with current stressing, the IMCs thickness increases from parabola‐like curves to a linear‐like relationship. The degree of influence decreases in the order of Cu 6 Sn 5 on anode, Cu 6 Sn 5 on cathode, Cu 3 Sn on anode, and Cu 3 Sn on cathode. Electromigration Cu flux in Sn is the critical factor that accelerates the anode's Cu 6 Sn 5 growth, and its influence on the growth rate over 1000 times that on the anode's Cu 3 Sn. After Sn solder is depleted, Cu 6 Sn 5 gradually converts into Cu 3 Sn, and its thickness is linearly decreases with square root of annealing time. When coupling with a current density of 1.0 × 10 5 A cm −2 , the thickness ratio of Cu 3 Sn/Cu 6 Sn 5 reduces from 1:2 to 1:6. Remarkably, irrespective of whether current exists or not, the depletion of Cu 6 Sn 5 always takes much longer than that of Sn solder.
    Type of Medium: Online Resource
    ISSN: 2513-0390 , 2513-0390
    URL: Issue
    URL: Article
    DOI: 10.1002/adts.v6.4
    DOI: 10.1002/adts.202200881
    Language: English
    Publisher: Wiley
    Publication Date: 2023
    detail.hit.zdb_id: 2894557-8
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  • 3
    Online Resource
    Online Resource
    Role‐Specialized Division of Labor in CO 2 Reduction with Doubly‐Functionalized Iron Porphyrin Atropisomers
    Wiley ; 2022
    In:  Angewandte Chemie International Edition Vol. 61, No. 35 ( 2022-08-26)
    Details
    In: Angewandte Chemie International Edition, Wiley, Vol. 61, No. 35 ( 2022-08-26)
    Abstract: In enzymes, the active site residues function differently to promote chemical reactions. Such a role‐specialized division of labor has been rarely realized by synthetic catalysts. We report herein on catalytic CO 2 reduction with Fe porphyrins decorated with two cationic N,N,N ‐trimethylbenzylamine groups in cis ‐ or trans ‐arrangement. The cis ‐isomer outperforms the trans ‐isomer and reaches a TOF max of 4.4×10 5 s −1 in acetonitrile using phenol proton source. Theoretical studies revealed that the two cationic units in the cis ‐isomer are more effective than a single cationic unit to improve the CO 2 binding, and more importantly, they function differently but cooperatively to promote the C−O bond cleavage: one interacts with the CO 2 ‐adduct, while the other one interacts with the phenol molecule through electrostatic interactions. This work therefore presents a significant example of synthetic catalysts, which boost chemical reactions using a role‐specialized strategy for substrate activation.
    Type of Medium: Online Resource
    ISSN: 1433-7851 , 1521-3773
    URL: Issue
    URL: Article
    DOI: 10.1002/anie.v61.35
    DOI: 10.1002/anie.202209602
    RVK:
    VA 2100
    Language: English
    Publisher: Wiley
    Publication Date: 2022
    detail.hit.zdb_id: 2011836-3
    detail.hit.zdb_id: 123227-7
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  • 4
    Online Resource
    Online Resource
    Role‐Specialized Division of Labor in CO 2 Reduction with Doubly‐Functionalized Iron Porphyrin Atropisomers
    Wiley ; 2022
    In:  Angewandte Chemie Vol. 134, No. 35 ( 2022-08-26)
    Details
    In: Angewandte Chemie, Wiley, Vol. 134, No. 35 ( 2022-08-26)
    Abstract: In enzymes, the active site residues function differently to promote chemical reactions. Such a role‐specialized division of labor has been rarely realized by synthetic catalysts. We report herein on catalytic CO 2 reduction with Fe porphyrins decorated with two cationic N,N,N ‐trimethylbenzylamine groups in cis ‐ or trans ‐arrangement. The cis ‐isomer outperforms the trans ‐isomer and reaches a TOF max of 4.4×10 5 s −1 in acetonitrile using phenol proton source. Theoretical studies revealed that the two cationic units in the cis ‐isomer are more effective than a single cationic unit to improve the CO 2 binding, and more importantly, they function differently but cooperatively to promote the C−O bond cleavage: one interacts with the CO 2 ‐adduct, while the other one interacts with the phenol molecule through electrostatic interactions. This work therefore presents a significant example of synthetic catalysts, which boost chemical reactions using a role‐specialized strategy for substrate activation.
    Type of Medium: Online Resource
    ISSN: 0044-8249 , 1521-3757
    URL: Issue
    URL: Article
    DOI: 10.1002/ange.v134.35
    DOI: 10.1002/ange.202209602
    RVK:
    VA 2100
    RVK:
    VN 5020
    Language: English
    Publisher: Wiley
    Publication Date: 2022
    detail.hit.zdb_id: 505868-5
    detail.hit.zdb_id: 506609-8
    detail.hit.zdb_id: 514305-6
    detail.hit.zdb_id: 505872-7
    detail.hit.zdb_id: 1479266-7
    detail.hit.zdb_id: 505867-3
    detail.hit.zdb_id: 506259-7
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  • 5
    Online Resource
    Online Resource
    Dominance complementation of parental heading date alleles of Hd1, Ghd7 , DTH8 , and PRR37 confers transgressive late maturation in hybrid rice
    Wiley ; 2024
    In:  The Plant Journal Vol. 118, No. 6 ( 2024-06), p. 2108-2123
    Details
    In: The Plant Journal, Wiley, Vol. 118, No. 6 ( 2024-06), p. 2108-2123
    Abstract: We identified the genetic basis of transgressive late maturation in hybrid rice, which is dependent on dominance complementation effects of Hd1 , Ghd7 , DTH8 , and PRR37 from both parents and developed effective methods for parental selection and gene editing to facilitate the breeding of hybrid varieties with the desired photoperiod sensitivity. Our study lays an important foundation for improving the breeding efficiency and latitude adaptability of hybrid rice.
    Type of Medium: Online Resource
    ISSN: 0960-7412 , 1365-313X
    URL: Issue
    URL: Article
    DOI: 10.1111/tpj.v118.6
    DOI: 10.1111/tpj.16732
    Language: English
    Publisher: Wiley
    Publication Date: 2024
    detail.hit.zdb_id: 2020961-7
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  • 6
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    Binary Nanoparticle Superlattices for Plasmonically Modulating Upconversion Luminescence
    Wiley ; 2020
    In:  Small Vol. 16, No. 38 ( 2020-09)
    Details
    In: Small, Wiley, Vol. 16, No. 38 ( 2020-09)
    Abstract: Engineering a facile and controllable approach to modulate the spectral properties of lanthanide‐doped upconversion nanoparticles (UCNPs) is always an ongoing challenge. Herein, long‐range ordered, distinct two‐dimensional (2D) binary nanoparticle superlattices (BNSLs) composed of NaREF 4 :Yb/Er (RE = Y and Gd) UCNPs and plasmonic metallic nanoparticles (Au NPs), including AB, AB 3 , and AB 13 lattices, are fabricated via a slow evaporation‐driven self‐assembly to achieve plasmonic modulation of upconversion luminescence (UCL). Optical measurements reveal that typical red–green UCL from UCNPs can be effectively modulated into reddish output in BNSLs, with a drastically shortened lifetime. Notably, for AB 3 ‐ and AB 13 ‐type BNSLs with more proximal Au NPs around each UCNP, modified UCL with fine‐structured spectral lineshape is observed. These differences could be interpreted by the interplay of collective plasmon resonance introduced by 2D periodic Au arrays and spectrally selective energy transfer between UCNPs and Au. Thus, fabricating UCNP‐Au BNSLs with desired lattice parameters and NP configurations could be a promising way to tailor the UCL through controlled plasmonic modulation.
    Type of Medium: Online Resource
    ISSN: 1613-6810 , 1613-6829
    URL: Issue
    URL: Article
    DOI: 10.1002/smll.v16.38
    DOI: 10.1002/smll.202002066
    Language: English
    Publisher: Wiley
    Publication Date: 2020
    detail.hit.zdb_id: 2168935-0
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  • 7
    Online Resource
    Online Resource
    Microwave‐Assisted Ultrafast Synthesis of Molybdenum Carbide Nanoparticles Grown on Carbon Matrix for Efficient Hydrogen Evolution Reaction
    Wiley ; 2019
    In:  Small Methods Vol. 3, No. 11 ( 2019-11)
    Details
    In: Small Methods, Wiley, Vol. 3, No. 11 ( 2019-11)
    Abstract: Molybdenum carbide (Mo 2 C) coupled with carbon materials has received widespread attention in catalysis and energy storge/conversion. However, most of the existing synthetic pathways involve high operating temperature, time‐consuming processes, and flammable gases. Herein, a novel, facile, and rapid method to synthesize Mo 2 C nanoparticles grown on a series of carbon substrates (such as graphene, carbon nanotubes, and commercial carbon black) in a few minutes by using the strong interaction between the microwave and the carbon materials, in which the carbon matrix acts as the in situ heating media and carbon sources to accelerate carbon diffusion during the formation of Mo 2 C, is presented. Moreover, this method can also be extended to prepare a self‐standing electrode (Mo 2 C/CF) in just 10 s, the uniformly dispersed Mo 2 C nanoparticles anchored on carbon fiber paper, which demonstrates superior catalytic performance and long‐term stability ( 〉 100 h) in both acid and alkaline conditions for hydrogen evolution reaction.
    Type of Medium: Online Resource
    ISSN: 2366-9608 , 2366-9608
    URL: Issue
    URL: Article
    DOI: 10.1002/smtd.v3.11
    DOI: 10.1002/smtd.201900259
    Language: English
    Publisher: Wiley
    Publication Date: 2019
    detail.hit.zdb_id: 2884448-8
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  • 8
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    Online Resource
    Population differentiation and epidemic tracking of Bursaphelenchus xylophilus in China based on chromosome‐level assembly and whole‐genome sequencing data
    Wiley ; 2022
    In:  Pest Management Science Vol. 78, No. 3 ( 2022-03), p. 1213-1226
    Details
    In: Pest Management Science, Wiley, Vol. 78, No. 3 ( 2022-03), p. 1213-1226
    Abstract: Bursaphelenchus xylophilus , the pinewood nematode, kills millions of pine trees worldwide every year, and causes enormous economic and ecological losses. Despite extensive research on population variation, there is little understanding of the population‐wide variation spectrum in China. RESULTS We sequenced an inbred B. xylophilus strain using Pacbio+Illumina+Bionano+Hi‐C and generated a chromosome‐level assembly (AH1) with six chromosomes of 77.1 Mb (chromosome N50: 12 Mb). The AH1 assembly shows very high continuity and completeness, and contains novel genes with potentially important functions compared with previous assemblies. Subsequently, we sequenced 181 strains from China and the USA and found ~7.8 million single nucleotide polymorphisms (SNPs). Analysis shows that the B. xylophilus population in China can be divided into geographically bounded subpopulations with severe cross‐infection and potential migrations. In addition, distribution of B. xylophilus is dominated by temperature zones while geographically associated SNPs are mainly located on adaptation related GPCR gene families, suggesting the nematode has been evolving to adapt to different temperatures. A machine‐learning based epidemic tracking method has been established to predict their geographical origins, which can be applied to any other species. CONCLUSION Our study provides the community with the first high‐quality chromosome‐level assembly which includes a comprehensive catalogue of genetic variations. It provides insights into population structure and effective tracking method for this invasive species, which facilitates future studies to address a variety of applied, genomic and evolutionary questions in B. xylophilus as well as related species.
    Type of Medium: Online Resource
    ISSN: 1526-498X , 1526-4998
    URL: Issue
    URL: Article
    DOI: 10.1002/ps.v78.3
    DOI: 10.1002/ps.6738
    Language: English
    Publisher: Wiley
    Publication Date: 2022
    detail.hit.zdb_id: 2003455-6
    SSG: 12
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  • 9
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    Millennial‐ to centennial‐scale anti‐phase relationship between the Westerlies and the East Asian summer monsoon and its cultural response along the Silk Roads after a great earthquake in southern Altay ~ 3500 cal a BP
    Wiley ; 2023
    In:  Journal of Quaternary Science Vol. 38, No. 1 ( 2023-01), p. 123-137
    Details
    In: Journal of Quaternary Science, Wiley, Vol. 38, No. 1 ( 2023-01), p. 123-137
    Abstract: It is strongly debated whether the Westerlies and the East Asian summer monsoon (EASM) are in‐phase, anti‐phase or out‐of‐phase, and how hydroclimatic changes in the above two climate systems affected trans ‐Eurasian cultural exchanges during the late Holocene. In this study, we establish a 3500‐a‐long paleoclimatic sequence based on high‐resolution analyses of sedimentological and geochemical data of a well‐dated sediment core from Yileimu Lake in southern Altay. High percentages of the 〉 63‐µm fraction and high values of Zr/Rb and Rb/Sr ratios indicate strong transport of weakly weathered, coarse sediments into the depocenter of the lake caused by enhanced surface runoff and catchment erosion associated with a wet climate, and vice versa. High values of Ca and total inorganic carbon (TIC) contents imply increased precipitation of endogenic carbonates in the lake water under intense evaporation associated with a dry climate, and vice versa. This new record indicates two wet intervals at 3500–2300 and 600–100 cal a bp , interrupted by a severe and prolonged dry interval from 2300 to 1000 cal a bp , and a mild dry interval with occasionally wet conditions from 1000 to 600 cal a bp. These results are broadly consistent with other paleoclimatic records in Westerlies‐dominated Asia and are generally anti‐phase with those in the EASM region. We suggest that a strengthening/weakening and southward/northward migration of the Westerlies during a negative/positive phase of the North Atlantic Oscillation (NAO) transported more/less water vapor into arid Asia. Meanwhile, a decreasing/increasing El Niño‐Southern Oscillation (ENSO) superimposed on a southward/northward shift of the Intertropical Convergence Zone (ITCZ) triggered a weakening/strengthening and southward/northward movement of the West‐Pacific subtropical high (WPSH), resulting in decreasing/increasing EASM intensity. In addition, the wet climate from 3500 to 2300 cal a bp may have contributed to the development of nomadic herding in the eastern Eurasian Steppe and Altay region, and to the opening of the proto‐Silk Roads. Potentially, intense seismic activities in the Altay Mountains ~3500 cal a bp may have also promoted the opening of the proto‐Silk Roads by forcing the herdsmen to move to the inter‐mountainous basins. The strong EASM intensity from 2300 to 1000 cal a bp in eastern China may have contributed to the creation of the ancient Silk Roads by the Han Dynasty.
    Type of Medium: Online Resource
    ISSN: 0267-8179 , 1099-1417
    URL: Issue
    URL: Article
    DOI: 10.1002/jqs.v38.1
    DOI: 10.1002/jqs.3468
    Language: English
    Publisher: Wiley
    Publication Date: 2023
    detail.hit.zdb_id: 2031875-3
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    SSG: 14
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  • 10
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    Flexible Ferroelectric Devices: Status and Applications
    Wiley ; 2022
    In:  Advanced Functional Materials Vol. 32, No. 45 ( 2022-11)
    Details
    In: Advanced Functional Materials, Wiley, Vol. 32, No. 45 ( 2022-11)
    Abstract: Flexible electronic devices have been extensively studied for their advantages of distinguished portability, conformal contact characteristics, and human‐friendly interfaces compared with conventional bulk Si technology. Flexible electronics can be attached to various surfaces like skin and internal organs for human–machine interaction, which has made significant advances in electronics, medicine, neuromorphic computing, etc. Owing to the innovation and maturation of the thin film preparation process, which have promoted the successful preparation of high‐quality flexible ferroelectric films. Herein, the preparation of flexible ferroelectric devices and the progress of their applications in recent years are reviewed. Prevailing methods for preparing flexible ferroelectric films including the van der Waals heteroepitaxy on flexible substrate, delamination of the ferroelectric films on rigid substrate by chemical etching techniques, and direct use of novel 2D ferroelectric materials etc. are summarized. The research progress of flexible ferroelectric devices applied to memories, sensors, photovoltaic devices, and energy harvesters are also be discussed in detail. Moreover, the potential applications of flexible ferroelectric devices in the field of neuromorphic computing are studied, a new trend which contributes to the further development of brain‐like chip systems. Finally, the challenges and prospects of flexible ferroelectric devices in the future advanced electronics are briefly proposed.
    Type of Medium: Online Resource
    ISSN: 1616-301X , 1616-3028
    URL: Issue
    URL: Article
    DOI: 10.1002/adfm.v32.45
    DOI: 10.1002/adfm.202205933
    Language: English
    Publisher: Wiley
    Publication Date: 2022
    detail.hit.zdb_id: 2029061-5
    detail.hit.zdb_id: 2039420-2
    SSG: 11
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