In:
Optics Letters, Optica Publishing Group, Vol. 45, No. 23 ( 2020-12-01), p. 6450-
Abstract:
Highly efficient tandem organic light-emitting diodes (TOLEDs) were achieved based on a non-doped charge generation unit (CGU) consisting of LiF/Al/C60/4,4’,4”-tris(N-3-methylphenyl-N-phenyl-amino) triphenylamine (m-MTDATA) and ultrathin emitting layers. The current–voltage characteristics of the CGU devices and electron-only devices and the capacitance–voltage characteristics of the CGU-based capacitance devices were characterized to explore the charge generation and injection mechanisms. The charge generation process occurs at the interface of C60/m–MTDATA through electron transferring from the highest occupied molecular orbital of m-MTDATA to the lowest unoccupied molecular orbital of C60. It is found that the thinner C60 layer contributes to efficient electron injection. Under the optimal structure, the blue TOLEDs exhibit a maximum current efficiency ( C E max ) of 43.3 cd/A. The C E max and maximum external quantum efficiency ( E Q E max ) of the white TOLEDs reach 84.6 cd/A and 26.7%, respectively.
Type of Medium:
Online Resource
ISSN:
0146-9592
,
1539-4794
Language:
English
Publisher:
Optica Publishing Group
Publication Date:
2020
detail.hit.zdb_id:
243290-0
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