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  • Copernicus GmbH  (4)
  • 1
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 23, No. 9 ( 2023-05-17), p. 5517-5531
    Abstract: Abstract. Reliable observations of aerosol optical properties are crucial for quantifying the radiative forcing of climate. The simultaneous measurements of aerosol optical properties at three wavelengths for PM1 and PM10 were conducted in urban Beijing from March 2018 to February 2022. The aerosol absorption coefficient (σab) at 550 nm of PM10 and PM1 decreased by 55.0 % and 53.5 % from 2018 to 2021. The significant reduction in σab may be related to reduced primary emissions caused by effective air pollution control measures. PM2.5 mass concentration decreased by 34.4 % from 2018 to 2021. Single scattering albedo (SSA) increased from 0.89±0.04 for PM10 (0.87±0.05 for PM1) in 2018 to 0.93±0.03 for PM10 (0.91±0.04 for PM1) in 2021. Increasing SSA and decreasing PM2.5 mass concentration suggest that the fraction of absorbing aerosols decreased with improved air quality due to pollution control measures being taken. The annual average submicron absorption ratio (Rab) increased from 86.1 % in 2018 to 89.2 % in 2021, suggesting that fine particles are the main contributors to total PM10 absorption and that the contribution of fine particles to absorption became more important. The absorption Ångström exponent (AAE) in winter decreased from 2018 to 2021, implying a decreasing contribution from brown carbon to light absorption, which may relate to the reduced emissions of biomass burning and coal combustion. During the study period, aerosol radiative forcing efficiency became more negative, mainly influenced by increasing SSA and was −27.0 and −26.2 W m−2 per aerosol optical depth (AOD) for PM10 and PM1 in 2021. Higher σab and PM2.5 mass concentrations were primarily distributed in clusters 4 and 5, transported from the south and the west of Beijing each year. σab and PM2.5 corresponding to clusters 4 and 5 decreased evidently from 2018 to 2021, which may result from the control of source emissions in surrounding regions of Beijing. The 4-year data presented in this study provide critical optical parameters for radiative forcing assessment within two size ranges and are helpful for evaluating the effectiveness of clean air action.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2023
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 2
    In: Earth System Dynamics, Copernicus GmbH, Vol. 12, No. 1 ( 2021-03-01), p. 253-293
    Abstract: Abstract. The Scenario Model Intercomparison Project (ScenarioMIP) defines and coordinates the main set of future climate projections, based on concentration-driven simulations, within the Coupled Model Intercomparison Project phase 6 (CMIP6). This paper presents a range of its outcomes by synthesizing results from the participating global coupled Earth system models. We limit our scope to the analysis of strictly geophysical outcomes: mainly global averages and spatial patterns of change for surface air temperature and precipitation. We also compare CMIP6 projections to CMIP5 results, especially for those scenarios that were designed to provide continuity across the CMIP phases, at the same time highlighting important differences in forcing composition, as well as in results. The range of future temperature and precipitation changes by the end of the century (2081–2100) encompassing the Tier 1 experiments based on the Shared Socioeconomic Pathway (SSP) scenarios (SSP1-2.6, SSP2-4.5, SSP3-7.0 and SSP5-8.5) and SSP1-1.9 spans a larger range of outcomes compared to CMIP5, due to higher warming (by close to 1.5 ∘C) reached at the upper end of the 5 %–95 % envelope of the highest scenario (SSP5-8.5). This is due to both the wider range of radiative forcing that the new scenarios cover and the higher climate sensitivities in some of the new models compared to their CMIP5 predecessors. Spatial patterns of change for temperature and precipitation averaged over models and scenarios have familiar features, and an analysis of their variations confirms model structural differences to be the dominant source of uncertainty. Models also differ with respect to the size and evolution of internal variability as measured by individual models' initial condition ensemble spreads, according to a set of initial condition ensemble simulations available under SSP3-7.0. These experiments suggest a tendency for internal variability to decrease along the course of the century in this scenario, a result that will benefit from further analysis over a larger set of models. Benefits of mitigation, all else being equal in terms of societal drivers, appear clearly when comparing scenarios developed under the same SSP but to which different degrees of mitigation have been applied. It is also found that a mild overshoot in temperature of a few decades around mid-century, as represented in SSP5-3.4OS, does not affect the end outcome of temperature and precipitation changes by 2100, which return to the same levels as those reached by the gradually increasing SSP4-3.4 (not erasing the possibility, however, that other aspects of the system may not be as easily reversible). Central estimates of the time at which the ensemble means of the different scenarios reach a given warming level might be biased by the inclusion of models that have shown faster warming in the historical period than the observed. Those estimates show all scenarios reaching 1.5 ∘C of warming compared to the 1850–1900 baseline in the second half of the current decade, with the time span between slow and fast warming covering between 20 and 27 years from present. The warming level of 2 ∘C of warming is reached as early as 2039 by the ensemble mean under SSP5-8.5 but as late as the mid-2060s under SSP1-2.6. The highest warming level considered (5 ∘C) is reached by the ensemble mean only under SSP5-8.5 and not until the mid-2090s.
    Type of Medium: Online Resource
    ISSN: 2190-4987
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2578793-7
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  • 3
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 23, No. 14 ( 2023-07-25), p. 8241-8257
    Abstract: Abstract. Mineral dust is a major natural atmospheric aerosol that impacts the Earth's radiation balance. The significant scavenging process of fine particles by the strong wind during the dust episodes provided a relatively clean environment that was favourable for new particle formation (NPF) occurrence. In this study, the NPF occurred following the dust episodes (dust-related NPF), and other cases under clean and polluted conditions were classified based on the long-term particle number size distribution (PNSD) in urban Beijing in spring from 2017 to 2021. It was found that the observed formation (Jobs) and growth rate (GR) of dust-related NPF events were approximately 50 % and 30 % lower than the values of other NPF days, respectively. A typical severe dust storm that originated from Mongolia and swept over northern China on 15–16 March 2021 was analysed, to illustrate how the dust storm influences the NPF event. The maximum hourly mean PM10 mass concentration reached 8000 µg m−3 during this dust storm. The occurrence of an NPF event after a dust storm was facilitated due to the low condensation sink (∼ 0.005 s−1) caused by the strong dilution process of pre-existing particles. However, a downward trend of particle hygroscopicity was found during dust storm and NPF event as compared with the polluted episode, resulting in an increasing trend of the critical diameter at different supersaturations (ss), where aerosols are activated as cloud condensation nuclei (CCN), although the NPF event occurred when dust faded. The critical diameter was elevated by approximately 6 %–10 % (ss = 0.2 % and 0.7 %) during the dust storm, resulting in a lower CCN activation ratio, especially at low supersaturation. Modifications of the nucleation and growth process, as well as the particle-size distribution and hygroscopicity of the dust particles, provide valuable information that reveals the underlying climate and air quality effects of Asian mineral dust.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2023
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 4
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 21, No. 9 ( 2021-05-07), p. 7039-7052
    Abstract: Abstract. Influenced by the spread of the global 2019 novel coronavirus (COVID-19) pandemic, primary emissions of particles and precursors associated with anthropogenic activities decreased significantly in China during the Chinese New Year of 2020 and the lockdown period (24 January–16 February 2020). The 2-month measurements of the number size distribution of neutral particles and charged ions showed that during the lockdown (LCD) period, the number concentration of particles smaller than 100 nm decreased by approximately 40 % compared to the pre-LCD period in January. However, the accumulation mode particles increased by approximately 20 % as several polluted episodes contributed to secondary aerosol formation. In this study, new particle formation (NPF) events were found to be enhanced in the nucleation and growth processes during the LCD period, as indicated by the higher formation rate of 2 nm particles (J2) and the subsequent growth rate (GR). The relevant precursors, e.g., SO2 and NO2, showed a clear reduction, and O3 increased by 80 % during LCD period, as compared with pre-LCD. The volatile organic vapors showed different trends due to their sources. The proxy sulfuric acid during the LCD period increased by approximately 26 %, as compared with pre-LCD. The major oxidants (O3, OH, and NO3) of VOCs were also found to be elevated during LCD. That indicated higher J2 and GR (especially below 5 nm) during the LCD period were favored by the increased concentration level of condensing vapors and decreased condensation sink. Several heavy haze episodes have been reported by other studies during the LCD period; however, the increase in nanoparticle number concentration should also be considered. Some typical NPF events produced a high number concentration of nanoparticles that intensified in the following days to create severe aerosol pollution under unfavorable meteorological conditions. Our study confirms a significant enhancement of the nucleation and growth process of nanoparticles during the COVID-19 LCD in Beijing and highlights the necessity of controlling nanoparticles in current and future air quality management.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
    Location Call Number Limitation Availability
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