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  • 1
    Electronic Resource
    Electronic Resource
    Crosslinked polyimide foams derived from poly(imidepropylene oxide) copolymers (1997)
    Weinheim : Wiley-Blackwell
    Macromolecular Chemistry and Physics 198 (1997), S. 549-559 
    Details
    ISSN: 1022-1352
    Keywords: Chemistry ; Polymer and Materials Science
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology , Physics
    Notes: A new route for the synthesis of high glass transition temperature, thermally stable polymer foams has been developed, using compositionally asymmetric microphase-separated block copolymers where the minor component (poly(propylene oxide)) is thermally labile and the major component (polyimide) is thermally stable. The minor component decomposes to low molecular weight species upon heating, and the decomposition products diffuse out of the film, leaving behind pores embedded in a matrix of the thermally stable component. In this study, the polyimide block was crosslinked with ethynyl functionalities to obtain a stable porous structure. The decomposition of the propylene oxide in the block copolymer was studied by thermogravimetric, dynamic mechanical and thermomechanical analyses. Mild conditions were required to avoid rapid depolymerization of the propylene oxide and plasticization of the polyimide matrix. The foams showed pore sizes with diameters up to a micrometer in size as well as the expected reduction in the mass density.
    Additional Material: 5 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/macp.1997.021980227
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    Paper (German National Licenses)
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  • 2
    Electronic Resource
    Electronic Resource
    Transmission electron microscopy of 3F/PMDA-polypropylene oxide triblock copolymer based nanofoams (1997)
    Bognor Regis [u.a.] : Wiley-Blackwell
    Journal of Polymer Science Part B: Polymer Physics 35 (1997), S. 1067-1076 
    Details
    ISSN: 0887-6266
    Keywords: transmission electron microscopy ; block copolymer ; polyimide ; nanofoam ; porous films ; polymer foam ; Physics ; Polymer and Materials Science
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology , Physics
    Notes: Transmission electron microscopy was performed on a polymeric nanofoam material, derived from a triblock copolymer composed of a fluorinated polyimide center block, 3F/PMDA (derived from pyromelletic dianhydride (PMDA) and 1,1-bis(4-aminophenyl)-1-phenyl-2,2,2-trifluoroethane (3F)) and polypropylene oxide (PO) end blocks. The cast and imidized polymer exhibits a microphase-separated morphology consisting of PO microdomains within a polyimide matrix. The final nanofoam material is obtained by decomposing PO microdomains into low molecular weight products, which diffuse out of the polyimide matrix leaving nanometer length scale voids. Ruthenium tetroxide staining prior to microscopy was used to enhance the contrast between the 3F/PMDA matrix and the PO microdomains or voids, which permitted a more detailed view of the microstructure of both the foamed and unfoamed materials. From the power spectra of the micrographs, spatial correlation between the PO microdomains in the unfoamed material and between the voids in the foam were found. An interdomain separation distance of ca. 37 nm was observed. Analysis of the image yielded an average area of 411 nm2 for the PO domains. The analysis indicated that the PO domains were oblong, having average major and minor dimensions of 35 and 12.5 nm, respectively. An autocorrelation of the image showed that the domain center of masses were positioned 41 nm apart, in close agreement with the domain spacing (ca. 37 nm) found as described above. © 1997 John Wiley & Sons, Inc. J Polym Sci B: Polym Phys 35: 1067-1076, 1997
    Additional Material: 7 Ill.
    Type of Medium: Electronic Resource
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  • 3
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    Interventions to improve screening and appropriate referral of patients with cancer for distress: systematic review protocol (2015)
    BMJ Publishing
    In: BMJ Open
    Details
    Publication Date: 2015-09-23
    Description: Introduction It is estimated that 35–40% of patients with cancer experience distress at some stage during their illness. Distress may affect functioning, capacity to cope, treatment compliance, quality of life and survival of patients with cancer. Best practice clinical guidelines recommend routine psychosocial distress screening and referral for further assessment and/or psychosocial support for patients with cancer. However, evidence suggests this care is not provided consistently. Methods and analysis We developed our methods following the Preferred Reporting Items for Systematic Reviews and Meta-Analysis (PRISMA) statement. The review is registered with PROSPERO and any amendments to the protocol will be tracked. The primary aim of this systematic review is to examine the impact of interventions delivered in healthcare settings that are aimed at (1) improving routine screening of patients for psychosocial distress and (2) referral of distressed patients with cancer for further assessment and/or psychosocial support. The effectiveness of such interventions in reducing psychosocial distress, and any unintended adverse effect of the intervention will also be assessed in patients with cancer. Data sources will include the bibliographic databases Cochrane Central Register of Controlled trials (CENTRAL) in the Cochrane Library, MEDLINE, EMBASE, PsycINFO and CINAHL. Eligible studies must compare an intervention (or two or more interventions) in a healthcare setting to improve the rate of screening for psychosocial distress and/or referral for further assessment and/or psychosocial support for patients with cancer with no intervention or ‘usual’ practice. Two investigators will independently review titles and abstracts, followed by full article reviews and data extraction. Disagreements will be resolved by consensus and if necessary, a third reviewer. Where studies are sufficiently homogenous, trial data will be pooled and meta-analyses performed. Ethics and dissemination No ethical issues are foreseen. The findings of this study will be disseminated widely via peer-reviewed publications and conference presentations. Systematic review registration PROSPERO registration number CRD4 2015017518.
    Keywords: Open access, Evidence based practice, Mental health, Oncology
    Electronic ISSN: 2044-6055
    Topics: Medicine
    Published by BMJ Publishing
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  • 4
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    Smoking cessation care among patients with head and neck cancer: a systematic review (2016)
    BMJ Publishing
    In: BMJ Open
    Details
    Publication Date: 2016-09-22
    Description: Objective To examine the effectiveness of smoking cessation interventions in improving cessation rates and smoking related behaviour in patients with head and neck cancer (HNC). Design A systematic review of randomised and non-randomised controlled trials. Methods We searched the following data sources: CENTRAL in the Cochrane Library, MEDLINE, EMBASE, PsycINFO and CINAHL up to February 2016. A search of reference lists of included studies and Google Scholar (first 200 citations published online between 2000 and February 2016) was also undertaken. The methodological quality of included studies was assessed using the Effective Public Health Practice Project Quality Assessment Tool (EPHPP). 2 study authors independently screened and extracted data with disagreements resolved via consensus. Results Of the 5167 studies identified, 3 were eligible and included in the review. Trial designs of included studies were 2 randomised controlled trials and 1 non-randomised controlled trial. 2 studies received a weak methodological rating and 1 received a moderate methodological rating. The trials examine the impact of the following interventions: (1) nurse delivered cognitive–behaviour therapy (CBT) via telephone and accompanied by a workbook, combined with pharmacotherapy; (2) nurse and physician brief advice to quit and information booklets combined with pharmacotherapy; and (3) surgeon delivered enhanced advice to quit smoking augmented by booster sessions. Only the trial of the nurse delivered CBT and pharmacotherapy reported significant increases in smoking cessation rates. 1 study measured quit attempts and the other assessed consumption of cigarettes per day and readiness to change. There was no significant improvement in quit attempts or cigarettes smoked per day among patients in the intervention groups, relative to control. Conclusions There are very few studies evaluating the effectiveness of smoking cessation interventions that report results specific to the HNC population. The 3 trials identified reported equivocal findings. Extended CBT counselling coupled with pharmacotherapy may be effective. Trial registration number CRD42016016421.
    Keywords: Open access, Evidence based practice, Oncology, Smoking and tobacco
    Electronic ISSN: 2044-6055
    Topics: Medicine
    Published by BMJ Publishing
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  • 5
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    A new dynamic approach for statistical optimization of GNSS radio occultation bending angles for optimal climate monitoring utility (2013)
    Wiley-Blackwell
    Details
    Publication Date: 2013-11-14
    Description: [1]  Global Navigation Satellite Systems (GNSS) based radio occultation (RO) is a satellite remote sensing technique providing accurate profiles of the Earth's atmosphere for weather and climate applications. Above about 30 km altitude, however, statistical optimization is a critical process for initializing the RO bending angles in order to optimize the climate monitoring utility of the retrieved atmospheric profiles. Here we introduce an advanced dynamic statistical optimization algorithm, which uses bending angles from multiple days of European Centre for Medium-range Weather Forecasts (ECMWF) short-term forecast and analysis fields, together with averaged-observed bending angles, to obtain background profiles and associated error covariance matrices with geographically varying background uncertainty estimates on a daily-updated basis. The new algorithm is evaluated against the existing Wegener Center Occultation Processing System version 5.4 (OPSv5.4) algorithm, using several days of simulated MetOp and observed CHAMP and COSMIC data, for January and July conditions. We find the following for the new method's performance compared to OPSv5.4: 1. it significantly reduces random errors (standard deviations), down to about half their size, and leaves less or about equal residual systematic errors (biases) in the optimized bending angles; 2. the dynamic (daily) estimate of the background error correlation matrix alone already improves the optimized bending angles; 3. the subsequently retrieved refractivity profiles and atmospheric (temperature) profiles benefit by improved error characteristics, especially above about 30 km. Based on these encouraging results we work to employ similar dynamic error covariance estimation also for the observed bending angles and to apply the method to full months and subsequently to entire climate data records.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
    Published by Wiley-Blackwell on behalf of American Geophysical Union (AGU).
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  • 6
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    On the occurrence of equatorial F-region irregularities during solar minimum using radio occultation measurements (2013)
    Wiley-Blackwell
    Details
    Publication Date: 2013-01-11
    Description: [1]  The technique of radio occultation (RO) is demonstrated to be a powerful tool for studying equatorial F-region irregularities (EFIs) associated with equatorial plasma bubbles (EPBs). The extensive 4.9-year RO dataset of the Constellation Observing System for Meteorology, Ionosphere and Climate (COSMIC) satellites was employed in this study and contains EFI observations under a wide variety of solar and geomagnetic conditions. From an analysis of the EFI occurrence dependence on season/longitude, it is found that the EFI occurrence statistics largely match those reported previously, with the exception of an equinoctial EFI occurrence maximum in the American sector that is absent from previous studies. It is revealed that this maximum is due to enhanced EFI occurrence near the South Atlantic Anomaly, where EFIs are expected to be suppressed by particle precipitation. An investigation into the solar activity dependence of the EFI occurrence characteristics revealed significant increases in the range of local times and latitudes with solar activity for most longitude sectors and seasons. Finally, the EFI suppression and enhancement effects of storm-time electric fields are also investigated using the COSMIC data.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
    Published by Wiley-Blackwell on behalf of American Geophysical Union (AGU).
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  • 7
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    Interventions to improve screening and appropriate referral of patients with cancer for psychosocial distress: systematic review (2018)
    BMJ Publishing
    In: BMJ Open
    Details
    Publication Date: 2018-01-07
    Description: Objectives The primary aim of the review was to determine the effectiveness of strategies to improve clinician provision of psychosocial distress screening and referral of patients with cancer. Design Systematic review. Data sources Electronic databases (Cochrane Central Register of Controlled Trials, MEDLINE, EMBASE, PsycINFO and Cumulative Index to Nursing and Allied Health Literature (CINAHL)) were searched until July 2016. Inclusion criteria Population: adult patients with cancer and clinical staff members. Intervention: any strategy that aimed to improve the rate of routine screening and referral for detected distress of patients with cancer. Comparison: no intervention controls, ‘usual’ practice or alternative interventions. Outcome: (primary) any measure of provision of screening and/or referral for distress, (secondary) psychosocial distress, unintended adverse effects. Design: trials with or without a temporal comparison group, including randomised and non-randomised trials, and uncontrolled pre–post studies. Data extraction and analysis Two review authors independently extracted data. Heterogeneity across studies precluded quantitative assessment via meta-analysis and so a narrative synthesis of the results is presented. Results Five studies met the inclusion criteria. All studies were set in oncology clinics or departments and used multiple implementation strategies. Using the Grades of Recommendation, Assessment, Development and Evaluation, the overall rating of the certainty of the body of evidence reported in this review was assessed as very low. Three studies received a methodological quality rating of weak and two studies received a rating of moderate. Only one of the five studies reported a significant improvement in referrals. Conclusions The review identified five studies of predominantly poor quality examining the effectiveness of strategies to improve the routine implementation of distress screening and referral for patients with cancer. Future research using robust research designs, including randomised assignment, are needed to identify effective support strategies to maximise the potential for successful implementation of distress screening and referral for patients with cancer. PROSPERO registration number CRD42015017518 .
    Keywords: Open access, Oncology, Screening (epidemiology)
    Electronic ISSN: 2044-6055
    Topics: Medicine
    Published by BMJ Publishing
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