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  • Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences  (128)
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  • Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences  (128)
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  • 1
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 71, No. 6 ( 2022), p. 060702-
    Abstract: The structural properties and local contact potential difference of Au on Si(111)-(7×7) surface are studied by the homemade ultra-high vacuum non-contact Kelvin probe force microscope. Although scanning tunneling microscopy has been widely used to study the metal- adsorbed semiconductor surfaces on an atomic scale, the tunnel current measured by scanning tunneling microscopy is easy to lead the charge states to accidentally switch in the measurement process, and it is limited only to the observation of metal and semiconductor surfaces. Kelvin probe force microscope allows us to directly measure the charges at different positions of various flat surfaces by local contact potential difference on an atomic scale, which has become a more convenient and accurate means of charge characterization. In this paper, the topography and local contact potential difference of Au adsorbed Si(111)-(7×7) surface are measured on an atomic scale by Kelvin probe force microscope at room temperature, and the corresponding adsorption model and first principle calculation are established. The differential charge density distribution of the stable adsorption position of Au/Si(111)-(7×7) is obtained, and the local contact potential energy difference relationship of the stable adsorption position of Au on Si surface is given, The mechanism of charge transfer between Au atom and Si(111)-(7×7) surface during adsorption is analyzed. The experimental results show that at room temperature, single Au atom will form triangular delocalized adsorption state in the half unit cell of Si(111)-(7×7). The delocalized adsorption state is due to the fact that the moving speed of a single Au atom in the HUC is faster than the scanning speed of Kelvin probe force microscope, and the local contact potential difference measurement of Au/Si(111)-(7×7) adsorbed surface can effectively identify Au and Si atoms. Obviously, this research is of great significance in promoting the development of surface charge precision measurement, and is expected to provide some insights into the charge properties of metal adsorbed semiconductor surfaces.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2022
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  • 2
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 72, No. 11 ( 2023), p. 110701-
    Abstract: The physicochemical properties of Au atoms adsorbed on the surface on an atomic scale play a very important role in preparing nanodevices and surface catalysis. In this paper, we use frequency modulated Kelvin probe force microscopy (FM-KPFM)to study the multi-bit adsorbed charge distribution of Au on the surface of Si(111)-(7×7) at room temperature. Firstly, the surface topography and local contact potential difference (LCPD) of Au at different adsorption sites in Si(111)-(7×7) are successfully obtained by using home-made ultra-high vacuum Kelvin probe force microscopy. Secondly, we analyze the atomic characteristics of specific atomic positions of Au/Si(111)-(7×7) by force spectroscopy and potential difference, and realize the atomic identification . The adsorption characteristics of Au/Si(111)-(7×7) surface charge transfer and Au are explained by combining differential charge density calculations. The results show that Au atom adsorption mainly is in the form of single atom and cluster . Specifically, the Au cluster is adsorbed at the three central positions of Si(111)-(7×7) in a hexagonal structure of six atoms. Individual Au atoms are adsorbed to the positions of central adatoms of Si(111)-(7×7). At the same time, through the measurement of potential difference, it is known that a single Au atom and Au cluster lose electrons, presenting a positive electrical characteristic. The results of surface differential charge density show that Au undergoes charge transfer during adsorption, losing part of the charge, which locally reduces the work function at the position of the adsorbed atom. In the range of distances where short-range forces, local contact potential energy differences and differential charge densities change, the theoretical results and experimental results are in reasonable agreement.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2023
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  • 3
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 71, No. 23 ( 2022), p. 237501-
    Abstract: Fe-based amorphous and nanocrystalline alloys are considered as the preferred dual-green energy-saving materials due to their unique magnetic properties, such as high permeability, low coercivity, and near-zero saturation magnetostriction. As such, they have received extensive attention in applications like magnetic core material for high-frequency transformers, common model chokes, ground fault interrupters, and rotors in motors, over the past decades. In this work, Fe〈sub〉64.8〈/sub〉Co〈sub〉7.2〈/sub〉Nb〈sub〉4〈/sub〉Si〈sub〉4.8〈/sub〉B〈sub〉19.2〈/sub〉 (in atom percent) amorphous alloy ribbons are prepared by using the single roller quenching method, then subsequently subjected to multi-field coupling heating treatment in the air which includes heating by Joule heating effect and tensile stress field. Furthermore, the longitudinally driven giant magneto-impedance effect and magnetic domain structures of ribbons are observed by using 4294A impedance analyzer and magnetic force microscopy, respectively. The magneto-crystalline anisotropy field and stress anisotropy field of ribbons are analyzed by using X-ray diffraction, random anisotropy model, and numerical fitting. Meanwhile, the concept of magnetic anisotropy competing factor (〈i〉k〈/i〉) is proposed, from the viewpoint of magnetic anisotropy, a mechanism for regulating giant magneto-impedance effect of ribbons prepared with multi-field coupling is studied. It is found that the longitudinally driven giant magneto-impedance effect gradually transforms from the single peak to dome-like with tensile stress increasing. However, a spike and dome-like giant magneto-impedance effect appears during such transformation, which is composed of two parts: spike-like top and dome-like base. Based on the magnetic domain structure of ribbons, it is found that the typical stress-annealed transversal magnetic domain structure is observed in ribbons of 〈inline-formula〉〈tex-math id="Z-20221115160531"〉\begin{document}$k \leqslant 0.147$\end{document}〈/tex-math〉〈alternatives〉〈graphic xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="23-20221376_Z-20221115160531.jpg"/〉〈graphic xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="23-20221376_Z-20221115160531.png"/〉〈/alternatives〉〈/inline-formula〉, while nucleation and splitting phenomenon of new domains are observed at the transversal magnetic domain wall in ribbons of 〈i〉k〈/i〉 〉 0.147. Both longitudinally driven giant magneto-impedance effect and domain structures provide evidence to support the competing inhibition effect of magnetic anisotropy which exists in Fe-based alloy ribbon. Therefore, it is suggested that Fe-based alloys exhibit excellent stress-sensitive properties that can be understood by the competing inhibition effects of magnetic anisotropy. It is further shown that the competing inhibition effect of magnetic anisotropy is the main reason for regulating the giant magneto-impedance effect of soft magnetic materials. This multi-field coupling Fe-based alloy has good application prospects in regulating magnetic properties of magnetic materials.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2022
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  • 4
    Online Resource
    Online Resource
    Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences ; 2004
    In:  Acta Physica Sinica Vol. 53, No. 8 ( 2004), p. 2720-
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 53, No. 8 ( 2004), p. 2720-
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2004
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  • 5
    Online Resource
    Online Resource
    Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences ; 2003
    In:  Acta Physica Sinica Vol. 52, No. 5 ( 2003), p. 1307-
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 52, No. 5 ( 2003), p. 1307-
    Abstract: Differential optical absorption spectroscopy (DOAS) has become a widely used method to measure trace gases in the atmosphere.Their concentrations can be retrieved by a numerical analysis of the atmospheric absorption spectra. But it has been found that DOAS could not gain continuous data under a bad weather condition.Thus it could not fully fit for the demand of the environment monitoring statute.A prediction technology has been developed, based on the stepwise regression analysis method.It is shown that the forecasting data using this method is consistent with the real data after doing a great deal of experiments. This technology has been used in practice.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2003
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  • 6
    Online Resource
    Online Resource
    Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences ; 2014
    In:  Acta Physica Sinica Vol. 63, No. 16 ( 2014), p. 167502-
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 63, No. 16 ( 2014), p. 167502-
    Abstract: The Mn3Sn1-xCoxC1.1 compounds are synthesized by a solid-state reaction method. The effects of Co doping on the magnetic properties, phase transition and entropy change are investigated in Mn3Sn1-xCoxC1.1 compounds. The Curie temperature first decreases from 283 K to 212 K (Mn3Sn0.9Co0.1C1.1) with increasing the Co concentration, and then increases to 332 K (Mn3Sn0.2Co0.8C1.1) with further increasing the Co concentration in Mn3Sn1-xCoxC1.1. The first-order transition of Mn3Sn1-xCoxC1.1 gradually changes into the second-order transition, in the mean time, the entropy change decreases and the phase transition region broadens from 9 K to 300 K with increasing the Co content. Both the magnetic entropy change and broadening the transition temperature span can influence the relative cooling power R. Finally we obtain the large R=103 J/kg (H=1.6 MA/m) in Mn3Sn0.8Co0.2C1.1, which could be used as the room-temperature magnetic refrigerant materials.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2014
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  • 7
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 69, No. 21 ( 2020), p. 210701-
    Abstract: 〈sec〉Transition-metal-oxide as a typical model surface for investigating the catalytic mechanism has been widely studied. Over the past years, the TiO〈sub〉2〈/sub〉 properties have been reported. It is commonly accepted that the catalytic activity of reduced TiO〈sub〉2〈/sub〉 is related to its defects, with the accompanying excess electrons leading to n-type conductivity. It is realized that subsurface charge is of key importance for the redox chemistry of TiO〈sub〉2〈/sub〉 (110).〈/sec〉〈sec〉Subsurface charge is explored by atomic force microscopy (AFM) and Kelvin probe force microscopy (KPFM). Subsurface charge exerts an additional attractive force on the scanning AFM tip, resulting in the relative retraction of tip motion in order to keep a constant frequency shift. As a result, the subsurface charged region is imaged as protrusion in an AFM topographic image. The height of bright hillock is mainly distributed in three different ranges, which means that the subsurface charges are at three different subsurface layers. The AFM results show such subsurface charges repel the electropositive oxygen vacancy, hydrogen atoms and step edges. It is obvious that there is not only an O〈sub〉v〈/sub〉 depletion zone but also the subsurface charge free region in the proximity of the 〈inline-formula〉〈tex-math id="Z-20201022132953"〉\begin{document}$\left\langle {001} \right\rangle $\end{document}〈/tex-math〉〈alternatives〉〈graphic xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="21-20200773_Z-20201022132953.jpg"/〉〈graphic xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="21-20200773_Z-20201022132953.png"/〉〈/alternatives〉〈/inline-formula〉 and 〈inline-formula〉〈tex-math id="Z-20201022132947"〉\begin{document}$\left\langle {1\bar 11} \right\rangle$\end{document}〈/tex-math〉〈alternatives〉〈graphic xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="21-20200773_Z-20201022132947.jpg"/〉〈graphic xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="21-20200773_Z-20201022132947.png"/〉〈/alternatives〉〈/inline-formula〉 step edge.〈/sec〉〈sec〉The KPFM image indicates that the subsurface charges are the positive charges. which is consistent with common sense. After oxygen exposure, it is found that the oxygen adatom is electronegative, but it is absent in the vicinity of positive subsurface charges. Irrespective of adsorbate being electropositive or electronegative, an adsorbate-free zone generally exists in the proximity of the charged region. Obviously, the present study is expected to provide some insights into clarifying the nature of subsurface charge and improving catalytic design.〈/sec〉
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2020
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  • 8
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 65, No. 10 ( 2016), p. 108501-
    Abstract: In recent decades, infrared (IR) detection technology has been widely used in many fields such as weather monitoring, environmental protection, medical diagnostics, security protection, etc. With the progress and mature of the technologies, more attention has been paid to the imaging detections of weak IR signals. So the higher efficiency of the device is required. Moreover the next-generation IR photodetection technology focuses on large-scale, high-speed and low-dark-current imaging. The mechanical bonding between infrared detector chip and silicon readout circuit inevitably causes a thermal mismatch problem. Up-conversion IR photodetectors can solve the problem about the performance deterioration of photodetector and the thermal mismatch with silicon-based readout circuit, hence they have great advantages in realizing large-format focal plane array detection.However, the poor light extraction efficiency due to total reflection severely restricts the overall efficiency of the up-conversion device, which has become one of the bottlenecks to improve the device efficiency. In this paper, surface microstructures with micro-pillar morphology are designed and fabricated on quantum-cascade up-conversion IR photodetectors. The effect on the up-conversion efficiency is investigated by enhancing the light extraction efficiency.Firstly, by the optical ray retracing method, the influence of surface microstructure on light extraction efficiency is studied when considering different morphology parameters, and optimized surface microstructure is designed to possess a pillar base length of 150 nm, height of 105 nm and side wall angle of 75.Then based on the results of simulation, up-conversion IR photodetectors with surface microstructures are fabricated using polystyrene nanospheres as mask. The self-assembled monolayer nanospheres are first etched to a proper size by using O2 plasma, then the patterns are transferred to SiNx film, which acts as an ICP dry etching mask of the micro-pillars. Finally, the up-conversion device and a silicon detector are together loaded on a cold finger of a cryogenic dewar. The characteristics of the up-converter and up-conversion system are evaluated using a blackbody source.The experimental results show that the devices with and without surface microstructure exhibit similar IR responses and dark currents, while the emission of device with microstructure is obviously increased. Taking into consideration other factors related to external quantum efficiency, the light extraction efficiency of the device with micro-pillar structure on surface can be increased by up to 130%. Therefore it can be concluded that this method is an efficient way to improve the efficiency of up-conversion IR photodetector. The finding in this paper can also be applied to other semiconductor device with light extraction efficiency.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2016
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  • 9
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 64, No. 17 ( 2015), p. 178502-
    Abstract: Infrared (IR) photodetectors have been widely used in the fields of both civil and military applications such as environmental monitoring, medical diagnostics, satellite remote sensing and missile guidance, etc. In conventional large scale focal plane array (FPA) IR imaging, the thermal mismatch between IR photodetectors and silicon readout circuits will inevitably lead to the degradation of the device performance. An up-conversion IR photodetector, which converts IR photons to short-wavelength photons for Si-CCD-based imaging, can avoid thermal mismatch caused by hybridization with silicon readout circuits, resulting in a low-cost way for large array IR imaging. The operation principle of the semiconductor up-conversion IR photodetector is based on electron transitions and carrier transportation in different functional sections including absorption section, transportation section and emission section, hence the carrier distribution in the device structure has a crucial influence on the device performance. In order to achieve low dark current, carriers are expected to be non-uniformly distributed in the up-conversion device structure. Designing and optimizing the carrier-blocking structure are usually the key issues to acquire inhomogeneous carrier distribution. In this paper, up-conversion infrared photodetectors with various hole-blocking structures are investigated both theoretically and experimentally. Firstly the carrier distributions are calculated by self-consistently solving the Schr?dinger equation, Poisson equation, current continuity equation and carrier rate equation. Then the influence of the carrierblocking structure on the device performance is analyzed by electroluminescence measurements on the corresponding epitaxial structures. According to the theoretical and experimental results, it is found that a 2-nm-thick AlAs barrier layer can block holes effectively without hampering the electron transportation, which is necessary for the up-conversion infrared photodetectors. However, other attempts to block holes, such as light n-doping in the transportation section or lowering the injection barrier, do not work well. In addition, the influences of the thickness and height of the blocking barrier and the operation temperature on the carrier distributions are also studied. When the thickness of the blocking barrier is less than 2 nm, the thicker or the higher is the barrier, the better is the blocking effect. However, when the thickness of the blocking barrier is larger than 2 nm, the blocking effect is not persistently enhanced with increasing thickness because the tunneling process is almost fully suppressed. Furthermore, with the same blocking barrier parameters, lowering the operation temperature can lead to better blocking effect. This work demonstrates the utilization and effect of carrier-blocking structures in semiconductor devices which deamnd an inhomogeneous carrier distribution.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2015
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  • 10
    Online Resource
    Online Resource
    Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences ; 2011
    In:  Acta Physica Sinica Vol. 60, No. 5 ( 2011), p. 050301-
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 60, No. 5 ( 2011), p. 050301-
    Abstract: A sine-Gordon soliton star model with the action of exotic matter and dark energy is studied in this article, the solutions of state equation and mass of star are calculated by using field equation. We found that the density and pressure of matter are connected with the soliton state and the mass of star. Moreover, star equilibrium and stability of dark energy are analyzed and discussed, the result shown that the state of soliton star interior exist in the form of mixed state.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2011
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