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  • Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences  (50)
  • 1
    Online Resource
    Online Resource
    Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences ; 2013
    In:  Acta Physica Sinica Vol. 62, No. 6 ( 2013), p. 066801-
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 62, No. 6 ( 2013), p. 066801-
    Abstract: In the present paper, we synthesize CdSe quantum dots (QDs) that are stabilized by thioglycolic acid according to the water-phase synthesis. The X-ray diffraction and HRTEM results confirm that the samples prepared each possess a sphalerite structure. The EDS and FT-IR spectra of the samples show that a core-shell structure is formed between the CdSe nanoparticles and the ligand. The fine band structures and the characteristics of the surface states in a connection with the structures are identified by the surface photovoltage (SPV) spectrum of the samples. Two SPV response peaks, located at 475 nm (2.61 eV) and 400 nm (3.1 eV), are closely related to the band-band transitions of the core-CdSe and the shell-CdS, respectively; the SPV response at 370 nm (3.35 eV) is correlated with the n → π* transition between the hydroxyl and sulfydryl (or hydroxyl). It is because of an obvious quantum size effect of the samples that both PL line broadens and SPV response intensity increases with the decrease of the grain size of the sample. The change trend of the surface photoacoustic signal intensity is contrary to that of the SPV response intensity of the samples synthesized at varying pH. Moreover, the fine band structures at surfaces and grain boundaries of CdSe QDs prepared are probed by the SPV spectra of the samples at varying pH values. The relationship between the grain size and the photo-generated carrier transport behavior is discussed according to the detected EFISPV results of the QDs.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2013
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  • 2
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 55, No. 9 ( 2006), p. 4602-
    Abstract: The application of diffractive surface in the bifocal optical system is investigated by taking the advantage of the negative dispersion and the arbitrary phase modulation characteristics of binary elements, an analysis on the zoom equation is made and a sample design is presented. It is shown that good imaging quality can be achieved with the implementation of only four Germanium lenses. When the focal length of the system is 80 mm and the F-number is 0.8, the longitudinal aberration is less than 72 μm, the modulation transfer function (MTF) of 10 lp/mm is greater than 0.8 ;when the focal length is 160 mm and the F-number is 1.6, the longitudinal aberration is less than 35 μm, MTF of 10 lp/mm is greater than 0.7.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2006
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  • 3
    Online Resource
    Online Resource
    Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences ; 2021
    In:  Acta Physica Sinica Vol. 70, No. 8 ( 2021), p. 082901-
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 70, No. 8 ( 2021), p. 082901-
    Abstract: At present, there exist few proton-beam terminals for the detector calibration in the world. Meanwhile, most of these terminals provide monoenergetic protons. Back-n white neutron source from China Spallation Neutron Source(CSNS) was put into operation in 2018. Based on the white neutron flux ranging from 0.5 eV to 200 MeV from the CSNS Back-n white neutron source, continuous-energy protons involved in a wide energy spectrum can be acquired from the 〈sup〉1〈/sup〉H(n, el) reaction. Adopting this method, a new research platform for researches such as proton calibration is realized at CSNS. As hydrogen exists as gas at normal temperature and pressure, in the selecting of the proton-converting target, the hydrogen-rich compounds are preferential considered. Considering the reaction cross sections of the 〈sup〉1〈/sup〉H(n, el), 〈sup〉12〈/sup〉C(n, p)〈sup〉12〈/sup〉B, 〈sup〉12〈/sup〉C(n, d)〈sup〉11〈/sup〉B, 〈sup〉12〈/sup〉C(n, t)〈sup〉10〈/sup〉B, 〈sup〉12〈/sup〉C(n, 〈sup〉3〈/sup〉He)〈sup〉10〈/sup〉Be, 〈sup〉12〈/sup〉C(n, α)〈sup〉9〈/sup〉Be and 〈sup〉1〈/sup〉H(n, γ)〈sup〉2〈/sup〉H, polyethylene and polypropylene are suitable for serving as targets in this research. Based on a 3U PXIe, digitizers with 1 GSps sampling rate and 12 bit resolution are utilized to digitize and record the output signals of telescopes. The time and amplitude information of each signal are extracted from its recorded waveform. Proton fluxes can be calculated by using the neutron energy spectrum and the cross section of the 〈sup〉1〈/sup〉H(n, el) reaction. Using the γ-flash event as the starting time of the time-of-flight (TOF) and the time information of signal in detector as the stopping time, the kinematic energy of each secondary proton can be deduced from the TOF and the angle of the detector. A calibration experiment on three charged particle telescopes, with each telescope consisting of a silicon detector and a CsI(Tl) detector, is carried out on this research platform. The readout methods of the CsI(Tl) detectors in these three telescopes are different. In the calibration experiment, Δ〈i〉E-〈/i〉〈i〉E〈/i〉 two-dimensional spectra and amplitude-〈i〉E〈/i〉〈sub〉p〈/sub〉 two-dimensional spectra of these telescopes are obtained. Through comparing these particle identification spectra, the SiPM is chosen as the signal readout method for CsI(Tl) detectors in the charged particle telescopes. These researches provide experimental evidence for the construction of the charged particle telescope at Back-n, and also illustrate the feasibility of wide-energy spectrum proton calibration based on the Back-n white neutron source.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2021
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  • 4
    Online Resource
    Online Resource
    Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences ; 2021
    In:  Acta Physica Sinica Vol. 70, No. 22 ( 2021), p. 222801-
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 70, No. 22 ( 2021), p. 222801-
    Abstract: The data of neutron capture cross section are very important for the research of nuclear astrophysics, advanced nuclear energy development. Owing to the limitation of neutron source and detector, the experimental data of neutron capture cross section in an energy range of 1 eV–10 keV were almost blank in China. The first Chinese gamma-ray total absorption facility has been constructed in the key laboratory of nuclear data at China institute of atomic energy, which consists of 40 BaF〈sub〉2〈/sub〉 detector units. The BaF〈sub〉2〈/sub〉 crystal shell with a thickness of 15 cm and an inner radius of 10 cm covers 95.2% of the solid angle. On-line measurement method of neutron capture reaction cross section is established on the back-streaming white neutron source of China spallation neutron source by using the upgraded facility. The cross section of 〈sup〉197〈/sup〉Au neutron capture reaction is measured for the first time under the experimental condition of irregular 30 mm neutron beam spot. The measured position of resonance peak is well consistent with the relevant data of ENDF evaluation database, which verifies the reliability of the measurement device and measurement technology, and thus laying the foundation for the acquisition of high precision cross section in future.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2021
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  • 5
    Online Resource
    Online Resource
    Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences ; 2024
    In:  Acta Physica Sinica Vol. 73, No. 7 ( 2024), p. 072801-
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 73, No. 7 ( 2024), p. 072801-
    Abstract: Neutron capture reaction is one of the neutron reactions and plays an important role in using reactor control rods and shell materials, designing nuclear device structures, and studying nuclear astrophysics S processes and element origins. The 4π BaF 〈 sub 〉 2 〈 /sub 〉 detection device has advantages such as high time resolution, low neutron sensitivity, and high detection efficiency, thus making it suitable for measuring neutron radiation capture reaction cross-section data. In order to fill the gap in our neutron capture reaction data in the keV energy range and improve their accuracy, the Key Laboratory of Nuclear Data at the Chinese Institute of Atomic Energy (CIAE) has established a Gamma Total Absorption Facility (GTAF), which consists of 28 hexagonal BaF 〈 sub 〉 2 〈 /sub 〉 crystals and 12 pentagonal BaF 〈 sub 〉 2 〈 /sub 〉 crystals to form a spherical shell with an external diameter of 25 cm and an internal diameter of 10 cm, covering 95.2% of the solid angles. The Back-n beam line of the Chinese Spallation Neutron Source (CSNS) is a back-streaming white beam line that covers neutron energy ranging from a few eV to several hundred MeV, making it suitable for measuring neutron capture cross-sections. The reaction cross-section data of 〈 sup 〉 197 〈 /sup 〉 Au is measured by using GTAF on the Back-n beam line. The measurement data are preliminarily background deducted through energy screening, PSD method, and crystal multiplicity screening. Subsequently, the background is analyzed and deducted based on the measurement data of 〈 sup 〉 nat 〈 /sup 〉 C and empty samples, and the yield of 〈 sup 〉 197 〈 /sup 〉 Au capture reaction is obtained. Resonance parameters are a set of parameters extracted from experimental data to describe the resonance curve, which can eliminate the influence of experimental conditions on resonance data and are more important than the cross-section obtained from experiments. The resonance energy, neutron resonance width, and gamma resonance width parameters of 〈 sup 〉 197 〈 /sup 〉 Au at 1–100 eV are fitted by using the SAMMY program. From the comparison between the resonance curves obtained from experimental measurements and the resonance parameters obtained from fitting with the ENDF/B-VIII.0 database, it can follow that the experimental measurement results are in good agreement with the database, nevertheless, there exist some differences in the resonance parameter, which may be due to the GTAF energy resolution, Back-n neutron spectrum measurement accuracy, and the experimental background deduction method. Our next work is to identify the sources of difference.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2024
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  • 6
    Online Resource
    Online Resource
    Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences ; 2020
    In:  Acta Physica Sinica Vol. 69, No. 17 ( 2020), p. 172901-
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 69, No. 17 ( 2020), p. 172901-
    Abstract: The back-streaming neutron beam line (Back-n) was built in the beginning of 2018, which is part of the China Spallation Neutron Source (CSNS). The Back-n is the first white neutron beam line in China, and its main application is for nuclear data measurement. For most of neutron-induced nuclear reaction measurements based on white neutron facilities, the beam of gamma rays accompanied with neutron beam is one of the most important experimental backgrounds. The back streaming neutron beam is transported directly from the spallation target to the experimental station without any moderator or shielding, the flux of the in-beam gamma rays in the experimental station is much larger than those of these facilities with neutron moderator and shielding. Therefore, it is necessary to consider the influence of in-beam gamma rays on the experimental results. Studies of the in-beam gamma rays are carried out at the back-n. Monte-Carlo simulation is employed to obtain the energy distribution and the time structure of the in-beam gamma rays. According to the simulation results, when the neutron flight time is longer than 1.0 μs the energy distribution of the in-beam gamma rays does not vary with flight time. Therefore, the time structure of these gamma rays can be measured without the correction of the detection efficiency. In this work, the time structure of the in-beam gamma rays in the low neutron energy region is measured by both direct and indirect methods. In the direct measurement, a 〈sup〉6〈/sup〉Li loaded ZnS(Ag) scintillator is located on the neutron beam line and the time of flight method is used to determine the time structure of neutrons and gamma rays. The gamma rays are separated from neutrons with pulse-shape discrimination. The black filter method is used to verify the particle discrimination results. In the indirect measurement, the C〈sub〉6〈/sub〉D〈sub〉6〈/sub〉 scintillation detectors are used to measure the gamma rays scattered off a Pb sample on the way of the neutron beam. The time structure of the in-beam gamma rays is derived from that of the scattered gamma rays. The experimental results are in good agreement with the simulations with the time-of-flight between 12 μs and 2.0 ms. Besides, according to the simulation results, the intensity of the in-beam gamma rays is 1.21 × 10〈sup〉6〈/sup〉 s〈sup〉–1〈/sup〉·cm〈sup〉–2〈/sup〉 in the center of the experimental station 2 of Back-n, which is 76.5 m away from the spallation target of CSNS.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2020
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  • 7
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 69, No. 22 ( 2020), p. 228101-
    Abstract: Terahertz (THz) has the characteristics of non ionization, penetration, water absorption, high resolution, etc. It has shown an important application prospect in many fields, such as non-destructive testing, imaging and communication. However, THz is in the transition frequency band ranges from macro-electronics to micro-photonics, so, it belongs to the interdisciplinary field, forming the “terahertz gap” in electromagnetic wave. In recent years, with the continuous development and improvement of THz radiation source and detection technology, the THz modulation technology has gradually aroused the interest of researchers. Metamaterials with many properties that natural materials do not possess provide a common way to control THz. The two-dimensional structure of a metamaterial is called a metasurface. The coding metasurface encodes the phase digitally so that the electromagnetic wave can be regulated. It is proposed that it is first in the microwave band and then extended to the THz band. In the microwave band, the number, direction and amplitude of the far-field beams can be changed dynamically by programming, which is connected with the integrated circuit such as FPGA by using diodes, but due to the limitation of diode size and micro-nano manufacturing technology, the programmable metasurface in microwave band cannot be well used in THz band. In order to improve the flexibility of THz coding metasurface, in this paper we choose the phase change material vanadium dioxide (VO〈sub〉2〈/sub〉) to active modulation coding metasurface. In this paper, we analyze the VO〈sub〉2〈/sub〉’s insulating state before the phase transformation and metallic state after the phase transformation. Then designing an active control 1 bit coding metasurface by using the influence of the two states on the amplitude and phase of the unit structure, which is composed of VO〈sub〉2〈/sub〉, polyimide and aluminum, can not only realize the basic function of coding metasurface adjusting the electromagnetic wave beams, but alsoimplement the switching of two kinds of far-field beams at 1.1 THz for the same coding sequence by thermal stimulated VO〈sub〉2〈/sub〉. The coding metasurface also realizes the switching between two near-field focal points at 1.1 THz for the same coding sequence. Based on the effect of VO〈sub〉2〈/sub〉 on the phase, this coding metasurface provides a new way to adjust and control the THz wave flexibly, and will have a great application prospect in THz transmission, imaging and communication.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2020
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  • 8
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 72, No. 16 ( 2023), p. 168101-
    Abstract: 〈sec〉Recently, the power conversion efficiency (PCE) of organic-inorganic hybrid perovskite solar cells has been enhanced rapidly from 3.8% to 25.8%, which is a top research topic in the field of photovoltaic power generation. However, the preparation of the hybrid perovskite solar cells has high environmental requirements, and the absorber layer is easily caused by the environmental influence and decomposition, resulting in the degradation of device performance. The all-inorganic CsPbBr〈sub〉3〈/sub〉 perovskite material has good stability, can be prepared directly in air, and is more economical, showing great potential applications. However, the PCE of all-inorganic CsPbBr〈sub〉3〈/sub〉 perovskite solar cells is not high, and at this stage, there is still much room for exploring high-quality controllable preparation of CsPbBr〈sub〉3〈/sub〉 films. In this paper, we aim to prepare efficient and stable CsPbBr〈sub〉3〈/sub〉 perovskite solar cells with additive engineering.〈/sec〉〈sec〉Polymer is one of the most effective additives in perovskite solar cells. The use of polymer additive in perovskite layer can improve the shape-form, structure, and band gap of the film, thus improving the quality of perovskite film. Polyvinylidene fluoride (PVDF) is a cheap polymer with hydrophobic F ions and long flexible polymer chains, and can be used to prepare efficient and stable perovskite solar cells.〈/sec〉〈sec〉In this paper, CsPbBr〈sub〉3〈/sub〉 perovskite films are prepared by multi-part spin-coating method. PVDF with enriched hydrophobic F is added into the PbBr〈sub〉2〈/sub〉 precursor solution as an additive to adjust the crystalline quality of the perovskite film, and the effects of PVDF on the growth process and device performance of the perovskite film are systematically studied. The results show that the PVDF can be used as a template to promote the growth of perovskite crystals, improve the crystal structure and film shape, thus reducing the defect density and charge recombination, and increasing the PCE of the device to 8.17%. The original efficiency of more than 90% can be maintained after 1400 h of storage under unencapsulated condition. Finally, high-efficiency, stable and low-cost CsPbBr〈sub〉3〈/sub〉 perovskite solar cells are obtained, which is important in further expanding the optimized design ideas of CsPbBr〈sub〉3〈/sub〉 perovskite solar cells. The PVDF can form hydrogen bonds with perovskite or interact with lead ions to improve the structural stability of perovskite, and the F ions in PVDF can improve the moisture stability of perovskite layers.〈/sec〉
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2023
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  • 9
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 60, No. 9 ( 2011), p. 093201-
    Abstract: Absolute photoabsorption spectrum of CO molecule in the region 14—20 eV(620—890 Å) is measured using synchrotron radiation and multi-stage photoionization chamber, and its ionization energy is obtained. According to the absorption spectrum of CO and theoretical calculation, the Rydberg series converging to the Χ2Σ+, Α2Π, and B2Σ+ states of CO+ are assigned separately. Rydberg series assigned before are extended, Rydberg series converging to the Χ2Σ+ (ν+=2 and 3) of CO+, and n=2 (the real value of n is 3) progressions of the series converging to the Α2Π state of CO+ are identified. At the same time, the absorption spectrum of CO in the region 17.0—17.5 eV (710—730 Å) is also discussed deeply.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2011
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  • 10
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 69, No. 7 ( 2020), p. 077401-
    Abstract: YBa〈sub〉2〈/sub〉Cu〈sub〉3〈/sub〉O〈sub〉7−〈i〉δ〈/i〉〈/sub〉 (YBCO) high temperature superconductor materials have many promising applications in energy, transportation and so on. Nonetheless, the application of YBCO in high magnetic field was limited because of low critical current. One-dimensional latent tracks produced by swift heavy ions irradiation can be effective pinning centers, thus enhancing superconductivity in external field. YBCO high temperature superconducting films were irradiated with 1.9 GeV Ta ions at room temperature and vacuum condition. Structure damages in irradiated samples were characterized by transmission electron microscopy (TEM). Continuous amorphous latent tracks, with diameter from 5 nm to 15 nm, throughout the whole superconducting layer can be observed from TEM images. Physical property measurement system (PPMS) was used to measure superconducting properties of samples before and after irradiation. When irradiated at optimal fluence of 8 × 10〈sup〉10〈/sup〉 ions/cm〈sup〉2〈/sup〉, critical current reaches its maximum value and pinning force was twice of unirradiated sample, while critical temperature almost unchanged. The analysis of experimental results shows that latent tracks produced by swift heavy ions irradiation can enhance in-field current-carrying capability, without decreasing critical temperature. In the power-law regime 〈inline-formula〉〈tex-math id="M2"〉\begin{document}${J_c} \propto {B^{ - \alpha }}$\end{document}〈/tex-math〉〈alternatives〉〈graphic xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="7-20191914_M2.jpg"/〉〈graphic xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="7-20191914_M2.png"/〉〈/alternatives〉〈/inline-formula〉 values of 〈i〉ɑ〈/i〉 decreased with the increasing of fluence, indicating a weaker magnetic field dependence of critical current. 〈i〉ɑ〈/i〉 reaches its lowest value 0.375 when irradiated at a fluence of 5.0 × 10〈sup〉11〈/sup〉 ions/cm〈sup〉2〈/sup〉, corresponding to a lowest in-field 〈i〉J〈sub〉c〈/sub〉〈/i〉. This result may be a combination of increasing pinning centers and decreasing superconductor volumes that work together. Normalized pinning force 〈i〉f〈/i〉〈sub〉p〈/sub〉 = 〈i〉F〈/i〉〈sub〉p〈/sub〉/〈i〉F〈/i〉〈sub〉p,max〈/sub〉 of sample irradiated with different fluence as a function of magnetic field 〈i〉h〈/i〉 = 〈i〉H〈/i〉/〈i〉H〈/i〉〈sub〉max〈/sub〉 was analyzed using Higuchi model. Fitting results show that planar defects are main source of pinning when 〈i〉h〈/i〉 〉 1, independent of irradiation. Whereas, dominate pinning centers shifting from surface pinning to isotropic normal point pinning with increasing fluence when 〈i〉h〈/i〉 〈 1. Given that latent tracks produced by Ta ions irradiation act as strong anisotropic pinning centers, the reason of the dominate pinning centers change with increasing fluence remains to be further studied.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2020
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