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  • AIP Publishing  (3)
  • 1
    In: AIP Advances, AIP Publishing, Vol. 9, No. 10 ( 2019-10-01)
    Abstract: Utilizing the self-assembly method, we have successfully prepared a two-dimensional photonic crystal (PhC) of monolayer SiO2 spheres onto the Bismuth Germinate (Bi4Ge3O12, BGO) crystal and therefore supply another photonic crystal structure with the advantages of low-cost and large-area preparation to improve the light extraction efficiency of scintillator. A light extraction enhancement ratio up to 145.3% as compared the BGO coated by the PhC with the plain reference sample is observed and the underlying mechanism of scintillator light extraction is discussed in detail via a rigorous coupled-wave analysis calculation. The calculated transmission spectra and electric-field distribution exhibit the electric-field eigenmodes confined in SiO2 spheres resonating by the way of whispering gallery modes (WGMs) and becoming leaky modes due to the diffraction effect. Since almost no SiO2 nanospheres over the polystyrene spheres are immersed in preparation, we have demonstrated that the introduction of PhC structures using the SiO2 nanospheres onto the scintillator surface is an effective way to solve the light-trapping problem and therefore the design is very useful to be applied to the particle detection of radiation field.
    Type of Medium: Online Resource
    ISSN: 2158-3226
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2019
    detail.hit.zdb_id: 2583909-3
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  • 2
    In: AIP Advances, AIP Publishing, Vol. 10, No. 2 ( 2020-02-01)
    Abstract: A (Lu,Y)2SiO5:Ce (LYSO) crystal, as a heavy inorganic scintillator, is currently in high demand for various applications in the fields of particle detection. However, its high refractive index (n = 1.83) gives restriction on the measurements of rare events or weak particle flow, where high energy resolution is urgently required for detectors based on the crystal. Utilizing the electron beam lithography technique and the ion beam lithography method, we have successfully prepared a 2.0 × 2.0 mm2 large area two-dimensional photonic crystal (PhC) structure on the LYSO crystal surface. Compared with the plain reference sample, the optical measurements show a 53% enhancement of light extraction for the LYSO nanostructured surface, and the resulted improvement of energy resolution (full width at half maximum) is measured to be 43.8% by gaussian fittings to the energy spectra excited by the 241Am α source. With the advantage of high-resolution patterning, high thermal stability, and firm stickiness on the substrate, the present prescription of the PhC fabrication is still favorable for some special fields (e.g., homeland security and space exploration) though the writing process is extremely time consuming and expensive to use.
    Type of Medium: Online Resource
    ISSN: 2158-3226
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2020
    detail.hit.zdb_id: 2583909-3
    Location Call Number Limitation Availability
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  • 3
    In: AIP Advances, AIP Publishing, Vol. 11, No. 11 ( 2021-11-01)
    Abstract: All-inorganic CsPbBr3 perovskites exhibit great potential in optoelectronic application due to their outstanding physical properties for optoelectronics. However, the relatively low luminescence efficiency of the bulk CsPbBr3 crystal hampers its further application. Here, we report a facile method to enhance the optical efficiency of halide perovskite powder via doping the transition metal Ni ions. It is demonstrated that Ni doping results in the formation of the Cs(NiPb)Br3 alloy and also triggers the phase transition of CsPbBr3 from orthorhombic to cubic. Both the Cs(NiPb)Br3 alloy and cubic CsPbBr3 are found to contribute to the asymmetric photoluminescence (PL) spectra in the green-yellow light band. The splitting-peak fitting experiments for the overlapped PL spectrum based on the bi-Gaussian line model reveal that the Cs(NiPb)Br3 alloy dominates the contribution of the observed PL enhancement. The Ni2+ doping is also beneficial for optimizing the crystallinity of the CsPbBr3 perovskite, suppressing the nonradiative recombination and significantly enhancing the photoluminescence consequently. Our investigation provides a novel insight into the effect of environmentally friendly metal doping in perovskites.
    Type of Medium: Online Resource
    ISSN: 2158-3226
    Language: English
    Publisher: AIP Publishing
    Publication Date: 2021
    detail.hit.zdb_id: 2583909-3
    Location Call Number Limitation Availability
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