Note: Intro -- Preface -- Contents -- Part I FEM -- 1 Observations of Individual Cu-Phthalocyanine Molecules Deposited on Nano-Tips in the Field Emission Microscope -- Abstract -- 1…Introduction -- 2…Experimental Setup and Molecule Images -- 3…Current Voltage Emission Characteristics Through the Molecule -- 4…Computer Simulation of the Molecule Adsorption on the Nano-Tip Apex -- 5…Conclusion -- References -- 2 High Voltage STM Imaging of Single Copper Phthalocyanine -- Abstract -- 1…Introduction -- 2…Experiments and Results -- 3…Interpretation -- 4…Conclusion -- Acknowledgments -- References -- Part II STEM -- 3 Motional Analysis of a Single Organic Molecule by TEM Using Nanocarbon Materials: Scope of Atomic Level Imaging and Spectroscopy -- Abstract -- 1…Organic Single Molecule Versus Organic Crystal -- 2…Putting Molecules Inside Carbon Nanotubes: Method -- 3…What Influences Molecular Motions? -- 4…Characterizing the Structure with Atomic Resolution -- 5…Conclusion -- Acknowledgments -- References -- Part III Photo-Emission (PE) -- 4 Imaging Orbitals by Ionization or Electron Attachment: The Role of Dyson Orbitals -- Abstract -- 1…Introduction -- 2…Dyson Orbitals in Pentacene -- 3…Dyson Orbitals and Super Atomic Molecular Orbital States in C60 -- 4…Time-Dependent Dyson Orbitals -- 5…Conclusions -- Acknowledgments -- References -- Part IV LT-UHV-STM -- 5 Mapping the Electronic Resonances of Single Molecule STM Tunnel Junctions -- Abstract -- 1…Introduction -- 2…Pentacene/Au(111) -- 3…Cu-Phthalocyanine/Au(111) -- 4…Hexabenzocoronene/Au(111) -- 5…Conclusion -- Acknowledgments -- References -- 6 Manipulation and Spectroscopy of Individual Phthalocyanine Molecules on InAs(111)A with a Low-Temperature Scanning Tunneling Microscope -- Abstract -- 1…Introduction -- 2…Results and Discussion -- 2.1 Experimental Details -- 2.2 The Substrate Surface: InAs(111)A. , 2.3 Naphthalocyanine Molecules on InAs(111)A -- 2.4 Free-Base Phthalocyanine Molecules on InAs(111)A -- 3…Conclusions -- Acknowledgments -- References -- 7 Electronic Structure and Properties of Graphen Nanoribbons: Zigzag and Armchair Edges -- Abstract -- 1…Introduction -- 2…Experiment and Results -- 3…dI/dV Spectroscopy -- 4…dI/dV Mapping -- 5…Conclusion -- Acknowledgments -- References -- 8 Imaging and Manipulation of Molecular Electronic States on Metal Surfaces with Scanning Tunneling Microscopy -- Abstract -- 1…Introduction -- 2…Formation of a Metal--Ligand Bond with Cu and PVBA -- 3…Actuated Transitory Metal--Ligand Bond as Tunable Electromechanical Switch -- 4…Summary -- Acknowledgments -- References -- 9 SPM Imaging of Trinaphthylene Molecular States on a Hydrogen Passivated Ge(001) Surface -- Abstract -- 1…Introduction -- 2…Ge(001) Surface Preparation and Molecule Deposition -- 3…Molecular State Imaging of Heptastarphene Molecules Anchored on the Ge(001):H Surface with LT-STM -- 4…3D Molecular State Probing with Simultaneous Tunneling Current and Force Imaging with a qPlus Sensor -- 5…Concluding Remarks -- Acknowledgments -- References -- Part V STM Theory and Image Interpretation -- 10 Simulations of Constant Current STM Images of Open-Shell Systems -- Abstract -- 1…Introduction -- 2…Simulation of Constant Current STM Images -- 3…Beyond the Perturbative Approach -- 4…A NCA Approach to the Kondo Effect -- 4.1 The Anderson Hamiltonian -- 4.2 The Noncrossing Approximation -- 5…Summary and Conclusions -- Acknowledgments -- References -- 11 Electronic Transmission Through a Single Impurity in a Multi-configuration Scattering Matrix Approach -- Abstract -- 1…Introduction -- 2…The Multi-Configuration Basis Set -- 3…Calculation of the Scattering Matrix on a Multi-Configuration Basis Set. , 4…Application to a Weakly Coupled Two-States Molecule Filled Up with Two Electrons -- 4.1 The Simple U=0 eV Non-interacting Case -- 4.2 A Large U = 4 eV Electron--Electron Interaction Case -- 5…Application to a Weakly Coupled Four-States Molecule with a Four Electrons Closed Shell Structure -- 6…Conclusion -- Appendix A: Parameters and Calculation Method for the Electron--Electron Interactions -- Appendix B: Some Useful Relations -- References -- 12 Electron Transport Through a Molecular Junction Using a Multi-configurational Description -- Abstract -- 1…Introduction -- 2…Theoretical Approach -- 2.1 Isolated Fragment Low-Energy Spectroscopy -- 2.2 Transport Through Magnetic Molecular Devices -- 3…Impact of the Electronic Structure of the Fragment -- 3.1 Influence of the Coulomb On-Site Repulsion U -- 3.2 Influence of the Multideterminantal Structure of the Wave-Function -- 4…Impact of the Spin-Polarization of the Electrodes -- 4.1 Parallel Magnetization -- 4.2 Antiparallel Magnetization -- 4.3 Magnetoresistance -- 4.4 Impact of the Multideterminantal Approach -- 5…Conclusion -- A.x(118). A. Coefficients -- A.x(118). B. Cancellation of Coefficients in {\bf i }_{\rm{ tot }} and {\bf P }^{{\rm{ i }}} for a Parallel Magnetization -- A.x(118). 8…C. Origin of the Quadratic Term in the Total Current for an Antiparallel Situation -- References -- 13 Visualizing Electron Correlation in Molecules Using a Scanning Tunneling Microscope: Theory and Ab Initio Prediction -- Abstract -- 1…Introduction -- 2…Many-Body Theory of STS with an Ideal Tip -- 3…Ab Initio Evaluation of the Quasiparticle Wave Function -- 4…Predicted STS Images of Copper-(deh-salen) -- 5…Conclusions -- Acknowledgments -- References -- Part VI NC-AFM -- 14 Submolecular Resolution Imaging of C_{60}: From Orbital Density to Bond Order -- Abstract -- 1…Introduction -- 2…Do We See Orbitals?. , 3…STM Observations of Intramolecular Contrast in C60 -- 4…Probing the Probe -- 5…Imaging Atoms and Bonds in C_{60} -- 6…Conclusions -- Acknowledgments -- References.

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