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  • 1
    Publication Date: 2013-01-03
    Description: [1]  The impact of changes in the abundance of greenhouse gases (GHGs) on the evolution of tropospheric ozone (O 3 ) between 1960 and 2005 is examined using a version of the Goddard Earth Observing System chemistry-climate model (GEOS CCM) with a combined troposphere-stratosphere chemical mechanism. Simulations are performed to isolate the relative role of increases in methane (CH 4 ) and stratospheric ozone depleting substances (ODSs) on tropospheric O 3 . The 1960 to 2005 increases in GHGs (CO 2 , N 2 O, CH 4 , and ODSs) cause increases of around 1–8% in zonal-mean tropospheric O 3 in the tropics and northern extratropics, but decreases of 2–4% in most of the southern extratropics. These O 3 changes are due primarily to increases in CH 4 and ODSs, which cause changes of comparable magnitude but opposite sign. The CH 4 -related increases in O 3 are similar in each hemisphere (∼6%), but the ODS-related decreases in the southern extratropics are much larger than in northern extratropics (10% compared to 2%). This results in an interhemispheric difference in the sign of past O 3 change. Increases in the other GHGs (CO 2 and N 2 O) and SSTs have only a small impact on the total burden over this period, but do cause zonal variations in the sign of changes in tropical O 3 that are coupled to changes in vertical velocities and water vapor.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
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  • 2
    Publication Date: 2013-03-22
    Description: Based on an accurate atmospheric radiative transfer scheme, a parametrization of instantaneous global horizontal irradiance (GHI) at the Earth's surface has been developed. The scheme is named SUNFLUX and this article describes the development of the scheme for clear-sky conditions. The work dealing with clouds has been published in a separate article. Unlike traditional methods, this study applies the band model idea used in radiative transfer theory to the development of the surface radiation scheme and, importantly, includes absorption and scattering in the parametrization. Thus the scheme is more accurate compared with those using simple empirical approaches and may be applied to any site without being tuned for local conditions. The parametrization of aerosol transmittance and albedo developed by Kokhanovsky et al. is adopted to account for the effects of aerosols. All variables used in the scheme are available in climate models or from satellite observations. Therefore, the parametrization can be used to determine the GHI at the surface under clear-sky conditions The scheme is evaluated using observations obtained from three US Atmospheric Radiation Measurement (ARM) stations and three stations on the Tibetan Plateau, and the results demonstrate that the scheme is accurate. The relative mean bias difference is less than 4.3% and the relative root-mean-squared difference is less than 0.09%. Copyright © 2013 Royal Meteorological Society
    Print ISSN: 0035-9009
    Electronic ISSN: 1477-870X
    Topics: Geography , Physics
    Published by Wiley-Blackwell
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