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  • Song, Haoqiang  (3)
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Subjects(RVK)
  • 1
    Online Resource
    Online Resource
    Solid‐state Fluorescence from Carbon Dots Widely Tunable from Blue to Deep Red through Surface Ligand Modulation
    Wiley ; 2023
    In:  Angewandte Chemie International Edition Vol. 62, No. 12 ( 2023-03-13)
    Details
    In: Angewandte Chemie International Edition, Wiley, Vol. 62, No. 12 ( 2023-03-13)
    Abstract: Carbon dots (CDs) find widespread attention due to their remarkable fluorescent and electronic properties. However, aggregation‐caused quenching currently limits the application of CDs in colored displays. The construction of CDs with color‐tunable solid‐state fluorescence (SSF) is rarely reported, since the preparation of SSF CDs is technically challenging. Herein, through surface ligand modulation, SSF CDs with an emission‐color span of almost 300 nm (from blue to deep red) were obtained. In‐depth structure‐property studies reveal that intra‐ and inter‐molecular hydrogen‐bonding inside SSF CDs provokes the emission properties in the aggregated state. Photodynamic characterizations demonstrate emission wavelengths can be switched smoothly by deliberately altering conjugation ability between substituent ligands and CDs core. Three‐dimensional printing patterning is used to create a range of emissive objects, demonstrating the commercial potential for use in optical lamps.
    Type of Medium: Online Resource
    ISSN: 1433-7851 , 1521-3773
    URL: Issue
    URL: Article
    DOI: 10.1002/anie.v62.12
    DOI: 10.1002/anie.202217822
    RVK:
    VA 2100
    Language: English
    Publisher: Wiley
    Publication Date: 2023
    detail.hit.zdb_id: 2011836-3
    detail.hit.zdb_id: 123227-7
    Location Call Number Limitation Availability
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    Online Resource
  • 2
    Online Resource
    Online Resource
    Acid‐Triggered Aggregation of Carbon Dots Shifted Their Emission to Give Unexpected Deep‐Red Lasing
    Wiley ; 2023
    In:  Advanced Functional Materials Vol. 33, No. 34 ( 2023-08)
    Details
    In: Advanced Functional Materials, Wiley, Vol. 33, No. 34 ( 2023-08)
    Abstract: It is challenging to realize ultra‐pH‐responsive fluorescent carbon dots (CDs), especially reversibly adjustable multichromatic emission covering a broad wavelength range including deep‐red lasing. This study reports a one‐step solvothermal treatment of pyrogallol to obtain brilliant CDs with a substantial bathochromic shift (from blue to dark red emission) induced by pH changes. The CDs show an excellent reversible pH response: simple acid treatment instantaneously shifts their initial green emission by 140 nm to a deep‐red emission with high‐color‐purity and enhances brightness, subsequent alkali addition returned the green emission, suggesting smooth and reversible regulation of fluorescence. Detailed components analyses, morphology tracking, and photodynamic studies demonstrate the discrete, reversible shift of emission derived from structural transformations, which include protonation of the CDs and their subsequent assembly and partial aggregation triggered by hydrogen bonding. The abundant H‐bonds crosslink the network of CDs, ultimately raising the quantum yield from 11.3% to 16.0%. Furthermore, the aggregated CDs crystallized into sheet‐like structures that acted as a resonant cavity for lasing show excellent gain ability and lead to strong deep‐red lasing. This study draws together pH regulation, the effects of CD's assembly, and their lasing emission to demonstrate significant potential for the development of versatile CDs.
    Type of Medium: Online Resource
    ISSN: 1616-301X , 1616-3028
    URL: Issue
    URL: Article
    DOI: 10.1002/adfm.v33.34
    DOI: 10.1002/adfm.202303363
    Language: English
    Publisher: Wiley
    Publication Date: 2023
    detail.hit.zdb_id: 2029061-5
    detail.hit.zdb_id: 2039420-2
    SSG: 11
    Location Call Number Limitation Availability
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    Online Resource
  • 3
    Online Resource
    Online Resource
    Solid‐state Fluorescence from Carbon Dots Widely Tunable from Blue to Deep Red through Surface Ligand Modulation
    Wiley ; 2023
    In:  Angewandte Chemie Vol. 135, No. 12 ( 2023-03-13)
    Details
    In: Angewandte Chemie, Wiley, Vol. 135, No. 12 ( 2023-03-13)
    Abstract: Carbon dots (CDs) find widespread attention due to their remarkable fluorescent and electronic properties. However, aggregation‐caused quenching currently limits the application of CDs in colored displays. The construction of CDs with color‐tunable solid‐state fluorescence (SSF) is rarely reported, since the preparation of SSF CDs is technically challenging. Herein, through surface ligand modulation, SSF CDs with an emission‐color span of almost 300 nm (from blue to deep red) were obtained. In‐depth structure‐property studies reveal that intra‐ and inter‐molecular hydrogen‐bonding inside SSF CDs provokes the emission properties in the aggregated state. Photodynamic characterizations demonstrate emission wavelengths can be switched smoothly by deliberately altering conjugation ability between substituent ligands and CDs core. Three‐dimensional printing patterning is used to create a range of emissive objects, demonstrating the commercial potential for use in optical lamps.
    Type of Medium: Online Resource
    ISSN: 0044-8249 , 1521-3757
    URL: Issue
    URL: Article
    DOI: 10.1002/ange.v135.12
    DOI: 10.1002/ange.202217822
    RVK:
    VA 2100
    RVK:
    VN 5020
    Language: English
    Publisher: Wiley
    Publication Date: 2023
    detail.hit.zdb_id: 505868-5
    detail.hit.zdb_id: 506609-8
    detail.hit.zdb_id: 514305-6
    detail.hit.zdb_id: 505872-7
    detail.hit.zdb_id: 1479266-7
    detail.hit.zdb_id: 505867-3
    detail.hit.zdb_id: 506259-7
    Location Call Number Limitation Availability
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    Online Resource
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