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  • Copernicus GmbH  (2)
  • Huang, Wenjing  (2)
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  • Copernicus GmbH  (2)
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  • 1
    In: Atmospheric Chemistry and Physics, Copernicus GmbH, Vol. 21, No. 13 ( 2021-07-06), p. 10015-10037
    Abstract: Abstract. The atmospheric carbon dioxide (CO2) mixing ratio and its carbon isotope (δ13C-CO2) composition contain important CO2 sink and source information spanning from ecosystem to global scales. The observation and simulation for both CO2 and δ13C-CO2 can be used to constrain regional emissions and better understand the anthropogenic and natural mechanisms that control δ13C-CO2 variations. Such work remains rare for urban environments, especially megacities. Here, we used near-continuous CO2 and δ13C-CO2 measurements, from September 2013 to August 2015, and inverse modeling to constrain the CO2 budget and investigate the main factors that dominated δ13C-CO2 variations for the Yangtze River delta (YRD) region, one of the largest anthropogenic CO2 hotspots and densely populated regions in China. We used the WRF-STILT model framework with category-specified EDGAR v4.3.2 CO2 inventories to simulate hourly CO2 mixing ratios and δ13C-CO2, evaluated these simulations with observations, and constrained the total anthropogenic CO2 emission. We show that (1) top-down and bottom-up estimates of anthropogenic CO2 emissions agreed well (bias 〈 6 %) on an annual basis, (2) the WRF-STILT model can generally reproduce the observed diel and seasonal atmospheric δ13C-CO2 variations, and (3) anthropogenic CO2 emissions played a much larger role than ecosystems in controlling the δ13C-CO2 seasonality. When excluding ecosystem respiration and photosynthetic discrimination in the YRD area, δ13C-CO2 seasonality increased from 1.53 ‰ to 1.66 ‰. (4) Atmospheric transport processes in summer amplified the cement CO2 enhancement proportions in the YRD area, which dominated monthly δs (the mixture of δ13C-CO2 from all regional end-members) variations. These findings show that the combination of long-term atmospheric carbon isotope observations and inverse modeling can provide a powerful constraint on the carbon cycle of these complex megacities.
    Type of Medium: Online Resource
    ISSN: 1680-7324
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2021
    detail.hit.zdb_id: 2092549-9
    detail.hit.zdb_id: 2069847-1
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  • 2
    In: Earth System Science Data, Copernicus GmbH, Vol. 12, No. 4 ( 2020-10-31), p. 2635-2645
    Abstract: Abstract. Eddy covariance data are widely used for the investigation of surface–air interactions. Although numerous datasets exist in public depositories for land ecosystems, few research groups have released eddy covariance data collected over lakes. In this paper, we describe a dataset from the Lake Taihu eddy flux network, a network consisting of seven lake sites and one land site. Lake Taihu is the third-largest freshwater lake (area of 2400 km2) in China, under the influence of subtropical climate. The dataset spans the period from June 2010 to December 2018. Data variables are saved as half-hourly averages and include micrometeorology (air temperature, humidity, wind speed, wind direction, rainfall, and water or soil temperature profile), the four components of surface radiation balance, friction velocity, and sensible and latent heat fluxes. Except for rainfall and wind direction, all other variables are gap-filled, with each data point marked by a quality flag. Several areas of research can potentially benefit from the publication of this dataset, including evaluation of mesoscale weather forecast models, development of lake–air flux parameterizations, investigation of climatic controls on lake evaporation, validation of remote-sensing surface data products and global synthesis on lake–air interactions. The dataset is publicly available at https://yncenter.sites.yale.edu/data-access (last access: 24 October 2020) and from the Harvard Dataverse (https://doi.org/10.7910/DVN/HEWCWM; Zhang et al., 2020).
    Type of Medium: Online Resource
    ISSN: 1866-3516
    Language: English
    Publisher: Copernicus GmbH
    Publication Date: 2020
    detail.hit.zdb_id: 2475469-9
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