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  • 1
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 66, No. 24 ( 2017), p. 244211-
    Abstract: The ground-state structural optimization and the terahertz spectrum calculation of an organic electro-optical crystal of 4-N, N-dimethylamino-4'-N'-methyl-stilbazolium tosylate (DAST) are performed using dispersion-corrected density functional theory (DFT-D2). DAST consists of an organic pyridinium salt (cation), one of the most efficient non-linear optical active chromophores and a sulfonate (anion) for enhancing the stability of the noncentrosymmetric macroscopic crystal. Such an organic crystalline salt DAST exhibits highly electro-optical and nonlinear optical coefficients, and it is an efficient emitter of THz pulses. The steady ground-state structure of DAST is obtained by a step-by-step optimization method with gradually increasing the convergence accuracy. The calculated terahertz spectra in 0-4 THz are in good agreement with experimental measurements, implying the reasonability of DFT-D2 method. Moreover, the vibration displacement vector diagrams for DAST molecular structure are obtained using Cambridge sequential total energy package animation simulation function. The results indicate that the phonon modes of DAST crystal at 1.12 THz are attributed to the optical phonon modes of the anion and cation, and DAST cation (organic pyridinium salt) and anion (sulfonate) undergo translational vibrations in their respective (benzene ring) plane. In contrast the vibrations at 1.46 THz and 1.54 THz are mainly related to the vibration of the sulfonate, among which 1.46 THz vibration is caused by the rotation of the sulfonate along the a axis, while 1.54 THz is due to the motion of the whole sulfonate along the c axis. And the vibrations at 2.63 THz and 3.16 THz originate from the torsional vibrations of cations and the rotation of anions, respectively. The results presented in this work clearly illustrate the contributions of the anion and cation of DAST in the THz responses. The mode assignments provide important reference and guidance for further synthesis of new DAST derivatives with larger electro-optical coefficients. In particular, our results suggest that DFT method is a powerful theoretical tool for studying the THz photonics and it is helpful not only for better understanding the mechanisms of the THz responses of organic electro-optic crystals, but also for controlling their performances.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2017
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  • 2
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 64, No. 4 ( 2015), p. 045202-
    Abstract: The emission spectra from a flame-breakdown atmospheric pressure plasma generated by a nanosecond pulsed 1064 nm beam of Nd:YAG laser are investigated by using a PI-MAX-II intensified charge coupled device. The emission lines of the main elements, such as carbon, hydrogen, oxygen and nitrogen are identified according to the national institute of standards and technology database of atomic emission. It is found that the relative intensities of the atomic emission lines are different from each other under different combustion conditions by making a comparative analysis of the spectra of laser induced breakdown air plasma, alcohol burner flame plasma, and alcohol blast burner flame plasma. The obtained results in this work provide an experimental basis for applying the laser-induced breakdown technology to the combustion diagnostics, and have an important reference and significance for analyzing the characteristics of hydrocarbon fuel combusting in air.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2015
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  • 3
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 66, No. 12 ( 2017), p. 120502-
    Abstract: The researches on higher-order coherence and quantum statistics of light field are the important researching issues in quantum optics. In 1956, Hanbury-Brown and Twiss (HBT) (Hanbury-Brown R, Twiss R Q 1956 Nature 177 27) revolutionized optical coherence and demonstrated a new form of photon correlation. The landmark experiment has far-reaching influenced and even inspired the quantum theory of optical coherence that Glauber developed to account for the conclusive observation by HBT. Ever since then, the HBT effect has motivated extensive studies of higher-order coherence and quantum statistics in quantum optics, as well as in quantum information science and cryptography. Based on the HBT scheme, the degree of coherence and photon number distribution of light field can be derived from correlation measurement and photon counting technique. With the rapid development of the photoelectric detection technology, single-photon detection, which is the most sensitive and very widespread method of optical measurement, is used to characterize the natures of light sources and indicate their differences. More recently, HBT scheme combined with single-photon detection was used to study spatial interference, ghost imaging, azimuthal interference effect, deterministic manipulation and detection of single-photon source, etc. Due to broadband RF spectrum, noiselike feature, hypersensitivity to the initial conditions and long-term unpredictability, chaotic laser meets the essential requirements for information security and cryptography, and has been developed in many applications such as chaos-based secure communications and physical random number generation, as well as public-channel secure key distribution. But the research mainly focused on macroscopic dynamics of the chaotic laser. Moreover, the precision of measurement has reached a quantum level at present. Quantum statistcs of light field can also uncover profoundly the physical nature of the light. Thus, it is important to exploit the higher-order degree of coherence and photon statistics of chaotic field, which contribute to characterizing the field and distinguishing it from others. In this paper, photon number distribution and second-order degree of coherence of a chaotic laser are analyzed and measured based on HBT scheme. The chaotic laser is composed of a distributed feedback laser diode with optical feedback in fiber external cavity configuration. The bandwidth of the chaotic laser that we obtain experimentally is 6.7 GHz. The photon number distribution of chaotic laser is fitted by Gaussian random distribution, Possionian distribution and Bose-Einstein distribution. With the increase of the mean photon number, the photon number distribution changes from Bose-Einstein distribution into Poissonian distribution and always accords with Gaussian random distribution well. The second-order coherence g(2)(0) drops gradually from 2 to 1. By changing the bias current (I = 1.0Ith-2.0Ith) and feedback strength (010%), we compare and illustrate different chaotic dynamics and g(2)(0). From low frequency fluctuation to coherence collapse, the chaotic laser shows bunching effect and fully chaotic field can be obtained at the broadest bandwidth. Furthermore, the physical explanation for sub-chaotic or weakening of bunching effect is provided. It is concluded that this method can well reveal photon statistics of chaotic laser and will open up an avenue to the research of chaos with quantum optics, which merges two important fields of modern physics and is extremely helpful for the high-speed remote chaotic communication.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2017
    Location Call Number Limitation Availability
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  • 4
    In: Acta Physica Sinica, Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences, Vol. 68, No. 8 ( 2019), p. 080301-
    Abstract: Solitons as self-supported solitary waves are one of the most fundamental objects in nonlinear science. With the realization of Bose-Einstein condensate, matter-wave solitons have aroused enormous interest due to their potential applications in atomic transport and atomic interferometer. In recent years, the artificial spin-orbit coupling has been realized in ultracold atoms, thus providing a new platform to study the nonlinear matter wave solitons under a gauge field, and a variety of novel soliton phenomena have been successively predicted. In this paper, we analyze the effects of linear Zeeman splitting on the dynamics of bright-bright solitons in spin-orbit coupled two-component Bose-Einstein condensate, via the variational approximation and the numerical simulation of Gross-Pitaevskii (GP) equations. For the SU(2) spin-rotational invariant attractive atomic interaction in a uniform case without external trap, we take a hyperbolic secant function as the variational Ansatz for bright soliton in variational approximation, and derive the Euler-Lagrange equations describing the evolution of the Ansatz parameters. By solving the time-independent Euler-Lagrange equations, we find two stationary solitons each with a finite momentum for a weak spin-orbit coupling due to the linear Zeeman splitting. Linearizing the Euler-Lagrange equations around these stationary solitons, we further obtain a zero-energy Goldstone mode and an oscillation mode with frequency related to linear Zeeman splitting: the former indicates that the continuous translational symmetry of the stationary solitons will be broken under a perturbation, and the later shows that the stationary solitons will oscillate under a perturbation. Furthermore, by solving the time-dependent Euler-Lagrange equations, we also obtain the exact full dynamical solutions of Ansatz parameters, and observe that the linear Zeeman splitting affects the period and velocity of soliton's oscillation and linear motion, which may provide a new method to control the dynamics of solitons. All the variational calculations are also confirmed directly by the numerical simulation of GP equations.
    Type of Medium: Online Resource
    ISSN: 1000-3290 , 1000-3290
    Language: Unknown
    Publisher: Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
    Publication Date: 2019
    Location Call Number Limitation Availability
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