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  • 1
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    First In-Situ Measurements of Plume Chemistry at Mount Garet Volcano, Island of Gaua (Vanuatu) (2020)
    MDPI
    Details
    Publication Date: 2020-11-25
    Description: Recent volcanic gas compilations have urged the need to expand in-situ plume measurements to poorly studied, remote volcanic regions. Despite being recognized as one of the main volcanic epicenters on the planet, the Vanuatu arc remains poorly characterized for its subaerial emissions and their chemical imprints. Here, we report on the first plume chemistry data for Mount Garet, on the island of Gaua, one of the few persistent volatile emitters along the Vanuatu arc. Data were collected with a multi-component gas analyzer system (multi-GAS) during a field campaign in December 2018. The average volcanic gas chemistry is characterized by mean molar CO2/SO2, H2O/SO2, H2S/SO2 and H2/SO2 ratios of 0.87, 47.2, 0.13 and 0.01, respectively. Molar proportions in the gas plume are estimated at 95.9 11.6, 1.8 0.5, 2.0 0.01, 0.26 0.02 and 0.06 0.01, for H2O, CO2, SO2, H2S and H2. Using the satellite-based 10-year (2005–2015) averaged SO2 flux of ~434 t d􀀀1 for Mt. Garet, we estimate a total volatile output of about 6482 t d􀀀1 (CO2 ~259 t d􀀀1; H2O ~5758 t d􀀀1; H2S ~30 t d􀀀1; H2 ~0.5 t d􀀀1). This may be representative of a quiescent, yet persistent degassing period at Mt. Garet; whilst, as indicated by SO2 flux reports for the 2009–2010 unrest, emissions can be much higher during eruptive episodes. Our estimated emission rates and gas composition for Mount Garet provide insightful information on volcanic gas signatures in the northernmost part of the Vanuatu Arc Segment. The apparent CO2-poor signature of high-temperature plume degassing at Mount Garet raises questions on the nature of sediments being subducted in this region of the arc and the possible role of the slab as the source of subaerial CO2. In order to better address the dynamics of along-arc volatile recycling, more volcanic gas surveys are needed focusing on northern Vanuatu volcanoes.
    Description: This research was conducted as part of the Trail by Fire II—Closing the Ring Project (PI: Y. Moussallam) funded by the National Geographic Society (grant number CP-122R-17), the Rolex Awards for Enterprise and the French national Research Institute for Development (IRD). J.L. also acknowledges travel funding support from Ministero dell’istruzione, dell’università e della ricerca (MIUR;) under grant n. PRIN2017-2017LMNLAW).
    Description: Published
    Description: id 7293
    Description: 4V. Processi pre-eruttivi
    Description: JCR Journal
    Keywords: Vanuatu ; Gaua ; Mount Garet ; Multi-GAS ; volcanic gas composition ; volatile fluxes ; 04.08. Volcanology
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 2
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    Characterisation of the magmatic signature in gas emissions from Turrialba Volcano, Costa Rica (2020)
    EGU - Copernicus
    Details
    Publication Date: 2020-11-25
    Description: The equilibrium composition of volcanic gaseswith their magma is often overprinted by interaction with ashallow hydrothermal system. Identifying the magmatic sig-nature of volcanic gases is critical to relate their composi-tion to properties of the magma (temperature,fO2, gas-meltsegregation depth). We report measurements of the chemi-cal composition and flux of the major gas species emittedfrom Turrialba Volcano during March 2013. Measurementswere made of two vents in the summit region, one of whichopened in 2010 and the other in 2012. We determined an av-erage SO2flux of 5.2±1.9 kg s−1using scanning ultravio-let spectroscopy, and molar proportions of H2O, CO2, SO2,HCl, CO and H2gases of 94.16, 4.03, 1.56, 0.23, 0.003 and0.009 % respectively by open-path Fourier transform infrared(FTIR) spectrometry and a multi-species gas-sensing system.Together, these data imply fluxes of 88, 8, 0.44, 5×10−3and1×10−3kg s−1for H2O, CO2, HCl, CO and H2respectively.Although H2S was detected, its concentration could not beresolved. HF was not detected. The chemical signature of thegas from both vents was found to be broadly similar. Follow-ing the opening of the 2010 and 2012 vents we found limitedto negligible interaction of the magmatic gas with the hy-drothermal system has occurred and the gas composition ofthe volcanic plume is broadly representative of equilibriumwith the magma. The time evolution of the gas composition,the continuous emission of large quantities of SO2, and thephysical evolution of the summit area with new vent open-ings and more frequent eruptions all point towards a continu-ous drying of the hydrothermal system at Turrialba’s summitat an apparently increasing rate.
    Description: This research was supported by the RoyalGeographical Society (with IBG) with a Geographical FieldworkGrant. Y. Moussallam and N. Peters were additionally supportedby the Philip Lake funds from the Department of Geography,University of Cambridge. Y. Moussallam acknowledges a researchgrant from Mazamas and support through ERC project #279790.We thank the NERC Field Spectroscopy Facility for the loanof their infrared spectrometer. A. Aiuppa acknowledges supportthrough ERC grant no. 305377 (BRIDGE)
    Description: Published
    Description: 1341–1350
    Description: 4V. Processi pre-eruttivi
    Description: JCR Journal
    Keywords: volcanic degassing ; Multi-GAS ; UV spectroscopy ; FTIR ; 04.08. Volcanology
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 3
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    Sustaining persistent lava lakes: Observations from high-resolution gas measurements at Villarrica volcano, Chile (2020)
    Elsevier
    Details
    Publication Date: 2020-11-25
    Description: Active lava lakes – as the exposed upper part of magmatic columns – are prime locations to investigate the conduit flow processes operating at active, degassing volcanoes. Persistent lava lakes require a constant influx of heat to sustain a molten state at the Earth's surface. Several mechanisms have been proposed to explain how such heat transfer can operate efficiently. These models make contrasting predictions with respect to the flow dynamics in volcanic conduits and should result in dissimilar volatile emissions at the surface. Here we look at high-frequency SO2 fluxes, plume composition, thermal emissions and aerial video footage from the Villarrica lava lake in order to determine the mechanism sustaining its activity. We found that while fluctuations are apparent in all datasets, none shows a stable periodic behaviour. These observations suggest a continuous influx of volatiles and magma to the Villarrica lava lake. We suggest that ascending volatile-rich and descending degassed magmas are efficiently mixed within the volcanic conduit, resulting in no clear periodic oscillations in the plume composition and flux. We compare our findings to those of other lava lakes where equivalent gas emission time-series have been acquired, and suggest that gas flux, magma viscosity and conduit geometry are key parameters determining which flow mechanism operates in a given volcanic conduit. The range of conduit flow regimes inferred from the few studied lava lakes gives a glimpse of the potentially wide spectrum of conduit flow dynamics operating at active volcanoes.
    Description: This research was conducted as part of the “Trail By Fire” expedition (PI: Y. Moussallam). The project was supported by the Royal Geographical Society (with the Institute of British Geographers) with the Land Rover Bursary; the Deep Carbon Observatory DECADE Initiative; Ocean Optics; Crowcon; Air Liquide; Thermo Fisher Scientific; Santander; Cactus Outdoor; Turbo Ace and Team Black Sheep. We thank Sebastien Carretier and Rose-Marie Ojeda together with IRD South-America personnel for all their logistical help. We further thank the CONAF and DGAC for their help. YM acknowledges support from the Scripps Institution of Oceanography Postdoctoral Fellowship program. CIS acknowledges a research startup grant from Victoria University of Wellington
    Description: Published
    Description: 237-247
    Description: 6V. Pericolosità vulcanica e contributi alla stima del rischio
    Description: JCR Journal
    Keywords: volcanic degassing ; Multi-GAS ; UAV ; Trail By Fire ; 04.08. Volcanology
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 4
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    Measurements of volcanic SO2 and CO2 fluxes by combined DOAS, Multi-GAS and FTIR observations: a case study from Turrialba and Telica volcanoes (2020)
    Springer
    Details
    Publication Date: 2020-11-25
    Description: Over the past few decades, substantial progress has been made to overcome the technical difficulties of continuously measuring volcanic SO2 emissions. However, measurements of CO2 emissions still present many difficulties, partly due to the lack of instruments that can directly measure CO2 emissions and partly due to its strong atmospheric background. In order to overcome these difficulties, a commonly taken approach is to combine differential optical absorption spectroscopy (DOAS) by using NOVAC scan-DOAS instruments for continuous measurements of crateric SO2 emissions, and electrochemical/NDIR multi-component gas analyser system (multi-GAS) instruments for measuring CO2/SO2 ratios of excerpts of the volcanic plume. This study aims to quantify the representativeness of excerpts of CO2/SO2 ratios measured by Multi-GAS as a fraction of the whole plume composition, by comparison with simultaneously measured CO2/SO2 ratios using cross-crater Fourier transform infrared spectroscopy (FTIR). Two study cases are presented: Telica volcano (Nicaragua), with a homogenous plume, quiescent degassing from a deep source and ambient temperature, and Turrialba volcano (Costa Rica), which has a non-homogeneous plume from three main sources with different compositions and temperatures. Our comparison shows that in our “easier case” (Telica), FTIR and Multi-GAS CO2/SO2 ratios agree within a factor about 3 %. In our “complicated case” (Turrialba), Multi-GAS and FTIR yield CO2/SO2 ratios differing by approximately 13–25 % at most. These results suggest that a fair estimation of volcanic CO2 emissions can be provided by the combination of DOAS and Multi-GAS instruments for volcanoes with similar degassing conditions as Telica or Turrialba. Based on the results of this comparison, we report that by the time our measurements were made, Telica and Turrialba were emitting approximately 100 and 1,000 t day−1 of CO2, respectively.
    Description: This work was supported by the Swedish International Development Agency (SIDA), and the DECADE initiative in coordination with OVSICORI-UNA and INETER. The research leading to these results received funding from the European Research Council under the European Union’s Seventh Framework Programme (FP7/2007/2013)/ERC grant agreement n1305377 (PI Aiuppa)
    Description: Published
    Description: 2335–2347
    Description: 4V. Processi pre-eruttivi
    Description: JCR Journal
    Keywords: volcanic degassing ; Multi-GAS ; UV spectroscopy ; FTIR
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 5
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    Degassing regime of Hekla volcano 2012–2013 (2020)
    Elsevier
    Details
    Publication Date: 2020-12-18
    Description: Hekla is a frequently active volcano with an infamously short pre-eruptive warning period. Our project contributes to the ongoing work on improving Hekla’s monitoring and early warning systems. In 2012 we began monitoring gas release at Hekla. The dataset comprises semi-permanent near-real time measurements with a MultiGAS system, quantification of diffuse gas flux, and direct samples analysed for composition and isotopes (δ13C, δD and δ18O). In addition, we used reaction path modelling to derive information on the origin and reaction pathways of the gas emissions. Hekla’s quiescent gas composition was CO2-dominated (0.8 mol fraction) and the δ13C signature was consistent with published values for Icelandic magmas. The gas is poor in H2O and S compared to hydrothermal manifestations and syn-eruptive emissions from other active volcanic systems in Iceland. The total CO2 flux from Hekla central volcano (diffuse soil emissions) is at least 44 T d−1, thereof 14 T d−1 are sourced from a small area at the volcano’s summit. There was no detectable gas flux at other craters, even though some of them had higher ground temperatures and had erupted more recently. Our measurements are consistent with a magma reservoir at depth coupled with a shallow dike beneath the summit. In the current quiescent state, the composition of the exsolved gas is substantially modified along its pathway to the surface through cooling and interaction with wall-rock and groundwater. The modification involves both significant H2O condensation and scrubbing of S-bearing species, leading to a CO2-dominated gas emitted at the summit. We conclude that a compositional shift towards more S- and H2O-rich gas compositions if measured in the future by the permanent MultiGAS station should be viewed as sign of imminent volcanic unrest on Hekla.
    Description: The research leading to these results has received funding from the Icelandic Centre for Research (RANNIS, grant number 110002-0031); the European Community’s Seventh Framework Programme under Grant Agreement No. 308377 (Project FUTUREVOLC); and the International Civil Aviation Organization.
    Description: Published
    Description: 80-99
    Description: 6V. Pericolosità vulcanica e contributi alla stima del rischio
    Description: JCR Journal
    Keywords: Hekla ; Multi-GAS ; degassing ; volcanic unrest ; 04.08. Volcanology
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 6
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    Terminal Strombolian activity at Etna’s central craters during summer 2012: The most CO2-rich volcanic gas ever recorded at Mount Etna (2023)
    The Geochemical Society of Japan
    Details
    Publication Date: 2023-01-20
    Description: Abstract By using a permanent network of multi-component gas analyzer systems (Multi-GAS), we report for the first time the H2O-CO2-SO2 composition of the volcanic gases emitted prior to, during, and after terminal Strombolian activity at Mount Etna’s central craters (CCs). We show that the summer 2012 Strombolian episodes of the Bocca Nuova crater (BNC), the largest of Etna’s CCs, are associated with the emission of the most CO2-rich gas measured at the volcano thus far. The BNC plume was particularly CO2-rich with CO2/SO2 up to 100, H2O/CO2 〈 1 in the quiescent periods between Strombolian episodes. However, more CO2-poor gas with CO2/SO2 〈 27, H2O/CO2 〉 1 prevailed at the BNC and at other degassing vents such as Voragine and Northeast craters during Strombolian eruptions. Based on the results of numerical simulations of volcanic degassing, conclude that the shallow Etna plumbing system was invaded in summer 2012 by a CO2-rich gas front likely supplied by the deep (〉100 MPa pressure) volcano’s magmatic storage zone. This deep gas-bubble supply eventually caused a general rejuvenation of the resident magma in the upper conduits/shallow reservoirs, thereby triggering the first Strombolian episodes on the volcano’s summit after years of quiescence.
    Description: Published
    Description: 123-138
    Description: 6V. Pericolosità vulcanica e contributi alla stima del rischio
    Description: JCR Journal
    Keywords: volcanic gases ; Etna ; degassing ; Multi-GAS ; volcano monitoring ; 04.08. Volcanology
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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